Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion

We present methane (CH4) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH4 observations from 17 in situ and five dis...

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Published in:Atmospheric Chemistry and Physics
Main Authors: Thompson, Rona L., Sasakawa, Motoki, Machida, Toshinobu, Aalto, Tuula, Worthy, Doug, Lavric, Jost V., Lund Myhre, Cathrine, Stohl, Andreas
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2017
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Online Access:https://doi.org/10.5194/acp-17-3553-2017
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spelling ftnonlinearchiv:oai:noa.gwlb.de:cop_mods_00042636 2023-05-15T16:35:34+02:00 Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion Thompson, Rona L. Sasakawa, Motoki Machida, Toshinobu Aalto, Tuula Worthy, Doug Lavric, Jost V. Lund Myhre, Cathrine Stohl, Andreas 2017-03 electronic https://doi.org/10.5194/acp-17-3553-2017 https://noa.gwlb.de/receive/cop_mods_00042636 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00042256/acp-17-3553-2017.pdf https://acp.copernicus.org/articles/17/3553/2017/acp-17-3553-2017.pdf eng eng Copernicus Publications Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324 https://doi.org/10.5194/acp-17-3553-2017 https://noa.gwlb.de/receive/cop_mods_00042636 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00042256/acp-17-3553-2017.pdf https://acp.copernicus.org/articles/17/3553/2017/acp-17-3553-2017.pdf uneingeschränkt info:eu-repo/semantics/openAccess article Verlagsveröffentlichung article Text doc-type:article 2017 ftnonlinearchiv https://doi.org/10.5194/acp-17-3553-2017 2022-02-08T22:40:58Z We present methane (CH4) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH4 observations from 17 in situ and five discrete flask-sampling sites distributed over northern North America and Eurasia. CH4 fluxes are determined at monthly temporal resolution and on a variable grid with maximum resolution of 1° × 1°. Our inversion finds a CH4 source from the high northern latitudes of 82 to 84 Tg yr−1, constituting ∼ 15 % of the global total, compared to 64 to 68 Tg yr−1 (∼ 12 %) in the prior estimates. For northern North America, we estimate a mean source of 16.6 to 17.9 Tg yr−1, which is dominated by fluxes in the Hudson Bay Lowlands (HBL) and western Canada, specifically the province of Alberta. Our estimate for the HBL, of 2.7 to 3.4 Tg yr−1, is close to the prior estimate (which includes wetland fluxes from the land surface model, LPX-Bern) and to other independent inversion estimates. However, our estimate for Alberta, of 5.0 to 5.8 Tg yr−1, is significantly higher than the prior (which also includes anthropogenic sources from the EDGAR-4.2FT2010 inventory). Since the fluxes from this region persist throughout the winter, this may signify that the anthropogenic emissions are underestimated. For northern Eurasia, we find a mean source of 52.2 to 55.5 Tg yr−1, with a strong contribution from fluxes in the Western Siberian Lowlands (WSL) for which we estimate a source of 19.3 to 19.9 Tg yr−1. Over the 9-year inversion period, we find significant year-to-year variations in the fluxes, which in North America, and specifically in the HBL, appear to be driven at least in part by soil temperature, while in the WSL, the variability is more dependent on soil moisture. Moreover, we find significant positive trends in the CH4 fluxes in North America of 0.38 to 0.57 Tg yr−2, and northern Eurasia of 0.76 to 1.09 Tg yr−2. In North America, this could be due to an increase in soil temperature, while in North Eurasia, specifically Russia, the trend is likely due, at least in part, to an increase in anthropogenic sources. Article in Journal/Newspaper Hudson Bay Niedersächsisches Online-Archiv NOA Canada Hudson Hudson Bay Atmospheric Chemistry and Physics 17 5 3553 3572
institution Open Polar
collection Niedersächsisches Online-Archiv NOA
op_collection_id ftnonlinearchiv
language English
topic article
Verlagsveröffentlichung
spellingShingle article
Verlagsveröffentlichung
Thompson, Rona L.
Sasakawa, Motoki
Machida, Toshinobu
Aalto, Tuula
Worthy, Doug
Lavric, Jost V.
Lund Myhre, Cathrine
Stohl, Andreas
Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
topic_facet article
Verlagsveröffentlichung
description We present methane (CH4) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH4 observations from 17 in situ and five discrete flask-sampling sites distributed over northern North America and Eurasia. CH4 fluxes are determined at monthly temporal resolution and on a variable grid with maximum resolution of 1° × 1°. Our inversion finds a CH4 source from the high northern latitudes of 82 to 84 Tg yr−1, constituting ∼ 15 % of the global total, compared to 64 to 68 Tg yr−1 (∼ 12 %) in the prior estimates. For northern North America, we estimate a mean source of 16.6 to 17.9 Tg yr−1, which is dominated by fluxes in the Hudson Bay Lowlands (HBL) and western Canada, specifically the province of Alberta. Our estimate for the HBL, of 2.7 to 3.4 Tg yr−1, is close to the prior estimate (which includes wetland fluxes from the land surface model, LPX-Bern) and to other independent inversion estimates. However, our estimate for Alberta, of 5.0 to 5.8 Tg yr−1, is significantly higher than the prior (which also includes anthropogenic sources from the EDGAR-4.2FT2010 inventory). Since the fluxes from this region persist throughout the winter, this may signify that the anthropogenic emissions are underestimated. For northern Eurasia, we find a mean source of 52.2 to 55.5 Tg yr−1, with a strong contribution from fluxes in the Western Siberian Lowlands (WSL) for which we estimate a source of 19.3 to 19.9 Tg yr−1. Over the 9-year inversion period, we find significant year-to-year variations in the fluxes, which in North America, and specifically in the HBL, appear to be driven at least in part by soil temperature, while in the WSL, the variability is more dependent on soil moisture. Moreover, we find significant positive trends in the CH4 fluxes in North America of 0.38 to 0.57 Tg yr−2, and northern Eurasia of 0.76 to 1.09 Tg yr−2. In North America, this could be due to an increase in soil temperature, while in North Eurasia, specifically Russia, the trend is likely due, at least in part, to an increase in anthropogenic sources.
format Article in Journal/Newspaper
author Thompson, Rona L.
Sasakawa, Motoki
Machida, Toshinobu
Aalto, Tuula
Worthy, Doug
Lavric, Jost V.
Lund Myhre, Cathrine
Stohl, Andreas
author_facet Thompson, Rona L.
Sasakawa, Motoki
Machida, Toshinobu
Aalto, Tuula
Worthy, Doug
Lavric, Jost V.
Lund Myhre, Cathrine
Stohl, Andreas
author_sort Thompson, Rona L.
title Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_short Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_full Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_fullStr Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_full_unstemmed Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_sort methane fluxes in the high northern latitudes for 2005–2013 estimated using a bayesian atmospheric inversion
publisher Copernicus Publications
publishDate 2017
url https://doi.org/10.5194/acp-17-3553-2017
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https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00042256/acp-17-3553-2017.pdf
https://acp.copernicus.org/articles/17/3553/2017/acp-17-3553-2017.pdf
geographic Canada
Hudson
Hudson Bay
geographic_facet Canada
Hudson
Hudson Bay
genre Hudson Bay
genre_facet Hudson Bay
op_relation Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324
https://doi.org/10.5194/acp-17-3553-2017
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https://acp.copernicus.org/articles/17/3553/2017/acp-17-3553-2017.pdf
op_rights uneingeschränkt
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op_doi https://doi.org/10.5194/acp-17-3553-2017
container_title Atmospheric Chemistry and Physics
container_volume 17
container_issue 5
container_start_page 3553
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