The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances
Slowly degradable, semivolatile organic compounds (SOCs) may undergo more than one volatilization-transport-deposition cycle through the atmosphere (multi-hopping). The significance of this process for the potential for long-range transport (LRT) is addressed for the first time. We use a multicompar...
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ftpubman:oai:pure.mpg.de:item_994927 2023-08-27T04:07:51+02:00 The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances Semeena, V. Lammel, G. 2005-04-05 application/pdf http://hdl.handle.net/11858/00-001M-0000-0011-FF04-4 http://hdl.handle.net/11858/00-001M-0000-0011-FF03-6 eng eng info:eu-repo/semantics/altIdentifier/doi/10.1029/2004GL022229, http://hdl.handle.net/11858/00-001M-0000-0011-FF04-4 http://hdl.handle.net/11858/00-001M-0000-0011-FF03-6 info:eu-repo/semantics/openAccess Geophysical Research Letters info:eu-repo/semantics/article 2005 ftpubman https://doi.org/10.1029/2004GL022229, 2023-08-02T01:34:53Z Slowly degradable, semivolatile organic compounds (SOCs) may undergo more than one volatilization-transport-deposition cycle through the atmosphere (multi-hopping). The significance of this process for the potential for long-range transport (LRT) is addressed for the first time. We use a multicompartment model which in turn is based on a general circulation model. The results suggest that both transport by single-hopping and multi-hopping contribute significantly to LRT of DDT and γ-HCH (lindane) and to accumulation in high latitudes. A larger fraction of the molecules transported by multi-hopping than of the molecules transported by single-hopping is deposited to the world's oceans. Multi-hopping prevails in the boundary layer far from the source regions. However, single-hopping contributes an almost equal amount to the deposition of DDT and γ-HCH in the Arctic. Article in Journal/Newspaper Arctic Max Planck Society: MPG.PuRe Arctic |
institution |
Open Polar |
collection |
Max Planck Society: MPG.PuRe |
op_collection_id |
ftpubman |
language |
English |
description |
Slowly degradable, semivolatile organic compounds (SOCs) may undergo more than one volatilization-transport-deposition cycle through the atmosphere (multi-hopping). The significance of this process for the potential for long-range transport (LRT) is addressed for the first time. We use a multicompartment model which in turn is based on a general circulation model. The results suggest that both transport by single-hopping and multi-hopping contribute significantly to LRT of DDT and γ-HCH (lindane) and to accumulation in high latitudes. A larger fraction of the molecules transported by multi-hopping than of the molecules transported by single-hopping is deposited to the world's oceans. Multi-hopping prevails in the boundary layer far from the source regions. However, single-hopping contributes an almost equal amount to the deposition of DDT and γ-HCH in the Arctic. |
format |
Article in Journal/Newspaper |
author |
Semeena, V. Lammel, G. |
spellingShingle |
Semeena, V. Lammel, G. The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
author_facet |
Semeena, V. Lammel, G. |
author_sort |
Semeena, V. |
title |
The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
title_short |
The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
title_full |
The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
title_fullStr |
The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
title_full_unstemmed |
The significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
title_sort |
significance of the grasshopper effect on the atmospheric distribution of persistent organic substances |
publishDate |
2005 |
url |
http://hdl.handle.net/11858/00-001M-0000-0011-FF04-4 http://hdl.handle.net/11858/00-001M-0000-0011-FF03-6 |
geographic |
Arctic |
geographic_facet |
Arctic |
genre |
Arctic |
genre_facet |
Arctic |
op_source |
Geophysical Research Letters |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.1029/2004GL022229, http://hdl.handle.net/11858/00-001M-0000-0011-FF04-4 http://hdl.handle.net/11858/00-001M-0000-0011-FF03-6 |
op_rights |
info:eu-repo/semantics/openAccess |
op_doi |
https://doi.org/10.1029/2004GL022229, |
_version_ |
1775348558663254016 |