Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters

Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on the generation of SSA, and thereby clouds and...

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Bibliographic Details
Main Authors: Rocchi, Arianna, von Jackowski, Anabel, Welti, André, Li, Guangyu, Kanji, Zamin A, id_orcid:0 000-0001-8610-3921, Povazhnyy, Vasiliy, Engel, Anja, Schmale, Julia, Nenes, Athanasios, Berdalet, Elisa, Simó, Rafel, Dall'Osto, Manuel
Format: Article in Journal/Newspaper
Language:English
Published: American Chemical Society 2024
Subjects:
marine biogeochemistry
Arctic
polar aerosolproduction
aerosol chamber
organic matter
climate change
Arctic Ocean
Climate change
Global warming
Phytoplankton
Online Access:https://hdl.handle.net/20.500.11850/674705
https://doi.org/10.3929/ethz-b-000674705
Description
Summary:Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on the generation of SSA, and thereby clouds and fog formation in this region, are unknown. During the ship-based Arctic Century Expedition, we examined the dependency of forced SSA production on the biogeochemical characteristics of seawater using an on-board temperature-controlled aerosol generation chamber with a plunging jet system. Our results indicate that mainly seawater salinity and organic content influence the production and size distribution of SSA. However, we observed a 2-fold higher SSA production from waters with similar salinity collected north of 81 degrees N compared to samples collected south of this latitude. This variability was not explained by phytoplankton and bacterial abundances or Chlorophyll-a concentration but by the presence of glucose in seawater. The synergic action of sea salt (essential component) and glucose or glucose-rich saccharides (enhancer) accounts for >80% of SSA predictability throughout the cruise. Our results suggest that besides wind speed and salinity, SSA production in Arctic waters is also affected by specific organics released by the microbiota. ISSN:0013-936X ISSN:1520-5851

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