Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn
Aerosol physics measurements made onboard the Swedish icebreaker Oden in the late Summer and early Autumn of 1991 during the International Arctic Ocean Expedition (IAOE-91) have provided the first data on the size distribution of particles in the Arctic marine boundary layer (MBL) that cover both th...
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ftleibnizopen:oai:oai.leibnizopen.de:AEGWhIgBdbrxVwz6ljXr 2023-06-18T03:39:01+02:00 Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn Covert, D.S. Wiedensohler, A. Aalto, P. Heintzenberg, J. Mcmurry, P.H. Leck, C. 1996 application/pdf text/plain; charset=utf-8 https://oa.tib.eu/renate/handle/123456789/5414 https://doi.org/10.34657/4043 eng eng Copenhagen : Blackwell Munksgaard CC BY 3.0 Unported https://creativecommons.org/licenses/by/3.0/ Tellus, Series B: Chemical and Physical Meteorology 48 (1996), Nr. 2 accumulation mode aerosol size aerosols Aitken mode IAOE IAOE-91 marine boundary layer oceanic boundary layer particle number mode shipborne observation size distributions statistical analysis ultrafine mode Arctic Ocean 550 article Text 1996 ftleibnizopen https://doi.org/10.34657/4043 2023-06-04T23:24:50Z Aerosol physics measurements made onboard the Swedish icebreaker Oden in the late Summer and early Autumn of 1991 during the International Arctic Ocean Expedition (IAOE-91) have provided the first data on the size distribution of particles in the Arctic marine boundary layer (MBL) that cover both the number and mass modes of the size range from 3 to 500 nm diameter. These measurements were made in conjunction with atmospheric gas and condensed phase chemistry measurements in an effort to understand a part of the ocean-atmosphere sulfur cycle. Analysis of the particle physics data showed that there were three distinct number modes in the submicrometric aerosol in the Arctic MBL. These modes had geometric mean diameters of around 170 nm. 45 nm and 14 nm referred to as accumulation, Aitken and ultrafine modes, respectively. There were clear minima in number concentrations between the modes that appeared at 20 to 30 nm and at 80 to 100 nm. The total number concentration was most frequently between 30 and 60 particles cm-3 with a mean value of around 100 particles cm-3, but the hourly average concentration varied over two to three orders of magnitude during the 70 days of the expedition. On average, the highest concentration was in the accumulation mode that contained about 45% of the total number, while the Aitken mode contained about 40%. The greatest variability was in the ultrafine mode concentration which is indicative of active, earby sources (nucleation from the gas phase) and sinks; the Aitken and accumulation mode concentrations were much less variable. The ultrafine mode was observed about two thirds of the time and was dominant 10% of the time. A detailed description and statistical analysis of the modal aerosol parameters is presented here. publishedVersion Article in Journal/Newspaper Arctic Arctic Ocean oden LeibnizOpen (The Leibniz Association) Aitken ENVELOPE(-44.516,-44.516,-60.733,-60.733) Arctic Arctic Ocean |
institution |
Open Polar |
collection |
LeibnizOpen (The Leibniz Association) |
op_collection_id |
ftleibnizopen |
language |
English |
topic |
accumulation mode aerosol size aerosols Aitken mode IAOE IAOE-91 marine boundary layer oceanic boundary layer particle number mode shipborne observation size distributions statistical analysis ultrafine mode Arctic Ocean 550 |
spellingShingle |
accumulation mode aerosol size aerosols Aitken mode IAOE IAOE-91 marine boundary layer oceanic boundary layer particle number mode shipborne observation size distributions statistical analysis ultrafine mode Arctic Ocean 550 Covert, D.S. Wiedensohler, A. Aalto, P. Heintzenberg, J. Mcmurry, P.H. Leck, C. Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
topic_facet |
accumulation mode aerosol size aerosols Aitken mode IAOE IAOE-91 marine boundary layer oceanic boundary layer particle number mode shipborne observation size distributions statistical analysis ultrafine mode Arctic Ocean 550 |
description |
Aerosol physics measurements made onboard the Swedish icebreaker Oden in the late Summer and early Autumn of 1991 during the International Arctic Ocean Expedition (IAOE-91) have provided the first data on the size distribution of particles in the Arctic marine boundary layer (MBL) that cover both the number and mass modes of the size range from 3 to 500 nm diameter. These measurements were made in conjunction with atmospheric gas and condensed phase chemistry measurements in an effort to understand a part of the ocean-atmosphere sulfur cycle. Analysis of the particle physics data showed that there were three distinct number modes in the submicrometric aerosol in the Arctic MBL. These modes had geometric mean diameters of around 170 nm. 45 nm and 14 nm referred to as accumulation, Aitken and ultrafine modes, respectively. There were clear minima in number concentrations between the modes that appeared at 20 to 30 nm and at 80 to 100 nm. The total number concentration was most frequently between 30 and 60 particles cm-3 with a mean value of around 100 particles cm-3, but the hourly average concentration varied over two to three orders of magnitude during the 70 days of the expedition. On average, the highest concentration was in the accumulation mode that contained about 45% of the total number, while the Aitken mode contained about 40%. The greatest variability was in the ultrafine mode concentration which is indicative of active, earby sources (nucleation from the gas phase) and sinks; the Aitken and accumulation mode concentrations were much less variable. The ultrafine mode was observed about two thirds of the time and was dominant 10% of the time. A detailed description and statistical analysis of the modal aerosol parameters is presented here. publishedVersion |
format |
Article in Journal/Newspaper |
author |
Covert, D.S. Wiedensohler, A. Aalto, P. Heintzenberg, J. Mcmurry, P.H. Leck, C. |
author_facet |
Covert, D.S. Wiedensohler, A. Aalto, P. Heintzenberg, J. Mcmurry, P.H. Leck, C. |
author_sort |
Covert, D.S. |
title |
Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
title_short |
Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
title_full |
Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
title_fullStr |
Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
title_full_unstemmed |
Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
title_sort |
aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn |
publisher |
Copenhagen : Blackwell Munksgaard |
publishDate |
1996 |
url |
https://oa.tib.eu/renate/handle/123456789/5414 https://doi.org/10.34657/4043 |
long_lat |
ENVELOPE(-44.516,-44.516,-60.733,-60.733) |
geographic |
Aitken Arctic Arctic Ocean |
geographic_facet |
Aitken Arctic Arctic Ocean |
genre |
Arctic Arctic Ocean oden |
genre_facet |
Arctic Arctic Ocean oden |
op_source |
Tellus, Series B: Chemical and Physical Meteorology 48 (1996), Nr. 2 |
op_rights |
CC BY 3.0 Unported https://creativecommons.org/licenses/by/3.0/ |
op_doi |
https://doi.org/10.34657/4043 |
_version_ |
1769003844386160640 |