Stratospheric Aerosol Composition Observed by the Atmospheric Chemistry Experiment Following the 2019 Raikoke Eruption

• Main Authors: Boone, Chris D., Bernath, Peter F., Labelle, Keith, Crouse, Jeff
• Format: Article in Journal/Newspaper
• Language: unknown
• Published: ODU Digital Commons 2022
• Subjects: Aerosol; Composition; Sulfate; Volcanic eruption; Biological and Chemical Physics; Environmental Chemistry; Volcanology; Arctic
• Online Access: https://digitalcommons.odu.edu/chemistry_fac_pubs/229; https://digitalcommons.odu.edu/cgi/viewcontent.cgi?article=1233&context=chemistry_fac_pubs

Infrared aerosol spectra derived from Atmospheric Chemistry Experiment measurements following the June 2019 Raikoke volcanic eruption are used to evaluate the composition of stratospheric aerosols in the Arctic. A blanket of aerosols, spanning an altitude range from the tropopause (8–11 km) to 20 km, persisted in the stratosphere over northern latitudes for many months. The aerosols within this blanket were almost exclusively sulfates. The percentage of sulfuric acid in the aerosols decreased over time, dropping below 50% H2SO4 concentration at some altitudes by March 2020. Contrary to previous reports, the aerosol blanket was not comprised of smoke particles.