Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements
Understanding the recent evolution of methane emissions in the Arctic is necessary to interpret the global methane cycle. Emissions are affected by significant uncertainties and are sensitive to climate change, leading to potential feedbacks. A polar version of the CHIMERE chemistry-transport model...
Published in: | Atmospheric Chemistry and Physics |
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2017
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ftnonlinearchiv:oai:noa.gwlb.de:cop_mods_00042333 2023-05-15T14:31:45+02:00 Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements Thonat, Thibaud Saunois, Marielle Bousquet, Philippe Pison, Isabelle Tan, Zeli Zhuang, Qianlai Crill, Patrick M. Thornton, Brett F. Bastviken, David Dlugokencky, Ed J. Zimov, Nikita Laurila, Tuomas Hatakka, Juha Hermansen, Ove Worthy, Doug E. J. 2017-07 electronic https://doi.org/10.5194/acp-17-8371-2017 https://noa.gwlb.de/receive/cop_mods_00042333 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041953/acp-17-8371-2017.pdf https://acp.copernicus.org/articles/17/8371/2017/acp-17-8371-2017.pdf eng eng Copernicus Publications Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324 https://doi.org/10.5194/acp-17-8371-2017 https://noa.gwlb.de/receive/cop_mods_00042333 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041953/acp-17-8371-2017.pdf https://acp.copernicus.org/articles/17/8371/2017/acp-17-8371-2017.pdf uneingeschränkt info:eu-repo/semantics/openAccess article Verlagsveröffentlichung article Text doc-type:article 2017 ftnonlinearchiv https://doi.org/10.5194/acp-17-8371-2017 2022-02-08T22:41:06Z Understanding the recent evolution of methane emissions in the Arctic is necessary to interpret the global methane cycle. Emissions are affected by significant uncertainties and are sensitive to climate change, leading to potential feedbacks. A polar version of the CHIMERE chemistry-transport model is used to simulate the evolution of tropospheric methane in the Arctic during 2012, including all known regional anthropogenic and natural sources, in particular freshwater emissions which are often overlooked in methane modelling. CHIMERE simulations are compared to atmospheric continuous observations at six measurement sites in the Arctic region. In winter, the Arctic is dominated by anthropogenic emissions; emissions from continental seepages and oceans, including from the East Siberian Arctic Shelf, can contribute significantly in more limited areas. In summer, emissions from wetland and freshwater sources dominate across the whole region. The model is able to reproduce the seasonality and synoptic variations of methane measured at the different sites. We find that all methane sources significantly affect the measurements at all stations at least at the synoptic scale, except for biomass burning. In particular, freshwater systems play a decisive part in summer, representing on average between 11 and 26 % of the simulated Arctic methane signal at the sites. This indicates the relevance of continuous observations to gain a mechanistic understanding of Arctic methane sources. Sensitivity tests reveal that the choice of the land-surface model used to prescribe wetland emissions can be critical in correctly representing methane mixing ratios. The closest agreement with the observations is reached when using the two wetland models which have emissions peaking in August–September, while all others reach their maximum in June–July. Such phasing provides an interesting constraint on wetland models which still have large uncertainties at present. Also testing different freshwater emission inventories leads to large differences in modelled methane. Attempts to include methane sinks (OH oxidation and soil uptake) reduced the model bias relative to observed atmospheric methane. The study illustrates how multiple sources, having different spatiotemporal dynamics and magnitudes, jointly influence the overall Arctic methane budget, and highlights ways towards further improved assessments. Article in Journal/Newspaper arctic methane Arctic Climate change Niedersächsisches Online-Archiv NOA Arctic Atmospheric Chemistry and Physics 17 13 8371 8394 |
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Niedersächsisches Online-Archiv NOA |
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ftnonlinearchiv |
language |
English |
topic |
article Verlagsveröffentlichung |
spellingShingle |
article Verlagsveröffentlichung Thonat, Thibaud Saunois, Marielle Bousquet, Philippe Pison, Isabelle Tan, Zeli Zhuang, Qianlai Crill, Patrick M. Thornton, Brett F. Bastviken, David Dlugokencky, Ed J. Zimov, Nikita Laurila, Tuomas Hatakka, Juha Hermansen, Ove Worthy, Doug E. J. Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
