Exploring the uncertainties in the aviation soot–cirrus effect

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Righi, Mattia, Hendricks, Johannes, Beer, Christof Gerhard
• Format: Article in Journal/Newspaper
• Language: English
• Published: Copernicus Publications 2021
• Subjects: article; Verlagsveröffentlichung; Sea ice
• Online Access: https://doi.org/10.5194/acp-21-17267-2021; https://noa.gwlb.de/receive/cop_mods_00058966; https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00058576/acp-21-17267-2021.pdf; https://acp.copernicus.org/articles/21/17267/2021/acp-21-17267-2021.pdf

A global aerosol–climate model, including a two-moment cloud microphysical scheme and a parametrization for aerosol-induced ice formation in cirrus clouds, is applied in order to quantify the impact of aviation soot on natural cirrus clouds. Several sensitivity experiments are performed to assess the uncertainties in this effect related to (i) the assumptions on the ice nucleation abilities of aviation soot, (ii) the representation of vertical updrafts in the model, and (iii) the use of reanalysis data to relax the model dynamics (the so-called nudging technique). Based on the results of the model simulations, a radiative forcing from the aviation soot–cirrus effect in the range of −35 to 13 mW m−2 is quantified, depending on the assumed critical saturation ratio for ice nucleation and active fraction of aviation soot but with a confidence level below 95 % in several cases. Simple idealized experiments with prescribed vertical velocities further show that the uncertainties on this aspect of the model dynamics are critical for the investigated effect and could potentially add a factor of about 2 of further uncertainty to the model estimates of the resulting radiative forcing. The use of the nudging technique to relax model dynamics is proved essential in order to identify a statistically significant signal from the model internal variability, while simulations performed in free-running mode and with prescribed sea-surface temperatures and sea-ice concentrations are shown to be unable to provide robust estimates of the investigated effect. A comparison with analogous model studies on the aviation soot–cirrus effect show a very large model diversity, with a conspicuous lack of consensus across the various estimates, which points to the need for more in-depth analyses on the roots of such discrepancies.