The potential of direct air capture using adsorbents in cold climates

Global warming threatens the entire planet, and solutions such as direct air capture (DAC) can be used to meet net-zero goals and go beyond. This study investigates using DAC in a 5-step temperature vacuum swing adsorption (TVSA) cycle with adsorbents’ Li-X and Na-X, readily available industrial zeo...

Full description

Bibliographic Details
Published in:iScience
Main Author: Wilson, Sean M.W.
Format: Text
Language:English
Published: Elsevier 2022
Subjects:
Online Access:http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9720019/
https://doi.org/10.1016/j.isci.2022.105564
id ftpubmed:oai:pubmedcentral.nih.gov:9720019
record_format openpolar
spelling ftpubmed:oai:pubmedcentral.nih.gov:9720019 2023-05-15T13:48:32+02:00 The potential of direct air capture using adsorbents in cold climates Wilson, Sean M.W. 2022-11-13 http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9720019/ https://doi.org/10.1016/j.isci.2022.105564 en eng Elsevier http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9720019/ http://dx.doi.org/10.1016/j.isci.2022.105564 © 2022 The Author(s) https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/). CC-BY-NC-ND iScience Article Text 2022 ftpubmed https://doi.org/10.1016/j.isci.2022.105564 2022-12-11T01:59:26Z Global warming threatens the entire planet, and solutions such as direct air capture (DAC) can be used to meet net-zero goals and go beyond. This study investigates using DAC in a 5-step temperature vacuum swing adsorption (TVSA) cycle with adsorbents’ Li-X and Na-X, readily available industrial zeolites, to capture and concentrate CO(2) from air in cold climates. From this study, we report that Na-X in cold conditions has the highest known CO(2) adsorption capacity in air of 2.54 mmol/g. This combined with Na-X's low CO(2) heat of adsorption, and fast uptake-rate in comparison to other benchmark materials, allowed for Na-X operating in cold conditions to have the lowest reported DAC operating energy of 1.1 MWh/tonCO(2). These findings from this study show the promise of this process in cold climates of Canada, Alaska, Greenland, and Antarctica to be part of the solution to global warming. Text Antarc* Antarctica Greenland Alaska PubMed Central (PMC) Canada Greenland iScience 25 12 105564
institution Open Polar
collection PubMed Central (PMC)
op_collection_id ftpubmed
language English
topic Article
spellingShingle Article
Wilson, Sean M.W.
The potential of direct air capture using adsorbents in cold climates
topic_facet Article
description Global warming threatens the entire planet, and solutions such as direct air capture (DAC) can be used to meet net-zero goals and go beyond. This study investigates using DAC in a 5-step temperature vacuum swing adsorption (TVSA) cycle with adsorbents’ Li-X and Na-X, readily available industrial zeolites, to capture and concentrate CO(2) from air in cold climates. From this study, we report that Na-X in cold conditions has the highest known CO(2) adsorption capacity in air of 2.54 mmol/g. This combined with Na-X's low CO(2) heat of adsorption, and fast uptake-rate in comparison to other benchmark materials, allowed for Na-X operating in cold conditions to have the lowest reported DAC operating energy of 1.1 MWh/tonCO(2). These findings from this study show the promise of this process in cold climates of Canada, Alaska, Greenland, and Antarctica to be part of the solution to global warming.
format Text
author Wilson, Sean M.W.
author_facet Wilson, Sean M.W.
author_sort Wilson, Sean M.W.
title The potential of direct air capture using adsorbents in cold climates
title_short The potential of direct air capture using adsorbents in cold climates
title_full The potential of direct air capture using adsorbents in cold climates
title_fullStr The potential of direct air capture using adsorbents in cold climates
title_full_unstemmed The potential of direct air capture using adsorbents in cold climates
title_sort potential of direct air capture using adsorbents in cold climates
publisher Elsevier
publishDate 2022
url http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9720019/
https://doi.org/10.1016/j.isci.2022.105564
geographic Canada
Greenland
geographic_facet Canada
Greenland
genre Antarc*
Antarctica
Greenland
Alaska
genre_facet Antarc*
Antarctica
Greenland
Alaska
op_source iScience
op_relation http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9720019/
http://dx.doi.org/10.1016/j.isci.2022.105564
op_rights © 2022 The Author(s)
https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
op_rightsnorm CC-BY-NC-ND
op_doi https://doi.org/10.1016/j.isci.2022.105564
container_title iScience
container_volume 25
container_issue 12
container_start_page 105564
_version_ 1766249408197820416