Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements
The SPIRALE and SWIR balloon-borne instruments have been launched in the Arctic polar region (near Kiruna, Sweden, 67.9° N, 21.1° E) during summer on 7 and 24 August 2009 and on 14 August 2009, respectively. The SPIRALE instrument performed in situ measurements of several trace gases including CO an...
Published in: | Atmospheric Chemistry and Physics |
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Main Authors: | , , , , , , , , , , , , , |
Other Authors: | , , , , , , , , , , , , , , , , , , , , , |
Format: | Article in Journal/Newspaper |
Language: | English |
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HAL CCSD
2012
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Online Access: | https://hal.science/hal-00709289 https://hal.science/hal-00709289/document https://hal.science/hal-00709289/file/acp-12-11889-2012.pdf https://doi.org/10.5194/acp-12-11889-2012 |
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Météo-France: HAL |
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language |
English |
topic |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDE.MCG]Environmental Sciences/Global Changes |
spellingShingle |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDE.MCG]Environmental Sciences/Global Changes Krysztofiak, G. Thiéblemont, Rémi Huret, Nathalie Catoire, Valéry Té, Y. Jégou, Fabrice Coheur, Pierre-François Clerbaux, Cathy Payan, Sébastien Drouin, M. A. Robert, Claude Jeseck, P. Attié, Jean-Luc Camy-Peyret, Claude Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
topic_facet |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDE.MCG]Environmental Sciences/Global Changes |
description |
The SPIRALE and SWIR balloon-borne instruments have been launched in the Arctic polar region (near Kiruna, Sweden, 67.9° N, 21.1° E) during summer on 7 and 24 August 2009 and on 14 August 2009, respectively. The SPIRALE instrument performed in situ measurements of several trace gases including CO and O 3 between 9 and 34 km height, with very high vertical resolution (~5 m). The SWIR-balloon instrument measured total and partial column of several species including CO. The CO stratospheric profile from SPIRALE on 7 August 2009 shows some specific structures with strong abundance of CO in the low levels (potential temperatures between 320 and 380 K, i.e. 10-14 km height). These structures are not present in the CO vertical profile of SPIRALE on 24 August 2009, for which the volume mixing ratios are typical from polar latitudes (~30 ppb). CO total columns retrieved from the IASI-MetOp satellite sounder for the three dates of flights are used to understand this spatial and temporal CO variability. SPIRALE and SWIR CO partial columns between 9 and 34 km are compared, allowing us to confirm that the enhancement of CO is localised in the stratosphere. The measurements are investigated also in terms of CO:O 3 correlations and with the help of several modelling approaches (trajectory calculations, potential vorticity fields, results of chemistry transport model), in order to characterize the origin of the air masses sampled. The emission sources are qualified in terms of source type (fires, urban pollution) using NH 3 and CO measurements from IASI-MetOp and MODIS data on board the TERRA/AQUA satellite. The results give strong evidence that the unusual abundance of CO on 7 August is due to surface pollution plumes from East Asia and North America transported to the upper troposphere and then entering the lower stratosphere by isentropic advection. This study highlights that the composition of low polar stratosphere in summer can be affected by anthropogenic surface emissions through long range transport. |
author2 |
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E) Observatoire des Sciences de l'Univers en région Centre (OSUC) Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Centre National d’Études Spatiales Paris (CNES) Laboratoire de Physique Moleculaire pour l'Atmosphere et l'Astrophysique (LPMAA) Université Pierre et Marie Curie - Paris 6 (UPMC)-Centre National de la Recherche Scientifique (CNRS) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) Centre national de recherches météorologiques (CNRM) Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) ANR-08-BLAN-0300,StraPolEté,Dynamique, aérosols et brome dans la stratosphère polaire en été(2008) |
format |
Article in Journal/Newspaper |
author |
Krysztofiak, G. Thiéblemont, Rémi Huret, Nathalie Catoire, Valéry Té, Y. Jégou, Fabrice Coheur, Pierre-François Clerbaux, Cathy Payan, Sébastien Drouin, M. A. Robert, Claude Jeseck, P. Attié, Jean-Luc Camy-Peyret, Claude |
author_facet |
Krysztofiak, G. Thiéblemont, Rémi Huret, Nathalie Catoire, Valéry Té, Y. Jégou, Fabrice Coheur, Pierre-François Clerbaux, Cathy Payan, Sébastien Drouin, M. A. Robert, Claude Jeseck, P. Attié, Jean-Luc Camy-Peyret, Claude |
author_sort |
Krysztofiak, G. |
title |
Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
title_short |
Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
title_full |
Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
title_fullStr |
Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
title_full_unstemmed |
Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements |
title_sort |