topic_facet |
article Verlagsveröffentlichung |
description |
Understanding the recent evolution of methane emissions in the Arctic is necessary to interpret the global methane cycle. Emissions are affected by significant uncertainties and are sensitive to climate change, leading to potential feedbacks. A polar version of the CHIMERE chemistry-transport model is used to simulate the evolution of tropospheric methane in the Arctic during 2012, including all known regional anthropogenic and natural sources, in particular freshwater emissions which are often overlooked in methane modelling. CHIMERE simulations are compared to atmospheric continuous observations at six measurement sites in the Arctic region. In winter, the Arctic is dominated by anthropogenic emissions; emissions from continental seepages and oceans, including from the East Siberian Arctic Shelf, can contribute significantly in more limited areas. In summer, emissions from wetland and freshwater sources dominate across the whole region. The model is able to reproduce the seasonality and synoptic variations of methane measured at the different sites. We find that all methane sources significantly affect the measurements at all stations at least at the synoptic scale, except for biomass burning. In particular, freshwater systems play a decisive part in summer, representing on average between 11 and 26 % of the simulated Arctic methane signal at the sites. This indicates the relevance of continuous observations to gain a mechanistic understanding of Arctic methane sources. Sensitivity tests reveal that the choice of the land-surface model used to prescribe wetland emissions can be critical in correctly representing methane mixing ratios. The closest agreement with the observations is reached when using the two wetland models which have emissions peaking in August–September, while all others reach their maximum in June–July. Such phasing provides an interesting constraint on wetland models which still have large uncertainties at present. Also testing different freshwater emission inventories leads to large differences in modelled methane. Attempts to include methane sinks (OH oxidation and soil uptake) reduced the model bias relative to observed atmospheric methane. The study illustrates how multiple sources, having different spatiotemporal dynamics and magnitudes, jointly influence the overall Arctic methane budget, and highlights ways towards further improved assessments. |
format |
Article in Journal/Newspaper |
author |
Thonat, Thibaud Saunois, Marielle Bousquet, Philippe Pison, Isabelle Tan, Zeli Zhuang, Qianlai Crill, Patrick M. Thornton, Brett F. Bastviken, David Dlugokencky, Ed J. Zimov, Nikita Laurila, Tuomas Hatakka, Juha Hermansen, Ove Worthy, Doug E. J. |
author_facet |
Thonat, Thibaud Saunois, Marielle Bousquet, Philippe Pison, Isabelle Tan, Zeli Zhuang, Qianlai Crill, Patrick M. Thornton, Brett F. Bastviken, David Dlugokencky, Ed J. Zimov, Nikita Laurila, Tuomas Hatakka, Juha Hermansen, Ove Worthy, Doug E. J. |
author_sort |
Thonat, Thibaud |
title |
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
title_short |
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
title_full |
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
title_fullStr |
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
title_full_unstemmed |
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements |
title_sort |
detectability of arctic methane sources at six sites performing continuous atmospheric measurements |
publisher |
Copernicus Publications |
publishDate |
2017 |
url |
https://doi.org/10.5194/acp-17-8371-2017 https://noa.gwlb.de/receive/cop_mods_00042333 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041953/acp-17-8371-2017.pdf https://acp.copernicus.org/articles/17/8371/2017/acp-17-8371-2017.pdf |
geographic |
Arctic |
geographic_facet |
Arctic |
genre |
arctic methane Arctic Climate change |
genre_facet |
arctic methane Arctic Climate change |
op_relation |
Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324 https://doi.org/10.5194/acp-17-8371-2017 https://noa.gwlb.de/receive/cop_mods_00042333 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041953/acp-17-8371-2017.pdf https://acp.copernicus.org/articles/17/8371/2017/acp-17-8371-2017.pdf |
op_rights |
uneingeschränkt info:eu-repo/semantics/openAccess |
op_doi |
https://doi.org/10.5194/acp-17-8371-2017 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
17 |
container_issue |
13 |
container_start_page |
8371 |
op_container_end_page |
8394 |
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1766305296806838272 |