Growth of nucleation mode particles in the summertime Arctic: a case study
International audience The summertime Arctic lower troposphere is a relatively pristine background aerosol environment dominated by nucleation and Aitken mode particles. Understanding the mechanisms that control the formation and growth of aerosol is crucial for our ability to predict cloud properti...
Published in: | Atmospheric Chemistry and Physics |
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Main Authors: | , , , , , , , , , , , |
Other Authors: | , , , , , , , , , , , , , |
Format: | Article in Journal/Newspaper |
Language: | English |
Published: |
HAL CCSD
2016
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Subjects: | |
Online Access: | https://insu.hal.science/insu-01336721 https://insu.hal.science/insu-01336721/document https://insu.hal.science/insu-01336721/file/acp-16-7663-2016.pdf https://doi.org/10.5194/acp-16-7663-2016 |
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openpolar |
institution |
Open Polar |
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Institut national des sciences de l'Univers: HAL-INSU |
op_collection_id |
ftinsu |
language |
English |
topic |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology |
spellingShingle |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology Willis, Megan D. Burkart, Julia Thomas, Jennie L. Köllner, Franziska Schneider, Johannes Bozem, Heiko Hoor, Peter M. Aliabadi, Amir A. Schulz, Hannes Herber, Andreas B. Leaitch, W. Richard Abbatt, Jonathan P. D. Growth of nucleation mode particles in the summertime Arctic: a case study |
topic_facet |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology |
description |
International audience The summertime Arctic lower troposphere is a relatively pristine background aerosol environment dominated by nucleation and Aitken mode particles. Understanding the mechanisms that control the formation and growth of aerosol is crucial for our ability to predict cloud properties and therefore radiative balance and climate. We present an analysis of an aerosol growth event observed in the Canadian Arc-tic Archipelago during summer as part of the NETCARE project. Under stable and clean atmospheric conditions, with low inversion heights, carbon monoxide less than 80 ppb v , and black carbon less than 5 ng m −3 , we observe growth of small particles, < 20 nm in diameter, into sizes above 50 nm. Aerosol growth was correlated with the presence of organic species, trimethylamine, and methanesulfonic acid (MSA) in particles ∼ 80 nm and larger, where the organ-ics are similar to those previously observed in marine settings. MSA-to-sulfate ratios as high as 0.15 were observed during aerosol growth, suggesting an important marine influence. The organic-rich aerosol contributes significantly to particles active as cloud condensation nuclei (CCN, su-persaturation = 0.6 %), which are elevated in concentration during aerosol growth above background levels of ∼ 100 to ∼ 220 cm −3. Results from this case study highlight the potential importance of secondary organic aerosol formation and its role in growing nucleation mode aerosol into CCN-active sizes in this remote marine environment. |
author2 |
Department of Chemistry University of Toronto University of Toronto TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Max Planck Institute for Chemistry (MPIC) Max-Planck-Gesellschaft Johannes Gutenberg - Universität Mainz = Johannes Gutenberg University (JGU) Environment and Climate Change Canada Massachusetts Institute of Technology (MIT) Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung = Alfred Wegener Institute for Polar and Marine Research = Institut Alfred-Wegener pour la recherche polaire et marine (AWI) Helmholtz-Gemeinschaft = Helmholtz Association Natural Sciences and Engineering Research Council of Canada The Alfred Wegener Institute and Environment and Climate Change Canada |
format |
Article in Journal/Newspaper |
author |
Willis, Megan D. Burkart, Julia Thomas, Jennie L. Köllner, Franziska Schneider, Johannes Bozem, Heiko Hoor, Peter M. Aliabadi, Amir A. Schulz, Hannes Herber, Andreas B. Leaitch, W. Richard Abbatt, Jonathan P. D. |
author_facet |
Willis, Megan D. Burkart, Julia Thomas, Jennie L. Köllner, Franziska Schneider, Johannes Bozem, Heiko Hoor, Peter M. Aliabadi, Amir A. Schulz, Hannes Herber, Andreas B. Leaitch, W. Richard Abbatt, Jonathan P. D. |
author_sort |
Willis, Megan D. |
title |
Growth of nucleation mode particles in the summertime Arctic: a case study |
title_short |
Growth of nucleation mode particles in the summertime Arctic: a case study |
title_full |
Growth of nucleation mode particles in the summertime Arctic: a case study |
title_fullStr |
Growth of nucleation mode particles in the summertime Arctic: a case study |
title_full_unstemmed |
Growth of nucleation mode particles in the summertime Arctic: a case study |
