Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment

Substantial increases in the atmospheric concentration of well‐mixed greenhouse gases (notably CO2), such as those projected to occur by the end of the 21st century under large radiative forcing scenarios, have long been known to cause an acceleration of the Brewer‐Dobson circulation (BDC) in climat...

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Main Authors: Polvani, LM, Wang, L, Abalos, M, Butchart, N, Chipperfield, MP, Dameris, M, Deushi, M, Dhomse, SS, Joeckel, P, Kinnison, D, Michou, M, Morgenstern, O, Oman, LD, Plummer, DA, Stone, KA
Format: Article in Journal/Newspaper
Language:English
Published: American Geophysical Union 2019
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Online Access:https://eprints.whiterose.ac.uk/151051/
https://eprints.whiterose.ac.uk/151051/1/Polvani_et_al-2019-Journal_of_Geophysical_Research__Atmospheres.pdf
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spelling ftleedsuniv:oai:eprints.whiterose.ac.uk:151051 2023-05-15T18:22:52+02:00 Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment Polvani, LM Wang, L Abalos, M Butchart, N Chipperfield, MP Dameris, M Deushi, M Dhomse, SS Joeckel, P Kinnison, D Michou, M Morgenstern, O Oman, LD Plummer, DA Stone, KA 2019-07-16 text https://eprints.whiterose.ac.uk/151051/ https://eprints.whiterose.ac.uk/151051/1/Polvani_et_al-2019-Journal_of_Geophysical_Research__Atmospheres.pdf en eng American Geophysical Union https://eprints.whiterose.ac.uk/151051/1/Polvani_et_al-2019-Journal_of_Geophysical_Research__Atmospheres.pdf Polvani, LM, Wang, L, Abalos, M et al. (12 more authors) (2019) Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment. Journal of Geophysical Research: Atmospheres, 124 (13). pp. 6669-6680. ISSN 2169-8996 cc_by_nc_nd_4 CC-BY-NC-ND Article NonPeerReviewed 2019 ftleedsuniv 2023-01-30T22:22:30Z Substantial increases in the atmospheric concentration of well‐mixed greenhouse gases (notably CO2), such as those projected to occur by the end of the 21st century under large radiative forcing scenarios, have long been known to cause an acceleration of the Brewer‐Dobson circulation (BDC) in climate models. More recently, however, several single‐model studies have proposed that ozone‐depleting substances might also be important drivers of BDC trends. As these studies were conducted with different forcings over different periods, it is difficult to combine them to obtain a robust quantitative picture of the relative importance of ozone‐depleting substances as drivers of BDC trends. To this end, we here analyze—over identical past and future periods—the output from 20 similarly forced models, gathered from two recent chemistry‐climate modeling intercomparison projects. Our multimodel analysis reveals that ozone‐depleting substances are responsible for more than half of the modeled BDC trends in the two decades 1980–2000. We also find that, as a consequence of the Montreal Protocol, decreasing concentrations of ozone‐depleting substances in coming decades will strongly decelerate the BDC until the year 2080, reducing the age‐of‐air trends by more than half, and will thus substantially mitigate the impact of increasing CO2. As ozone‐depleting substances impact BDC trends, primarily, via the depletion/recovery of stratospheric ozone over the South Pole, they impart seasonal and hemispheric asymmetries to the trends which may offer opportunities for detection in coming decades. Article in Journal/Newspaper South pole White Rose Research Online (Universities of Leeds, Sheffield & York) South Pole
institution Open Polar
collection White Rose Research Online (Universities of Leeds, Sheffield & York)
op_collection_id ftleedsuniv
language English
description Substantial increases in the atmospheric concentration of well‐mixed greenhouse gases (notably CO2), such as those projected to occur by the end of the 21st century under large radiative forcing scenarios, have long been known to cause an acceleration of the Brewer‐Dobson circulation (BDC) in climate models. More recently, however, several single‐model studies have proposed that ozone‐depleting substances might also be important drivers of BDC trends. As these studies were conducted with different forcings over different periods, it is difficult to combine them to obtain a robust quantitative picture of the relative importance of ozone‐depleting substances as drivers of BDC trends. To this end, we here analyze—over identical past and future periods—the output from 20 similarly forced models, gathered from two recent chemistry‐climate modeling intercomparison projects. Our multimodel analysis reveals that ozone‐depleting substances are responsible for more than half of the modeled BDC trends in the two decades 1980–2000. We also find that, as a consequence of the Montreal Protocol, decreasing concentrations of ozone‐depleting substances in coming decades will strongly decelerate the BDC until the year 2080, reducing the age‐of‐air trends by more than half, and will thus substantially mitigate the impact of increasing CO2. As ozone‐depleting substances impact BDC trends, primarily, via the depletion/recovery of stratospheric ozone over the South Pole, they impart seasonal and hemispheric asymmetries to the trends which may offer opportunities for detection in coming decades.
format Article in Journal/Newspaper
author Polvani, LM
Wang, L
Abalos, M
Butchart, N
Chipperfield, MP
Dameris, M
Deushi, M
Dhomse, SS
Joeckel, P
Kinnison, D
Michou, M
Morgenstern, O
Oman, LD
Plummer, DA
Stone, KA
spellingShingle Polvani, LM
Wang, L
Abalos, M
Butchart, N
Chipperfield, MP
Dameris, M
Deushi, M
Dhomse, SS
Joeckel, P
Kinnison, D
Michou, M
Morgenstern, O
Oman, LD
Plummer, DA
Stone, KA
Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
author_facet Polvani, LM
Wang, L
Abalos, M
Butchart, N
Chipperfield, MP
Dameris, M
Deushi, M
Dhomse, SS
Joeckel, P
Kinnison, D
Michou, M
Morgenstern, O
Oman, LD
Plummer, DA
Stone, KA
author_sort Polvani, LM
title Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
title_short Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
title_full Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
title_fullStr Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
title_full_unstemmed Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment
title_sort large impacts, past and future, of ozone-depleting substances on brewer-dobson circulation trends: a multimodel assessment
publisher American Geophysical Union
publishDate 2019
url https://eprints.whiterose.ac.uk/151051/
https://eprints.whiterose.ac.uk/151051/1/Polvani_et_al-2019-Journal_of_Geophysical_Research__Atmospheres.pdf
geographic South Pole
geographic_facet South Pole
genre South pole
genre_facet South pole
op_relation https://eprints.whiterose.ac.uk/151051/1/Polvani_et_al-2019-Journal_of_Geophysical_Research__Atmospheres.pdf
Polvani, LM, Wang, L, Abalos, M et al. (12 more authors) (2019) Large Impacts, Past and Future, of Ozone-Depleting Substances on Brewer-Dobson Circulation Trends: A Multimodel Assessment. Journal of Geophysical Research: Atmospheres, 124 (13). pp. 6669-6680. ISSN 2169-8996
op_rights cc_by_nc_nd_4
op_rightsnorm CC-BY-NC-ND
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