Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada

Airborne dust from glacial outwash sediments may alter properties of clouds and climate at high latitudes by acting as ice nucleating particles (INPs). Nevertheless, the ice nucleating ability of airborne dust from glacial outwash sediments remains uncertain. To address this uncertainty, we measured...

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Main Authors: Xi, Yu, Xu, Cuishan, Downey, Arnold, Stevens, Robin, Bachelder, Jill, id_orcid:0 000-0003-3787-1128, King, James, Hayes, Patrick L., Bertram, Allan K.
Format: Article in Journal/Newspaper
Language:English
Published: Royal Society of Chemistry 2022
Subjects:
Online Access:https://hdl.handle.net/20.500.11850/559647
https://doi.org/10.3929/ethz-b-000559647
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spelling ftethz:oai:www.research-collection.ethz.ch:20.500.11850/559647 2023-10-09T21:51:48+02:00 Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada Xi, Yu Xu, Cuishan Downey, Arnold Stevens, Robin Bachelder, Jill id_orcid:0 000-0003-3787-1128 King, James Hayes, Patrick L. Bertram, Allan K. 2022 application/application/pdf https://hdl.handle.net/20.500.11850/559647 https://doi.org/10.3929/ethz-b-000559647 en eng Royal Society of Chemistry info:eu-repo/semantics/altIdentifier/doi/10.1039/d1ea00101a info:eu-repo/semantics/altIdentifier/wos/000826368900001 http://hdl.handle.net/20.500.11850/559647 doi:10.3929/ethz-b-000559647 info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by-nc/3.0/ Creative Commons Attribution-NonCommercial 3.0 Unported Environmental Science: Atmospheres, 2 (4) info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion 2022 ftethz https://doi.org/20.500.11850/55964710.3929/ethz-b-00055964710.1039/d1ea00101a 2023-09-17T23:49:49Z Airborne dust from glacial outwash sediments may alter properties of clouds and climate at high latitudes by acting as ice nucleating particles (INPs). Nevertheless, the ice nucleating ability of airborne dust from glacial outwash sediments remains uncertain. To address this uncertainty, we measured the ice nucleating ability of airborne dust near an actively retreating glacier in Yukon, Canada during a period when airborne dust concentrations were well above background levels and most likely originated from glacial outwash sediments in the region. The airborne dust caused freezing at temperatures from -6 to -23 degrees C. Based on a heat assay and an ammonium sulfate assay, the INPs from the airborne dust that caused freezing at temperatures warmer than -15 degrees C likely contained biological materials. We show that airborne dust from the retreating glacier likely led to high concentrations of ice nucleating particles at the site for at least most of May 2018. These concentrations, at a freezing temperature of -15 degrees C, were approximately one order of magnitude higher than predictions using a global chemical transport model that included low latitude natural dust sources, but not natural high latitude dust sources. ISSN:2634-3606 Article in Journal/Newspaper glacier* Yukon ETH Zürich Research Collection Canada Yukon
institution Open Polar
collection ETH Zürich Research Collection
op_collection_id ftethz
language English
description Airborne dust from glacial outwash sediments may alter properties of clouds and climate at high latitudes by acting as ice nucleating particles (INPs). Nevertheless, the ice nucleating ability of airborne dust from glacial outwash sediments remains uncertain. To address this uncertainty, we measured the ice nucleating ability of airborne dust near an actively retreating glacier in Yukon, Canada during a period when airborne dust concentrations were well above background levels and most likely originated from glacial outwash sediments in the region. The airborne dust caused freezing at temperatures from -6 to -23 degrees C. Based on a heat assay and an ammonium sulfate assay, the INPs from the airborne dust that caused freezing at temperatures warmer than -15 degrees C likely contained biological materials. We show that airborne dust from the retreating glacier likely led to high concentrations of ice nucleating particles at the site for at least most of May 2018. These concentrations, at a freezing temperature of -15 degrees C, were approximately one order of magnitude higher than predictions using a global chemical transport model that included low latitude natural dust sources, but not natural high latitude dust sources. ISSN:2634-3606
format Article in Journal/Newspaper
author Xi, Yu
Xu, Cuishan
Downey, Arnold
Stevens, Robin
Bachelder, Jill
id_orcid:0 000-0003-3787-1128
King, James
Hayes, Patrick L.
Bertram, Allan K.
spellingShingle Xi, Yu
Xu, Cuishan
Downey, Arnold
Stevens, Robin
Bachelder, Jill
id_orcid:0 000-0003-3787-1128
King, James
Hayes, Patrick L.
Bertram, Allan K.
Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
author_facet Xi, Yu
Xu, Cuishan
Downey, Arnold
Stevens, Robin
Bachelder, Jill
id_orcid:0 000-0003-3787-1128
King, James
Hayes, Patrick L.
Bertram, Allan K.
author_sort Xi, Yu
title Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
title_short Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
title_full Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
title_fullStr Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
title_full_unstemmed Ice nucleating properties of airborne dust from an actively retreating glacier in Yukon, Canada
title_sort ice nucleating properties of airborne dust from an actively retreating glacier in yukon, canada
publisher Royal Society of Chemistry
publishDate 2022
url https://hdl.handle.net/20.500.11850/559647
https://doi.org/10.3929/ethz-b-000559647
geographic Canada
Yukon
geographic_facet Canada
Yukon
genre glacier*
Yukon
genre_facet glacier*
Yukon
op_source Environmental Science: Atmospheres, 2 (4)
op_relation info:eu-repo/semantics/altIdentifier/doi/10.1039/d1ea00101a
info:eu-repo/semantics/altIdentifier/wos/000826368900001
http://hdl.handle.net/20.500.11850/559647
doi:10.3929/ethz-b-000559647
op_rights info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by-nc/3.0/
Creative Commons Attribution-NonCommercial 3.0 Unported
op_doi https://doi.org/20.500.11850/55964710.3929/ethz-b-00055964710.1039/d1ea00101a
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