Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere

The deposition of airborne microplastic particles, including those exceeding 1000 μm in the longest dimension, has been observed in the most remote places on earth. However, their deposition patterns are difficult to reproduce using current atmospheric transport models. These models usually treat pa...

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Published in:Environmental Science & Technology
Main Authors: Tatsii, D., Bucci, S., Bhowmick, T., Güttler, J., Bakels, L., Bagheri, G., Stohl, A.
Format: Article in Journal/Newspaper
Language:English
Published: 2024
Subjects:
Online Access:http://hdl.handle.net/21.11116/0000-000E-3B4D-B
http://hdl.handle.net/21.11116/0000-000E-3B4F-9
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spelling ftpubman:oai:pure.mpg.de:item_3562063 2024-02-11T10:01:25+01:00 Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere Tatsii, D. Bucci, S. Bhowmick, T. Güttler, J. Bakels, L. Bagheri, G. Stohl, A. 2024-01-09 application/pdf http://hdl.handle.net/21.11116/0000-000E-3B4D-B http://hdl.handle.net/21.11116/0000-000E-3B4F-9 eng eng info:eu-repo/grantAgreement/EC/H2020/675675 info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.est.3c08209 http://hdl.handle.net/21.11116/0000-000E-3B4D-B http://hdl.handle.net/21.11116/0000-000E-3B4F-9 info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by/4.0/ Environmental Science & Technology info:eu-repo/semantics/article 2024 ftpubman https://doi.org/10.1021/acs.est.3c08209 2024-01-22T00:47:33Z The deposition of airborne microplastic particles, including those exceeding 1000 μm in the longest dimension, has been observed in the most remote places on earth. However, their deposition patterns are difficult to reproduce using current atmospheric transport models. These models usually treat particles as perfect spheres, whereas the real shapes of microplastic particles are often far from spherical. Such particles experience lower settling velocities compared to volume equivalent spheres, leading to longer atmospheric transport. Here, we present novel laboratory experiments on the gravitational settling of microplastic fibers in air and find that their settling velocities are reduced by up to 76% compared to those of the spheres of the same volume. An atmospheric transport model constrained with the experimental data shows that shape-corrected settling velocities significantly increase the horizontal and vertical transport of particles. Our model results show that microplastic fibers of about 1 mm length emitted in populated areas are more likely to reach extremely remote regions of the globe, including the high Arctic, which is not the case for spheres of equivalent volume. We also calculate that fibers with lengths of up to 100 μm settle slowly enough to be lifted high into the stratosphere, where degradation by ultraviolet radiation may release chlorine and bromine, thus potentially damaging the stratospheric ozone layer. These findings suggest that the growing environmental burden and still increasing emissions of plastic pose multiple threats to life on earth. Article in Journal/Newspaper Arctic Max Planck Society: MPG.PuRe Arctic Environmental Science & Technology 58 1 671 682
institution Open Polar
collection Max Planck Society: MPG.PuRe
op_collection_id ftpubman
language English
description The deposition of airborne microplastic particles, including those exceeding 1000 μm in the longest dimension, has been observed in the most remote places on earth. However, their deposition patterns are difficult to reproduce using current atmospheric transport models. These models usually treat particles as perfect spheres, whereas the real shapes of microplastic particles are often far from spherical. Such particles experience lower settling velocities compared to volume equivalent spheres, leading to longer atmospheric transport. Here, we present novel laboratory experiments on the gravitational settling of microplastic fibers in air and find that their settling velocities are reduced by up to 76% compared to those of the spheres of the same volume. An atmospheric transport model constrained with the experimental data shows that shape-corrected settling velocities significantly increase the horizontal and vertical transport of particles. Our model results show that microplastic fibers of about 1 mm length emitted in populated areas are more likely to reach extremely remote regions of the globe, including the high Arctic, which is not the case for spheres of equivalent volume. We also calculate that fibers with lengths of up to 100 μm settle slowly enough to be lifted high into the stratosphere, where degradation by ultraviolet radiation may release chlorine and bromine, thus potentially damaging the stratospheric ozone layer. These findings suggest that the growing environmental burden and still increasing emissions of plastic pose multiple threats to life on earth.
format Article in Journal/Newspaper
author Tatsii, D.
Bucci, S.
Bhowmick, T.
Güttler, J.
Bakels, L.
Bagheri, G.
Stohl, A.
spellingShingle Tatsii, D.
Bucci, S.
Bhowmick, T.
Güttler, J.
Bakels, L.
Bagheri, G.
Stohl, A.
Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
author_facet Tatsii, D.
Bucci, S.
Bhowmick, T.
Güttler, J.
Bakels, L.
Bagheri, G.
Stohl, A.
author_sort Tatsii, D.
title Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
title_short Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
title_full Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
title_fullStr Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
title_full_unstemmed Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere
title_sort shape matters: long-range transport of microplastic fibers in the atmosphere
publishDate 2024
url http://hdl.handle.net/21.11116/0000-000E-3B4D-B
http://hdl.handle.net/21.11116/0000-000E-3B4F-9
geographic Arctic
geographic_facet Arctic
genre Arctic
genre_facet Arctic
op_source Environmental Science & Technology
op_relation info:eu-repo/grantAgreement/EC/H2020/675675
info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.est.3c08209
http://hdl.handle.net/21.11116/0000-000E-3B4D-B
http://hdl.handle.net/21.11116/0000-000E-3B4F-9
op_rights info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/4.0/
op_doi https://doi.org/10.1021/acs.est.3c08209
container_title Environmental Science & Technology
container_volume 58
container_issue 1
container_start_page 671
op_container_end_page 682
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