On the Identification of Ozone Recovery

As ozone depleting substances decline, stratospheric ozone is displaying signs of healing in the Antarctic lower stratosphere. Here we focus on higher altitudes and the global stratosphere. Two key processes that can influence ozone recovery are evaluated: dynamical variability and solar proton even...

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Published in:Geophysical Research Letters
Main Authors: Stone, Kane Adam, Solomon, Susan, Kinnison, Douglas E.
Other Authors: Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences, Massachusetts Institute of Technology. Department of Chemistry
Format: Article in Journal/Newspaper
Language:English
Published: American Geophysical Union (AGU) 2018
Subjects:
Online Access:https://hdl.handle.net/1721.1/122774
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spelling ftmit:oai:dspace.mit.edu:1721.1/122774 2023-06-11T04:06:00+02:00 On the Identification of Ozone Recovery Stone, Kane Adam Solomon, Susan Kinnison, Douglas E. Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences Massachusetts Institute of Technology. Department of Chemistry Solomon, Susan 2018-05 application/pdf https://hdl.handle.net/1721.1/122774 en_US eng American Geophysical Union (AGU) http://dx.doi.org/10.1029/2018gl077955 Geophysical Research Letters 0094-8276 https://hdl.handle.net/1721.1/122774 Stone, Kane A. et al. “On the Identification of Ozone Recovery.” Geophysical Research Letters 45, 10 (May 2018): 5158–5165 © 2018 American Geophysical Union Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. Prof. Solomon via Chris Sherratt Article http://purl.org/eprint/type/JournalArticle 2018 ftmit https://doi.org/10.1029/2018gl077955 2023-05-29T07:29:08Z As ozone depleting substances decline, stratospheric ozone is displaying signs of healing in the Antarctic lower stratosphere. Here we focus on higher altitudes and the global stratosphere. Two key processes that can influence ozone recovery are evaluated: dynamical variability and solar proton events (SPEs). A nine‐member ensemble of free‐running simulations indicates that dynamical variability dominates the relatively small ozone recovery signal over 1998–2016 in the subpolar lower stratosphere, particularly near the tropical tropopause. The absence of observed recovery there to date is therefore not unexpected. For the upper stratosphere, high latitudes (50–80°N/S) during autumn and winter show the largest recovery. Large halogen‐induced odd oxygen loss there provides a fingerprint of seasonal sensitivity to chlorine trends. However, we show that SPEs also have a profound effect on ozone trends within this region since 2000. Thus, accounting for SPEs is important for detection of recovery in the upper stratosphere. Keywords: ozone; recovery; stratosphere; variability National Science Foundation (Grant ACD-1539972) Article in Journal/Newspaper Antarc* Antarctic DSpace@MIT (Massachusetts Institute of Technology) Antarctic The Antarctic Geophysical Research Letters 45 10 5158 5165
institution Open Polar
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language English
description As ozone depleting substances decline, stratospheric ozone is displaying signs of healing in the Antarctic lower stratosphere. Here we focus on higher altitudes and the global stratosphere. Two key processes that can influence ozone recovery are evaluated: dynamical variability and solar proton events (SPEs). A nine‐member ensemble of free‐running simulations indicates that dynamical variability dominates the relatively small ozone recovery signal over 1998–2016 in the subpolar lower stratosphere, particularly near the tropical tropopause. The absence of observed recovery there to date is therefore not unexpected. For the upper stratosphere, high latitudes (50–80°N/S) during autumn and winter show the largest recovery. Large halogen‐induced odd oxygen loss there provides a fingerprint of seasonal sensitivity to chlorine trends. However, we show that SPEs also have a profound effect on ozone trends within this region since 2000. Thus, accounting for SPEs is important for detection of recovery in the upper stratosphere. Keywords: ozone; recovery; stratosphere; variability National Science Foundation (Grant ACD-1539972)
author2 Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
Massachusetts Institute of Technology. Department of Chemistry
Solomon, Susan
format Article in Journal/Newspaper
author Stone, Kane Adam
Solomon, Susan
Kinnison, Douglas E.
spellingShingle Stone, Kane Adam
Solomon, Susan
Kinnison, Douglas E.
On the Identification of Ozone Recovery
author_facet Stone, Kane Adam
Solomon, Susan
Kinnison, Douglas E.
author_sort Stone, Kane Adam
title On the Identification of Ozone Recovery
title_short On the Identification of Ozone Recovery
title_full On the Identification of Ozone Recovery
title_fullStr On the Identification of Ozone Recovery
title_full_unstemmed On the Identification of Ozone Recovery
title_sort on the identification of ozone recovery
publisher American Geophysical Union (AGU)
publishDate 2018
url https://hdl.handle.net/1721.1/122774
geographic Antarctic
The Antarctic
geographic_facet Antarctic
The Antarctic
genre Antarc*
Antarctic
genre_facet Antarc*
Antarctic
op_source Prof. Solomon via Chris Sherratt
op_relation http://dx.doi.org/10.1029/2018gl077955
Geophysical Research Letters
0094-8276
https://hdl.handle.net/1721.1/122774
Stone, Kane A. et al. “On the Identification of Ozone Recovery.” Geophysical Research Letters 45, 10 (May 2018): 5158–5165 © 2018 American Geophysical Union
op_rights Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.
op_doi https://doi.org/10.1029/2018gl077955
container_title Geophysical Research Letters
container_volume 45
container_issue 10
container_start_page 5158
op_container_end_page 5165
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