Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic
Secondary organic aerosol (SOA) formation through isoprene oxidation was investigated with the regional-scale climate model REMOTE. The applied modeling scheme includes a treatment for marine primary organic aerosol emissions, aerosol microphysics, and SOA formation through the gas/particle partitio...
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fthindawi:oai:hindawi.com:10.1155/2010/482603 2023-05-15T17:29:10+02:00 Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic Tatu Anttila Baerbel Langmann Saji Varghese Colin O'Dowd 2010 https://doi.org/10.1155/2010/482603 en eng Advances in Meteorology https://doi.org/10.1155/2010/482603 Copyright © 2010 Tatu Anttila et al. Research Article 2010 fthindawi https://doi.org/10.1155/2010/482603 2019-05-26T01:23:29Z Secondary organic aerosol (SOA) formation through isoprene oxidation was investigated with the regional-scale climate model REMOTE. The applied modeling scheme includes a treatment for marine primary organic aerosol emissions, aerosol microphysics, and SOA formation through the gas/particle partitioning of semivolatile, water-soluble oxidation products. The focus was on SOA formation taking place over the North-East Atlantic during a period of high biological activity. Isoprene SOA concentrations were up to ~5 ng m−3 over North Atlantic in the base case model runs, and isoprene oxidation made a negligible contribution to the marine organic aerosol (OA) mass. In particular, isoprene SOA did not account for the observed water-soluble organic carbon (WSOC) concentrations over North Atlantic. The performed model calculations, together with results from recent field measurements, imply a missing source of SOA over remote marine areas unless the isoprene oxidation products are considerably less volatile than the current knowledge indicates. Article in Journal/Newspaper North Atlantic North East Atlantic Hindawi Publishing Corporation Advances in Meteorology 2010 1 10 |
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Open Polar |
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Hindawi Publishing Corporation |
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language |
English |
description |
Secondary organic aerosol (SOA) formation through isoprene oxidation was investigated with the regional-scale climate model REMOTE. The applied modeling scheme includes a treatment for marine primary organic aerosol emissions, aerosol microphysics, and SOA formation through the gas/particle partitioning of semivolatile, water-soluble oxidation products. The focus was on SOA formation taking place over the North-East Atlantic during a period of high biological activity. Isoprene SOA concentrations were up to ~5 ng m−3 over North Atlantic in the base case model runs, and isoprene oxidation made a negligible contribution to the marine organic aerosol (OA) mass. In particular, isoprene SOA did not account for the observed water-soluble organic carbon (WSOC) concentrations over North Atlantic. The performed model calculations, together with results from recent field measurements, imply a missing source of SOA over remote marine areas unless the isoprene oxidation products are considerably less volatile than the current knowledge indicates. |
format |
Article in Journal/Newspaper |
author |
Tatu Anttila Baerbel Langmann Saji Varghese Colin O'Dowd |
spellingShingle |
Tatu Anttila Baerbel Langmann Saji Varghese Colin O'Dowd Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
author_facet |
Tatu Anttila Baerbel Langmann Saji Varghese Colin O'Dowd |
author_sort |
Tatu Anttila |
title |
Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
title_short |
Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
title_full |
Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
title_fullStr |
Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
title_full_unstemmed |
Contribution of Isoprene Oxidation Products to Marine Aerosol over the North-East Atlantic |
title_sort |
contribution of isoprene oxidation products to marine aerosol over the north-east atlantic |
publisher |
Advances in Meteorology |
publishDate |
2010 |
url |
https://doi.org/10.1155/2010/482603 |
genre |
North Atlantic North East Atlantic |
genre_facet |
North Atlantic North East Atlantic |
op_relation |
https://doi.org/10.1155/2010/482603 |
op_rights |
Copyright © 2010 Tatu Anttila et al. |
op_doi |
https://doi.org/10.1155/2010/482603 |
container_title |
Advances in Meteorology |
container_volume |
2010 |
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1 |
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10 |
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1766122792794718208 |