Carbon monoxide transport in the Arctic: A joint study using IASI satellite and aircraft data in spring and summer 2008

• Main Authors: Pommier, Matthieu, Law, Kathy S., Clerbaux, Cathy, Turquety, Solène, Hadji-Lazaro, Juliette, Hurtmans, Daniel, Coheur, Pierre-François, Schlager, H., Ancellet, Gérard, Paris, Jean-Daniel, Nédelec, Philippe, Diskin, Glenn S., Podolske, James R., Bernath, Peter
• Other Authors: TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL), Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique, Université libre de Bruxelles (ULB), DLR Institut für Physik der Atmosphäre = DLR Institute of Atmospheric Physics (IPA), Deutsches Zentrum für Luft- und Raumfahrt Oberpfaffenhofen-Wessling (DLR), Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA), Laboratoire d'aérologie (LAERO), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS), NASA Langley Research Center Hampton (LaRC), NASA Ames Research Center (ARC), Department of Chemistry Waterloo, University of Waterloo Waterloo
• Format: Conference Object
• Language: English
• Published: HAL CCSD 2009
• Subjects: [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph]; Arctic; Kiruna; Canada; Greenland; Kangerlussuaq; Inca; Climate change; IPY; Siberia
• Online Access: https://hal.science/hal-00440838

International audience Carbon monoxide (CO) is a reactive toxic gas, mainly produced by the combustion of fossil fuels and vegetation burning. It also plays an important role in the budget of tropospheric ozone and can be used a tracer for transport of sources of different origin. The impact of the transport of such pollutants on climate change in the Arctic still remains to be quantified with global models often failing to reproduce seasonal cycles especially in summertime. One possible explanation is the underestimation of modelled ozone production in forest fires plumes. This study focuses on the analysis of the POLARCAT/IPY spring and summer campaigns which took place, in Kiruna, Sweden in April 2008 and in Kangerlussuaq, Greenland in July 2008. During the campaigns different air masses were sampled including clean air, polluted plumes originating from anthropogenic sources in Europe and North America, and forest fire plumes from Siberia and Canada. These different transport pathways were well observed by the IASI (Infrared Atmospheric Sounding Interferometer) interferometer, onboard the METOP-A satellite. Measurements of CO collected by the ATR-42 aircraft as part of POLARCAT-France have been used to validate the satellite measurements. Furthermore, a more general validation procedure was developed to compare IASI with ATR-42, DLR-Falcon, NASA DC-8 and NOAA P3-B CO data. YAK summer flights in Siberia are also available for these comparisons. Both in-situ and satellite data are also compared to simulations from the LMDz-INCA global chemistry model. We will discuss how the good global coverage of IASI and regional flights allow can be used improve estimates of CO emissions and to evaluate the impact of forest fires on CO and O 3 (ozone) distributions.