New insights on the role of sea ice in intercepting atmospheric pollutants using 129I
Measurements of 129I carried out on sea ice samples collected in the central Arctic Ocean in 2007 revealed relatively high levels in the range of 100-1400×107 at L-1 that are comparable to levels measured in the surface mixed layer of the ocean at the same time. The 129I/127I ratio in sea ice is muc...
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Edith Cowan University, Research Online, Perth, Western Australia
2014
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ftedithcowan:oai:ro.ecu.edu.au:ecuworkspost2013-1146 2023-05-15T14:49:20+02:00 New insights on the role of sea ice in intercepting atmospheric pollutants using 129I Gómez-Guzmán, J M Cámara-Mor, P Suzuki, T López-Gutiérrez, J M Mas, J L Masqué, P Moran, S B Smith, J N 2014-01-01T08:00:00Z https://ro.ecu.edu.au/ecuworkspost2013/147 https://doi.org/10.1016/j.marpolbul.2014.10.004 unknown Edith Cowan University, Research Online, Perth, Western Australia https://ro.ecu.edu.au/ecuworkspost2013/147 http://dx.doi.org/10.1016/j.marpolbul.2014.10.004 subscription content Research outputs 2014 to 2021 AMS Arctic Ocean Atmospheric deposition Iodine-129 Reprocessing Sea ice Atmospheric movements Iodine Meteorological problems Scrap metal reprocessing Atmospheric depositions Atmospheric pollutants Atmospheric transport Back trajectories Surface mixed layers Nuclear fuel reprocessing iodine 129 accelerator mass spectrometry atmospheric pollution trajectory volatilization air pollutant air pollution Arctic Article concentration (parameters) oceanic regions pollution transport sea surface waters Basse Normandie Cumbria England France La Hague Manche Sellafield United Kingdom Marine Biology text 2014 ftedithcowan https://doi.org/10.1016/j.marpolbul.2014.10.004 2022-03-19T23:50:43Z Measurements of 129I carried out on sea ice samples collected in the central Arctic Ocean in 2007 revealed relatively high levels in the range of 100-1400×107 at L-1 that are comparable to levels measured in the surface mixed layer of the ocean at the same time. The 129I/127I ratio in sea ice is much greater than that in the underlying water, indicating that the 129I inventory in sea ice cannot be supported by direct uptake from seawater or by iodine volatilization from proximal (nearby) oceanic regimes. Instead, it is proposed that most of the 129I inventory in the sea ice is derived from direct atmospheric transport from European nuclear fuel reprocessing plants at Sellafield and Cap La Hague. This hypothesis is supported by back trajectory simulations indicating that volume elements of air originating in the Sellafield/La Hague regions would have been present at arctic sampling stations coincident with sampling collection. Text Arctic Arctic Ocean Sea ice Edith Cowan University (ECU, Australia): Research Online Arctic Arctic Ocean Marine Pollution Bulletin 89 1-2 180 190 |
institution |
Open Polar |
collection |
Edith Cowan University (ECU, Australia): Research Online |
op_collection_id |
ftedithcowan |
language |
unknown |
topic |
AMS Arctic Ocean Atmospheric deposition Iodine-129 Reprocessing Sea ice Atmospheric movements Iodine Meteorological problems Scrap metal reprocessing Atmospheric depositions Atmospheric pollutants Atmospheric transport Back trajectories Surface mixed layers Nuclear fuel reprocessing iodine 129 accelerator mass spectrometry atmospheric pollution trajectory volatilization air pollutant air pollution Arctic Article concentration (parameters) oceanic regions pollution transport sea surface waters Basse Normandie Cumbria England France La Hague Manche Sellafield United Kingdom Marine Biology |
spellingShingle |
AMS Arctic Ocean Atmospheric deposition Iodine-129 Reprocessing Sea ice Atmospheric movements Iodine Meteorological problems Scrap metal reprocessing Atmospheric depositions Atmospheric pollutants Atmospheric transport Back trajectories Surface mixed layers Nuclear fuel reprocessing iodine 129 accelerator mass spectrometry atmospheric pollution trajectory volatilization air pollutant air pollution Arctic Article concentration (parameters) oceanic regions pollution transport sea surface waters Basse Normandie Cumbria England France La Hague Manche Sellafield United Kingdom Marine Biology Gómez-Guzmán, J M Cámara-Mor, P Suzuki, T López-Gutiérrez, J M Mas, J L Masqué, P Moran, S B Smith, J N New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
topic_facet |
AMS Arctic Ocean Atmospheric deposition Iodine-129 Reprocessing Sea ice Atmospheric movements Iodine Meteorological problems Scrap metal reprocessing Atmospheric depositions Atmospheric pollutants Atmospheric transport Back trajectories Surface mixed layers Nuclear fuel reprocessing iodine 129 accelerator mass spectrometry atmospheric pollution trajectory volatilization air pollutant air pollution Arctic Article concentration (parameters) oceanic regions pollution transport sea surface waters Basse Normandie Cumbria England France La Hague Manche Sellafield United Kingdom Marine Biology |
description |
Measurements of 129I carried out on sea ice samples collected in the central Arctic Ocean in 2007 revealed relatively high levels in the range of 100-1400×107 at L-1 that are comparable to levels measured in the surface mixed layer of the ocean at the same time. The 129I/127I ratio in sea ice is much greater than that in the underlying water, indicating that the 129I inventory in sea ice cannot be supported by direct uptake from seawater or by iodine volatilization from proximal (nearby) oceanic regimes. Instead, it is proposed that most of the 129I inventory in the sea ice is derived from direct atmospheric transport from European nuclear fuel reprocessing plants at Sellafield and Cap La Hague. This hypothesis is supported by back trajectory simulations indicating that volume elements of air originating in the Sellafield/La Hague regions would have been present at arctic sampling stations coincident with sampling collection. |
format |
Text |
author |
Gómez-Guzmán, J M Cámara-Mor, P Suzuki, T López-Gutiérrez, J M Mas, J L Masqué, P Moran, S B Smith, J N |
author_facet |
Gómez-Guzmán, J M Cámara-Mor, P Suzuki, T López-Gutiérrez, J M Mas, J L Masqué, P Moran, S B Smith, J N |
author_sort |
Gómez-Guzmán, J M |
title |
New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
title_short |
New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
title_full |
New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
title_fullStr |
New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
title_full_unstemmed |
New insights on the role of sea ice in intercepting atmospheric pollutants using 129I |
title_sort |
new insights on the role of sea ice in intercepting atmospheric pollutants using 129i |
publisher |
Edith Cowan University, Research Online, Perth, Western Australia |
publishDate |
2014 |
url |
https://ro.ecu.edu.au/ecuworkspost2013/147 https://doi.org/10.1016/j.marpolbul.2014.10.004 |
geographic |
Arctic Arctic Ocean |
geographic_facet |
Arctic Arctic Ocean |
genre |
Arctic Arctic Ocean Sea ice |
genre_facet |
Arctic Arctic Ocean Sea ice |
op_source |
Research outputs 2014 to 2021 |
op_relation |
https://ro.ecu.edu.au/ecuworkspost2013/147 http://dx.doi.org/10.1016/j.marpolbul.2014.10.004 |
op_rights |
subscription content |
op_doi |
https://doi.org/10.1016/j.marpolbul.2014.10.004 |
container_title |
Marine Pollution Bulletin |
container_volume |
89 |
container_issue |
1-2 |
container_start_page |
180 |
op_container_end_page |
190 |
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1766320394203037696 |