Wintertime Arctic Air Pollution over central Alaska: pre-ALPACA campaign

• Main Authors: Ioannidis, Eleftherios, Law, Kathy S., Raut, Jean-Christophe, Onishi, Tatsuo, Marelle, Louis, Roberts, Tjarda, J, Barret, Brice, d'Anna, Barbara, Temine-Roussel, Brice, Mölders, Nicole, Mao, Jingqiu, Simpson, William
• Other Authors: TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E), Observatoire des Sciences de l'Univers en région Centre (OSUC), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Centre National d’Études Spatiales Paris (CNES), Laboratoire d'aérologie (LAERO), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS), Laboratoire Chimie de l'environnement (LCE), Aix Marseille Université (AMU)-Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS), Geophysical Institute Fairbanks, University of Alaska Fairbanks (UAF)
• Format: Conference Object
• Language: English
• Published: HAL CCSD 2021
• Subjects: [SDE]Environmental Sciences; Arctic; Alaska
• Online Access: https://insu.hal.science/insu-03194235; https://insu.hal.science/insu-03194235/document; https://insu.hal.science/insu-03194235/file/EGU21-15477-print.pdf; https://doi.org/10.5194/egusphere-egu21-15477

International audience The wintertime Arctic is influenced by air pollution transported from mid-latitudes, leading to formation of Arctic Haze, as well as local emissions such as combustion for heating and power production in very cold winter conditions. This contributes to severe air pollution episodes, with enhanced aerosol concentrations, inter-dispersed with cleaner periods. However, the formation of secondary aerosol particles (sulphate, organics, nitrate) in cold/dark wintertime Arctic conditions, which could contribute to these pollution episodes, is poorly understood.In this study, which contributes to the Air Pollution in the Arctic: Climate, Environment and Societies - Alaskan Layered Pollution and Arctic Chemical Analysis (PACES-ALPACA) initiative, the Weather Research Forecasting Model with chemistry (WRF-Chem) is used to investigate wintertime pollution over central Alaska focusing on the Fairbanks region, during the pre-ALPACA campaign in winter 2019-2020. Fairbanks is the most polluted city in the United States during wintertime, due to high local emissions and the occurrence of strong surface temperature inversions trapping pollutants near the surface.Firstly, different WRF meteorological and surface schemes were tested over Alaska with a particular focus on improving simulations of the wintertime boundary layer structure including temperature inversions. An optimal WRF set-up, with increased vertical resolution below 2km, was selected based on evaluation against available data.Secondly, a quasi-hemispheric WRF-Chem simulation, using the improved WRF setup, was used to assess large-scale synoptic conditions and to evaluate background aerosols originating from remote anthropogenic and natural sources affecting central Alaska during the campaign. The model was run with Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants (ECLIPSE) v6b anthropogenic emissions and improved sea-spray aerosol emissions. Discrepancies in modelled aerosols compared available data are being ...