Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska
Loss of sea ice is opening the Arctic to increasing development involving oil and gas extraction and shipping. Given the significant impacts of absorbing aerosol and secondary aerosol precursors emitted within the rapidly warming Arctic region, it is necessary to characterize local anthropogenic aer...
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ftleibnizopen:oai:oai.leibnizopen.de:sRN2DYsBBwLIz6xG7fC2 2023-11-05T03:38:52+01:00 Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska Gunsch, Matthew J. Kirpes, Rachel M. Kolesar, Katheryn R. Barrett, Tate E. China, Swarup Sheesley, Rebecca J. Laskin, Alexander Wiedensohler, Alfred Tuch, Thomas Pratt, Kerri A. 2017 application/pdf https://oa.tib.eu/renate/handle/123456789/11927 https://doi.org/10.34657/10960 eng eng Katlenburg-Lindau : EGU CC BY 3.0 Unported https://creativecommons.org/licenses/by/3.0 Atmospheric Chemistry and Physics 17 (2017), Nr. 17 aerosol atmospheric transport carbon emission chemical composition oil field particle size scanning electron microscopy size distribution X-ray spectroscopy Alaska Barrow Prudhoe Bay United States 550 article Text 2017 ftleibnizopen https://doi.org/10.34657/10960 2023-10-08T23:17:50Z Loss of sea ice is opening the Arctic to increasing development involving oil and gas extraction and shipping. Given the significant impacts of absorbing aerosol and secondary aerosol precursors emitted within the rapidly warming Arctic region, it is necessary to characterize local anthropogenic aerosol sources and compare to natural conditions. From August to September 2015 in Utqiaġvik (Barrow), AK, the chemical composition of individual atmospheric particles was measured by computer-controlled scanning electron microscopy with energy-dispersive X-ray spectroscopy (0.13-4 μm projected area diameter) and real-time single-particle mass spectrometry (0.2-1.5 μm vacuum aerodynamic diameter). During periods influenced by the Arctic Ocean (70 % of the study), our results show that fresh sea spray aerosol contributed ∼ 20 %, by number, of particles between 0.13 and 0.4 μm, 40-70 % between 0.4 and 1 μm, and 80-100 % between 1 and 4 μm particles. In contrast, for periods influenced by emissions from Prudhoe Bay (10 % of the study), the third largest oil field in North America, there was a strong influence from submicron (0.13-1 μm) combustion-derived particles (20-50 % organic carbon, by number; 5-10 % soot by number). While sea spray aerosol still comprised a large fraction of particles (90 % by number from 1 to 4 μm) detected under Prudhoe Bay influence, these particles were internally mixed with sulfate and nitrate indicative of aging processes during transport. In addition, the overall mode of the particle size number distribution shifted from 76 nm during Arctic Ocean influence to 27 nm during Prudhoe Bay influence, with particle concentrations increasing from 130 to 920 cm-3 due to transported particle emissions from the oil fields. The increased contributions of carbonaceous combustion products and partially aged sea spray aerosol should be considered in future Arctic atmospheric composition and climate simulations. publishedVersion Article in Journal/Newspaper Arctic Arctic Ocean Barrow Prudhoe Bay Sea ice Alaska LeibnizOpen (The Leibniz Association) |
institution |
Open Polar |
collection |
LeibnizOpen (The Leibniz Association) |
op_collection_id |
ftleibnizopen |
language |
English |
topic |
aerosol atmospheric transport carbon emission chemical composition oil field particle size scanning electron microscopy size distribution X-ray spectroscopy Alaska Barrow Prudhoe Bay United States 550 |
spellingShingle |
aerosol atmospheric transport carbon emission chemical composition oil field particle size scanning electron microscopy size distribution X-ray spectroscopy Alaska Barrow Prudhoe Bay United States 550 Gunsch, Matthew J. Kirpes, Rachel M. Kolesar, Katheryn R. Barrett, Tate E. China, Swarup Sheesley, Rebecca J. Laskin, Alexander Wiedensohler, Alfred Tuch, Thomas Pratt, Kerri A. Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
topic_facet |
aerosol atmospheric transport carbon emission chemical composition oil field particle size scanning electron microscopy size distribution X-ray spectroscopy Alaska Barrow Prudhoe Bay United States 550 |
description |
Loss of sea ice is opening the Arctic to increasing development involving oil and gas extraction and shipping. Given the significant impacts of absorbing aerosol and secondary aerosol precursors emitted within the rapidly warming Arctic region, it is necessary to characterize local anthropogenic aerosol sources and compare to natural conditions. From August to September 2015 in Utqiaġvik (Barrow), AK, the chemical composition of individual atmospheric particles was measured by computer-controlled scanning electron microscopy with energy-dispersive X-ray spectroscopy (0.13-4 μm projected area diameter) and real-time single-particle mass spectrometry (0.2-1.5 μm vacuum aerodynamic diameter). During periods influenced by the Arctic Ocean (70 % of the study), our results show that fresh sea spray aerosol contributed ∼ 20 %, by number, of particles between 0.13 and 0.4 μm, 40-70 % between 0.4 and 1 μm, and 80-100 % between 1 and 4 μm particles. In contrast, for periods influenced by emissions from Prudhoe Bay (10 % of the study), the third largest oil field in North America, there was a strong influence from submicron (0.13-1 μm) combustion-derived particles (20-50 % organic carbon, by number; 5-10 % soot by number). While sea spray aerosol still comprised a large fraction of particles (90 % by number from 1 to 4 μm) detected under Prudhoe Bay influence, these particles were internally mixed with sulfate and nitrate indicative of aging processes during transport. In addition, the overall mode of the particle size number distribution shifted from 76 nm during Arctic Ocean influence to 27 nm during Prudhoe Bay influence, with particle concentrations increasing from 130 to 920 cm-3 due to transported particle emissions from the oil fields. The increased contributions of carbonaceous combustion products and partially aged sea spray aerosol should be considered in future Arctic atmospheric composition and climate simulations. publishedVersion |
format |
Article in Journal/Newspaper |
author |
Gunsch, Matthew J. Kirpes, Rachel M. Kolesar, Katheryn R. Barrett, Tate E. China, Swarup Sheesley, Rebecca J. Laskin, Alexander Wiedensohler, Alfred Tuch, Thomas Pratt, Kerri A. |
author_facet |
Gunsch, Matthew J. Kirpes, Rachel M. Kolesar, Katheryn R. Barrett, Tate E. China, Swarup Sheesley, Rebecca J. Laskin, Alexander Wiedensohler, Alfred Tuch, Thomas Pratt, Kerri A. |
author_sort |
Gunsch, Matthew J. |
title |
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
title_short |
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
title_full |
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
title_fullStr |
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
title_full_unstemmed |
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska |
title_sort |
contributions of transported prudhoe bay oil field emissions to the aerosol population in utqiaġvik, alaska |
publisher |
Katlenburg-Lindau : EGU |
publishDate |
2017 |
url |
https://oa.tib.eu/renate/handle/123456789/11927 https://doi.org/10.34657/10960 |
genre |
Arctic Arctic Ocean Barrow Prudhoe Bay Sea ice Alaska |
genre_facet |
Arctic Arctic Ocean Barrow Prudhoe Bay Sea ice Alaska |
op_source |
Atmospheric Chemistry and Physics 17 (2017), Nr. 17 |
op_rights |
CC BY 3.0 Unported https://creativecommons.org/licenses/by/3.0 |
op_doi |
https://doi.org/10.34657/10960 |
_version_ |
1781694629768331264 |