title_sort |
growth of nucleation mode particles in the summertime arctic: a case study |
publisher |
HAL CCSD |
publishDate |
2016 |
url |
https://insu.hal.science/insu-01336721 https://insu.hal.science/insu-01336721/document https://insu.hal.science/insu-01336721/file/acp-16-7663-2016.pdf https://doi.org/10.5194/acp-16-7663-2016 |
long_lat |
ENVELOPE(-44.516,-44.516,-60.733,-60.733) |
geographic |
Aitken Arctic |
geographic_facet |
Aitken Arctic |
genre |
Arctic black carbon |
genre_facet |
Arctic black carbon |
op_source |
ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://insu.hal.science/insu-01336721 Atmospheric Chemistry and Physics, 2016, 16, pp.7663-7679. ⟨10.5194/acp-16-7663-2016⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-16-7663-2016 insu-01336721 https://insu.hal.science/insu-01336721 https://insu.hal.science/insu-01336721/document https://insu.hal.science/insu-01336721/file/acp-16-7663-2016.pdf doi:10.5194/acp-16-7663-2016 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.5194/acp-16-7663-2016 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
16 |
container_issue |
12 |
container_start_page |
7663 |
op_container_end_page |
7679 |
_version_ |
1790596777238331392 |
spelling |
ftinsu:oai:HAL:insu-01336721v1 2024-02-11T10:01:03+01:00 Growth of nucleation mode particles in the summertime Arctic: a case study Willis, Megan D. Burkart, Julia Thomas, Jennie L. Köllner, Franziska Schneider, Johannes Bozem, Heiko Hoor, Peter M. Aliabadi, Amir A. Schulz, Hannes Herber, Andreas B. Leaitch, W. Richard Abbatt, Jonathan P. D. Department of Chemistry University of Toronto University of Toronto TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) Max Planck Institute for Chemistry (MPIC) Max-Planck-Gesellschaft Johannes Gutenberg - Universität Mainz = Johannes Gutenberg University (JGU) Environment and Climate Change Canada Massachusetts Institute of Technology (MIT) Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung = Alfred Wegener Institute for Polar and Marine Research = Institut Alfred-Wegener pour la recherche polaire et marine (AWI) Helmholtz-Gemeinschaft = Helmholtz Association Natural Sciences and Engineering Research Council of Canada The Alfred Wegener Institute and Environment and Climate Change Canada 2016 https://insu.hal.science/insu-01336721 https://insu.hal.science/insu-01336721/document https://insu.hal.science/insu-01336721/file/acp-16-7663-2016.pdf https://doi.org/10.5194/acp-16-7663-2016 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-16-7663-2016 insu-01336721 https://insu.hal.science/insu-01336721 https://insu.hal.science/insu-01336721/document https://insu.hal.science/insu-01336721/file/acp-16-7663-2016.pdf doi:10.5194/acp-16-7663-2016 info:eu-repo/semantics/OpenAccess ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://insu.hal.science/insu-01336721 Atmospheric Chemistry and Physics, 2016, 16, pp.7663-7679. ⟨10.5194/acp-16-7663-2016⟩ [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology info:eu-repo/semantics/article Journal articles 2016 ftinsu https://doi.org/10.5194/acp-16-7663-2016 2024-01-17T17:29:53Z International audience The summertime Arctic lower troposphere is a relatively pristine background aerosol environment dominated by nucleation and Aitken mode particles. Understanding the mechanisms that control the formation and growth of aerosol is crucial for our ability to predict cloud properties and therefore radiative balance and climate. We present an analysis of an aerosol growth event observed in the Canadian Arc-tic Archipelago during summer as part of the NETCARE project. Under stable and clean atmospheric conditions, with low inversion heights, carbon monoxide less than 80 ppb v , and black carbon less than 5 ng m −3 , we observe growth of small particles, < 20 nm in diameter, into sizes above 50 nm. Aerosol growth was correlated with the presence of organic species, trimethylamine, and methanesulfonic acid (MSA) in particles ∼ 80 nm and larger, where the organ-ics are similar to those previously observed in marine settings. MSA-to-sulfate ratios as high as 0.15 were observed during aerosol growth, suggesting an important marine influence. The organic-rich aerosol contributes significantly to particles active as cloud condensation nuclei (CCN, su-persaturation = 0.6 %), which are elevated in concentration during aerosol growth above background levels of ∼ 100 to ∼ 220 cm −3. Results from this case study highlight the potential importance of secondary organic aerosol formation and its role in growing nucleation mode aerosol into CCN-active sizes in this remote marine environment. Article in Journal/Newspaper Arctic black carbon Institut national des sciences de l'Univers: HAL-INSU Aitken ENVELOPE(-44.516,-44.516,-60.733,-60.733) Arctic Atmospheric Chemistry and Physics 16 12 7663 7679 |