detection in the summer polar stratosphere of pollution plume from east asia and north america by balloon-borne in situ co measurements |
publisher |
HAL CCSD |
publishDate |
2012 |
url |
https://hal.science/hal-00709289 https://hal.science/hal-00709289/document https://hal.science/hal-00709289/file/acp-12-11889-2012.pdf https://doi.org/10.5194/acp-12-11889-2012 |
genre |
Arctic Kiruna |
genre_facet |
Arctic Kiruna |
op_source |
ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00709289 Atmospheric Chemistry and Physics, 2012, 12 (24), pp.11889-11906. ⟨10.5194/acp-12-11889-2012⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-12-11889-2012 hal-00709289 https://hal.science/hal-00709289 https://hal.science/hal-00709289/document https://hal.science/hal-00709289/file/acp-12-11889-2012.pdf doi:10.5194/acp-12-11889-2012 |
op_rights |
http://creativecommons.org/licenses/by-nc-nd/ info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.5194/acp-12-11889-2012 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
12 |
container_issue |
24 |
container_start_page |
11889 |
op_container_end_page |
11906 |
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1799476009061318656 |
spelling |
ftmeteofrance:oai:HAL:hal-00709289v1 2024-05-19T07:36:52+00:00 Detection in the summer polar stratosphere of pollution plume from East Asia and North America by balloon-borne in situ CO measurements Krysztofiak, G. Thiéblemont, Rémi Huret, Nathalie Catoire, Valéry Té, Y. Jégou, Fabrice Coheur, Pierre-François Clerbaux, Cathy Payan, Sébastien Drouin, M. A. Robert, Claude Jeseck, P. Attié, Jean-Luc Camy-Peyret, Claude Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E) Observatoire des Sciences de l'Univers en région Centre (OSUC) Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Centre National d’Études Spatiales Paris (CNES) Laboratoire de Physique Moleculaire pour l'Atmosphere et l'Astrophysique (LPMAA) Université Pierre et Marie Curie - Paris 6 (UPMC)-Centre National de la Recherche Scientifique (CNRS) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) Centre national de recherches météorologiques (CNRM) Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) ANR-08-BLAN-0300,StraPolEté,Dynamique, aérosols et brome dans la stratosphère polaire en été(2008) 2012 https://hal.science/hal-00709289 https://hal.science/hal-00709289/document https://hal.science/hal-00709289/file/acp-12-11889-2012.pdf https://doi.org/10.5194/acp-12-11889-2012 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-12-11889-2012 hal-00709289 https://hal.science/hal-00709289 https://hal.science/hal-00709289/document https://hal.science/hal-00709289/file/acp-12-11889-2012.pdf doi:10.5194/acp-12-11889-2012 http://creativecommons.org/licenses/by-nc-nd/ info:eu-repo/semantics/OpenAccess ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00709289 Atmospheric Chemistry and Physics, 2012, 12 (24), pp.11889-11906. ⟨10.5194/acp-12-11889-2012⟩ [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDE.MCG]Environmental Sciences/Global Changes info:eu-repo/semantics/article Journal articles 2012 ftmeteofrance https://doi.org/10.5194/acp-12-11889-2012 2024-04-25T00:45:50Z The SPIRALE and SWIR balloon-borne instruments have been launched in the Arctic polar region (near Kiruna, Sweden, 67.9° N, 21.1° E) during summer on 7 and 24 August 2009 and on 14 August 2009, respectively. The SPIRALE instrument performed in situ measurements of several trace gases including CO and O 3 between 9 and 34 km height, with very high vertical resolution (~5 m). The SWIR-balloon instrument measured total and partial column of several species including CO. The CO stratospheric profile from SPIRALE on 7 August 2009 shows some specific structures with strong abundance of CO in the low levels (potential temperatures between 320 and 380 K, i.e. 10-14 km height). These structures are not present in the CO vertical profile of SPIRALE on 24 August 2009, for which the volume mixing ratios are typical from polar latitudes (~30 ppb). CO total columns retrieved from the IASI-MetOp satellite sounder for the three dates of flights are used to understand this spatial and temporal CO variability. SPIRALE and SWIR CO partial columns between 9 and 34 km are compared, allowing us to confirm that the enhancement of CO is localised in the stratosphere. The measurements are investigated also in terms of CO:O 3 correlations and with the help of several modelling approaches (trajectory calculations, potential vorticity fields, results of chemistry transport model), in order to characterize the origin of the air masses sampled. The emission sources are qualified in terms of source type (fires, urban pollution) using NH 3 and CO measurements from IASI-MetOp and MODIS data on board the TERRA/AQUA satellite. The results give strong evidence that the unusual abundance of CO on 7 August is due to surface pollution plumes from East Asia and North America transported to the upper troposphere and then entering the lower stratosphere by isentropic advection. This study highlights that the composition of low polar stratosphere in summer can be affected by anthropogenic surface emissions through long range transport. Article in Journal/Newspaper Arctic Kiruna Météo-France: HAL Atmospheric Chemistry and Physics 12 24 11889 11906 |