High resolution modelling of long-range pollution transport
Air pollution can be transported between continents by large-scale atmospheric dynamics, where it can impact climate and regional air quality far from emission regions. During transport, concentrations in polluted plumes are affected by mixing with the background. Impacts of longrange pollution on c...
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Language: | French |
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2012
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ftinsu:oai:HAL:tel-00735198v1 2023-06-18T03:39:03+02:00 High resolution modelling of long-range pollution transport Modélisation à haute résolution du transport de polluants à longue distance Auby, Antoine TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Université Pierre et Marie Curie - Paris VI Kathy Law François Ravetta 2012-01-19 https://theses.hal.science/tel-00735198 https://theses.hal.science/tel-00735198/document https://theses.hal.science/tel-00735198/file/These_Auby.pdf fr fre HAL CCSD tel-00735198 https://theses.hal.science/tel-00735198 https://theses.hal.science/tel-00735198/document https://theses.hal.science/tel-00735198/file/These_Auby.pdf info:eu-repo/semantics/OpenAccess https://theses.hal.science/tel-00735198 Sciences de l'environnement. Université Pierre et Marie Curie - Paris VI, 2012. Français. ⟨NNT : ⟩ Atmospheric pollution Long-range transport Lagrangian modeling Mixing processes Arctic Passive tracer Processus de mélange Arctique Traceur passif Pollution atmosphérique Transport à longue distance Modélisation lagrangienne [SDE]Environmental Sciences info:eu-repo/semantics/doctoralThesis Theses 2012 ftinsu 2023-06-05T18:59:17Z Air pollution can be transported between continents by large-scale atmospheric dynamics, where it can impact climate and regional air quality far from emission regions. During transport, concentrations in polluted plumes are affected by mixing with the background. Impacts of longrange pollution on climate and air quality are usually quantified using global Eulerian models, that tend to overestimate mixing due to their low resolution. This induces errors in the simulated export of pollutants, and in the reaction rates due to the non-linearity of atmospheric chemistry. This thesis aims to better understand and quantify mixing of pollutant plumes in the free troposphere during long-range transport, and its representation in numerical models. It focuses on the Arctic, which is a region vulnerable to climate change, and where greenhouse gases and aerosol distributions are strongly influenced by transport of pollution from mid-latitudes. The work focuses on three case studies of transport into the Arctic troposphere during the POLARCAT campaign, in summer 2008. Results include estimates of the intensity of mixing in the Arctic troposphere, which was found to be lower than in mid-latitudes. The results also show that a Lagrangian modelling approach is able to reproduce the variability in observed concentrations in aged plumes, to simulate the transport of small-scale structures, and to evaluate the variability of ozone evolution in pollutant plumes due to differences in mixing scenarios. The model results are also used to assess pollutant transport simulated by global models in the Arctic, and to define the resolution neeeded for more accurate simulations. Overall, the results highlight the necessity to combine Lagrangian and Eulerian approaches to improve the representation of long-range pollution transport in numerical models. La pollution de l'air peut être transportée sur des distances de plusieurs milliers de kilomètres par la dynamique de grande échelle. Elle affecte ainsi le climat et la qualité de l'air loin ... Doctoral or Postdoctoral Thesis Arctic Arctique* Climate change Institut national des sciences de l'Univers: HAL-INSU Arctic |
institution |
Open Polar |
collection |
Institut national des sciences de l'Univers: HAL-INSU |
op_collection_id |
ftinsu |
language |
French |
topic |
Atmospheric pollution Long-range transport Lagrangian modeling Mixing processes Arctic Passive tracer Processus de mélange Arctique Traceur passif Pollution atmosphérique Transport à longue distance Modélisation lagrangienne [SDE]Environmental Sciences |
spellingShingle |
Atmospheric pollution Long-range transport Lagrangian modeling Mixing processes Arctic Passive tracer Processus de mélange Arctique Traceur passif Pollution atmosphérique Transport à longue distance Modélisation lagrangienne [SDE]Environmental Sciences Auby, Antoine High resolution modelling of long-range pollution transport |
topic_facet |
Atmospheric pollution Long-range transport Lagrangian modeling Mixing processes Arctic Passive tracer Processus de mélange Arctique Traceur passif Pollution atmosphérique Transport à longue distance Modélisation lagrangienne [SDE]Environmental Sciences |
description |
Air pollution can be transported between continents by large-scale atmospheric dynamics, where it can impact climate and regional air quality far from emission regions. During transport, concentrations in polluted plumes are affected by mixing with the background. Impacts of longrange pollution on climate and air quality are usually quantified using global Eulerian models, that tend to overestimate mixing due to their low resolution. This induces errors in the simulated export of pollutants, and in the reaction rates due to the non-linearity of atmospheric chemistry. This thesis aims to better understand and quantify mixing of pollutant plumes in the free troposphere during long-range transport, and its representation in numerical models. It focuses on the Arctic, which is a region vulnerable to climate change, and where greenhouse gases and aerosol distributions are strongly influenced by transport of pollution from mid-latitudes. The work focuses on three case studies of transport into the Arctic troposphere during the POLARCAT campaign, in summer 2008. Results include estimates of the intensity of mixing in the Arctic troposphere, which was found to be lower than in mid-latitudes. The results also show that a Lagrangian modelling approach is able to reproduce the variability in observed concentrations in aged plumes, to simulate the transport of small-scale structures, and to evaluate the variability of ozone evolution in pollutant plumes due to differences in mixing scenarios. The model results are also used to assess pollutant transport simulated by global models in the Arctic, and to define the resolution neeeded for more accurate simulations. Overall, the results highlight the necessity to combine Lagrangian and Eulerian approaches to improve the representation of long-range pollution transport in numerical models. La pollution de l'air peut être transportée sur des distances de plusieurs milliers de kilomètres par la dynamique de grande échelle. Elle affecte ainsi le climat et la qualité de l'air loin ... |
author2 |
TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Université Pierre et Marie Curie - Paris VI Kathy Law François Ravetta |
format |
Doctoral or Postdoctoral Thesis |
author |
Auby, Antoine |
author_facet |
Auby, Antoine |
author_sort |
Auby, Antoine |
title |
High resolution modelling of long-range pollution transport |
title_short |
High resolution modelling of long-range pollution transport |
title_full |
High resolution modelling of long-range pollution transport |
title_fullStr |
High resolution modelling of long-range pollution transport |
title_full_unstemmed |
High resolution modelling of long-range pollution transport |
title_sort |
high resolution modelling of long-range pollution transport |
publisher |
HAL CCSD |
publishDate |
2012 |
url |
https://theses.hal.science/tel-00735198 https://theses.hal.science/tel-00735198/document https://theses.hal.science/tel-00735198/file/These_Auby.pdf |
geographic |
Arctic |
geographic_facet |
Arctic |
genre |
Arctic Arctique* Climate change |
genre_facet |
Arctic Arctique* Climate change |
op_source |
https://theses.hal.science/tel-00735198 Sciences de l'environnement. Université Pierre et Marie Curie - Paris VI, 2012. Français. ⟨NNT : ⟩ |
op_relation |
tel-00735198 https://theses.hal.science/tel-00735198 https://theses.hal.science/tel-00735198/document https://theses.hal.science/tel-00735198/file/These_Auby.pdf |
op_rights |
info:eu-repo/semantics/OpenAccess |
_version_ |
1769003865098682368 |