Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean

Persistent organic pollutants (POPs) have received significant and ongoing attention. To establish favorable regulatory policies, it is vital to investigate the occurrence, source, and budgets of POPs worldwide. POPs including phthalic acid esters (PAEs), organophosphate esters (OPEs), brominated fl...

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Published in:Environmental Science & Technology
Main Authors: Cong, B., Li, S., Liu, S., Mi, W., Zhang, C., Xie, Z.
Format: Article in Journal/Newspaper
Language:English
Published: ACS 2022
Subjects:
Online Access:https://publications.hereon.de/id/50397
https://publications.hzg.de/id/50397
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spelling fthzgzmk:oai:publications.hereon.de:50397 2023-06-11T04:05:19+02:00 Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean Cong, B. Li, S. Liu, S. Mi, W. Zhang, C. Xie, Z. 2022 https://publications.hereon.de/id/50397 https://publications.hzg.de/id/50397 en eng ACS https://dx.doi.org/10.1021/acs.est.1c08743 urn:issn:0013-936X https://publications.hereon.de/id/50397 https://publications.hzg.de/id/50397 info:eu-repo/semantics/closedAccess issn:0013-936X Cong, B.; Li, S.; Liu, S.; Mi, W.; Liu, S.; Zhang, C.; Xie, Z.: Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean. In: Environmental Science and Technology. Vol. 56 (2022) 7, 4199 - 4209. (DOI: /10.1021/acs.est.1c08743) info:eu-repo/semantics/article Zeitschrift Artikel 2022 fthzgzmk https://doi.org/10.1021/acs.est.1c08743 2023-05-28T23:25:27Z Persistent organic pollutants (POPs) have received significant and ongoing attention. To establish favorable regulatory policies, it is vital to investigate the occurrence, source, and budgets of POPs worldwide. POPs including phthalic acid esters (PAEs), organophosphate esters (OPEs), brominated flame retardants (BFRs), and highly chlorinated flame retardants (HFRs) have not yet been examined in the Eastern Indian Ocean (EIO). In this study, the distribution of POPs has been investigated from surface sediments with the depth of 4369–5742 m in the Central Indian Ocean Basin (CIOB) and Wharton Basin (WB) of EIO. The average (±SD) concentrations of ∑11PAEs, ∑11OPEs, ∑4 BFRs, and ∑5HFRs were 1202.0 ± 274.36 ng g–1 dw, 15.3 ± 7.23 ng g–1 dw, 327.6 ± 211.74 pg g–1 dw, and 7.9 ± 7.45 pg g–1 dw, respectively. The high abundance of low-molecular-weight (LMW) PAEs, chlorinated OPEs, LMW BDEs, and anti-Dechlorane Plus indicated the pollution characteristics in the EIO. Correlation analysis demonstrated that LMW compounds may be derived from the high-molecular-weight compounds. The monsoon circulation, currents, and Antarctic Bottom Water may be the main drivers. POP accumulation rate, depositional flux, and mass inventory in the Indian Ocean were also estimated. Article in Journal/Newspaper Antarc* Antarctic Hereon Publications (Helmholtz-Zentrum) Antarctic Indian Wharton ENVELOPE(157.817,157.817,-81.050,-81.050) Environmental Science & Technology 56 7 4199 4209
institution Open Polar
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language English
description Persistent organic pollutants (POPs) have received significant and ongoing attention. To establish favorable regulatory policies, it is vital to investigate the occurrence, source, and budgets of POPs worldwide. POPs including phthalic acid esters (PAEs), organophosphate esters (OPEs), brominated flame retardants (BFRs), and highly chlorinated flame retardants (HFRs) have not yet been examined in the Eastern Indian Ocean (EIO). In this study, the distribution of POPs has been investigated from surface sediments with the depth of 4369–5742 m in the Central Indian Ocean Basin (CIOB) and Wharton Basin (WB) of EIO. The average (±SD) concentrations of ∑11PAEs, ∑11OPEs, ∑4 BFRs, and ∑5HFRs were 1202.0 ± 274.36 ng g–1 dw, 15.3 ± 7.23 ng g–1 dw, 327.6 ± 211.74 pg g–1 dw, and 7.9 ± 7.45 pg g–1 dw, respectively. The high abundance of low-molecular-weight (LMW) PAEs, chlorinated OPEs, LMW BDEs, and anti-Dechlorane Plus indicated the pollution characteristics in the EIO. Correlation analysis demonstrated that LMW compounds may be derived from the high-molecular-weight compounds. The monsoon circulation, currents, and Antarctic Bottom Water may be the main drivers. POP accumulation rate, depositional flux, and mass inventory in the Indian Ocean were also estimated.
format Article in Journal/Newspaper
author Cong, B.
Li, S.
Liu, S.
Mi, W.
Zhang, C.
Xie, Z.
spellingShingle Cong, B.
Li, S.
Liu, S.
Mi, W.
Zhang, C.
Xie, Z.
Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
author_facet Cong, B.
Li, S.
Liu, S.
Mi, W.
Zhang, C.
Xie, Z.
author_sort Cong, B.
title Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
title_short Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
title_full Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
title_fullStr Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
title_full_unstemmed Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean
title_sort source and distribution of emerging and legacy persistent organic pollutants in the basins of the eastern indian ocean
publisher ACS
publishDate 2022
url https://publications.hereon.de/id/50397
https://publications.hzg.de/id/50397
long_lat ENVELOPE(157.817,157.817,-81.050,-81.050)
geographic Antarctic
Indian
Wharton
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Indian
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genre Antarc*
Antarctic
genre_facet Antarc*
Antarctic
op_source issn:0013-936X
Cong, B.; Li, S.; Liu, S.; Mi, W.; Liu, S.; Zhang, C.; Xie, Z.: Source and Distribution of Emerging and Legacy Persistent Organic Pollutants in the Basins of the Eastern Indian Ocean. In: Environmental Science and Technology. Vol. 56 (2022) 7, 4199 - 4209. (DOI: /10.1021/acs.est.1c08743)
op_relation https://dx.doi.org/10.1021/acs.est.1c08743
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