Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms
The connection between marine biogenic dimethyl sulfide (DMS) and the formation of aerosol particles in the Arctic atmosphere was evaluated by analyzing atmospheric DMS mixing ratio, aerosol particle size distribution and aerosol chemical composition data that were concurrently collected at Ny-Ålesu...
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ftnonlinearchiv:oai:noa.gwlb.de:cop_mods_00042277 2023-05-15T14:39:37+02:00 Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms Park, Ki-Tae Jang, Sehyun Lee, Kitack Yoon, Young Jun Kim, Min-Seob Park, Kihong Cho, Hee-Joo Kang, Jung-Ho Udisti, Roberto Lee, Bang-Yong Shin, Kyung-Hoon 2017-08 electronic https://doi.org/10.5194/acp-17-9665-2017 https://noa.gwlb.de/receive/cop_mods_00042277 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041897/acp-17-9665-2017.pdf https://acp.copernicus.org/articles/17/9665/2017/acp-17-9665-2017.pdf eng eng Copernicus Publications Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324 https://doi.org/10.5194/acp-17-9665-2017 https://noa.gwlb.de/receive/cop_mods_00042277 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041897/acp-17-9665-2017.pdf https://acp.copernicus.org/articles/17/9665/2017/acp-17-9665-2017.pdf uneingeschränkt info:eu-repo/semantics/openAccess article Verlagsveröffentlichung article Text doc-type:article 2017 ftnonlinearchiv https://doi.org/10.5194/acp-17-9665-2017 2022-02-08T22:41:09Z The connection between marine biogenic dimethyl sulfide (DMS) and the formation of aerosol particles in the Arctic atmosphere was evaluated by analyzing atmospheric DMS mixing ratio, aerosol particle size distribution and aerosol chemical composition data that were concurrently collected at Ny-Ålesund, Svalbard (78.5° N, 11.8° E), during April and May 2015. Measurements of aerosol sulfur (S) compounds showed distinct patterns during periods of Arctic haze (April) and phytoplankton blooms (May). Specifically, during the phytoplankton bloom period the contribution of DMS-derived SO42− to the total aerosol SO42− increased by 7-fold compared with that during the proceeding Arctic haze period, and accounted for up to 70 % of fine SO42− particles (< 2.5 µm in diameter). The results also showed that the formation of submicron SO42− aerosols was significantly associated with an increase in the atmospheric DMS mixing ratio. More importantly, two independent estimates of the formation of DMS-derived SO42− aerosols, calculated using the stable S-isotope ratio and the non-sea-salt SO42− ∕ methanesulfonic acid ratio, respectively, were in close agreement, providing compelling evidence that the contribution of biogenic DMS to the formation of aerosol particles was substantial during the Arctic phytoplankton bloom period. Article in Journal/Newspaper Arctic Ny Ålesund Ny-Ålesund Phytoplankton Svalbard Niedersächsisches Online-Archiv NOA Arctic Ny-Ålesund Svalbard Atmospheric Chemistry and Physics 17 15 9665 9675 |
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Niedersächsisches Online-Archiv NOA |
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English |
topic |
article Verlagsveröffentlichung |
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article Verlagsveröffentlichung Park, Ki-Tae Jang, Sehyun Lee, Kitack Yoon, Young Jun Kim, Min-Seob Park, Kihong Cho, Hee-Joo Kang, Jung-Ho Udisti, Roberto Lee, Bang-Yong Shin, Kyung-Hoon Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
topic_facet |
article Verlagsveröffentlichung |
description |
The connection between marine biogenic dimethyl sulfide (DMS) and the formation of aerosol particles in the Arctic atmosphere was evaluated by analyzing atmospheric DMS mixing ratio, aerosol particle size distribution and aerosol chemical composition data that were concurrently collected at Ny-Ålesund, Svalbard (78.5° N, 11.8° E), during April and May 2015. Measurements of aerosol sulfur (S) compounds showed distinct patterns during periods of Arctic haze (April) and phytoplankton blooms (May). Specifically, during the phytoplankton bloom period the contribution of DMS-derived SO42− to the total aerosol SO42− increased by 7-fold compared with that during the proceeding Arctic haze period, and accounted for up to 70 % of fine SO42− particles (< 2.5 µm in diameter). The results also showed that the formation of submicron SO42− aerosols was significantly associated with an increase in the atmospheric DMS mixing ratio. More importantly, two independent estimates of the formation of DMS-derived SO42− aerosols, calculated using the stable S-isotope ratio and the non-sea-salt SO42− ∕ methanesulfonic acid ratio, respectively, were in close agreement, providing compelling evidence that the contribution of biogenic DMS to the formation of aerosol particles was substantial during the Arctic phytoplankton bloom period. |
format |
Article in Journal/Newspaper |
author |
Park, Ki-Tae Jang, Sehyun Lee, Kitack Yoon, Young Jun Kim, Min-Seob Park, Kihong Cho, Hee-Joo Kang, Jung-Ho Udisti, Roberto Lee, Bang-Yong Shin, Kyung-Hoon |
author_facet |
Park, Ki-Tae Jang, Sehyun Lee, Kitack Yoon, Young Jun Kim, Min-Seob Park, Kihong Cho, Hee-Joo Kang, Jung-Ho Udisti, Roberto Lee, Bang-Yong Shin, Kyung-Hoon |
author_sort |
Park, Ki-Tae |
title |
Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
title_short |
Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
title_full |
Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
title_fullStr |
Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
title_full_unstemmed |
Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms |
title_sort |
observational evidence for the formation of dms-derived aerosols during arctic phytoplankton blooms |
publisher |
Copernicus Publications |
publishDate |
2017 |
url |
https://doi.org/10.5194/acp-17-9665-2017 https://noa.gwlb.de/receive/cop_mods_00042277 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041897/acp-17-9665-2017.pdf https://acp.copernicus.org/articles/17/9665/2017/acp-17-9665-2017.pdf |
geographic |
Arctic Ny-Ålesund Svalbard |
geographic_facet |
Arctic Ny-Ålesund Svalbard |
genre |
Arctic Ny Ålesund Ny-Ålesund Phytoplankton Svalbard |
genre_facet |
Arctic Ny Ålesund Ny-Ålesund Phytoplankton Svalbard |
op_relation |
Atmospheric Chemistry and Physics -- http://www.atmos-chem-phys.net/volumes_and_issues.html -- http://www.bibliothek.uni-regensburg.de/ezeit/?2069847 -- 1680-7324 https://doi.org/10.5194/acp-17-9665-2017 https://noa.gwlb.de/receive/cop_mods_00042277 https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00041897/acp-17-9665-2017.pdf https://acp.copernicus.org/articles/17/9665/2017/acp-17-9665-2017.pdf |
op_rights |
uneingeschränkt info:eu-repo/semantics/openAccess |
op_doi |
https://doi.org/10.5194/acp-17-9665-2017 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
17 |
container_issue |
15 |
container_start_page |
9665 |
op_container_end_page |
9675 |
_version_ |
1766311581798367232 |