Iodine-129 in Snow and Seawater in the Antarctic: Level and Source
Anthropogenic 129 I has been released to the environment in different ways and chemical species by human nuclear activities since the 1940s. These sources provide ideal tools to trace the dispersion of volatile pollutants in the atmosphere. Snow and seawater samples collected in Bellingshausen, Amun...
Published in: | Environmental Science & Technology |
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Online Access: | https://orbit.dtu.dk/en/publications/439f7dc7-025e-4115-aa14-4091c150ca40 https://doi.org/10.1021/acs.est.5b01234 |
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ftdtupubl:oai:pure.atira.dk:publications/439f7dc7-025e-4115-aa14-4091c150ca40 2023-12-24T10:11:07+01:00 Iodine-129 in Snow and Seawater in the Antarctic: Level and Source Xing, Shan Hou, Xiaolin Aldahan, Ala Possnert, Göran Shi, Keliang Yi, Peng Zhou, Weijian 2015 https://orbit.dtu.dk/en/publications/439f7dc7-025e-4115-aa14-4091c150ca40 https://doi.org/10.1021/acs.est.5b01234 eng eng https://orbit.dtu.dk/en/publications/439f7dc7-025e-4115-aa14-4091c150ca40 info:eu-repo/semantics/closedAccess Xing , S , Hou , X , Aldahan , A , Possnert , G , Shi , K , Yi , P & Zhou , W 2015 , ' Iodine-129 in Snow and Seawater in the Antarctic: Level and Source ' , Environmental Science and Technology , vol. 49 , no. 11 , pp. 6691-6700 . https://doi.org/10.1021/acs.est.5b01234 Nuclear fuel reprocessing Nuclear weapons Seawater Snow Anthropogenic sources Northern Hemispheres Nuclear activities Nuclear weapons testing Orders of magnitude Reprocessing plant Southern Hemisphere Volatile pollutants Iodine /dk/atira/pure/sustainabledevelopmentgoals/life_below_water name=SDG 14 - Life Below Water article 2015 ftdtupubl https://doi.org/10.1021/acs.est.5b01234 2023-11-30T00:00:36Z Anthropogenic 129 I has been released to the environment in different ways and chemical species by human nuclear activities since the 1940s. These sources provide ideal tools to trace the dispersion of volatile pollutants in the atmosphere. Snow and seawater samples collected in Bellingshausen, Amundsen, and Ross Seas in Antarctica in 2011 were analyzed for 129 I and 127 I, including organic forms; it was observed that 129 I/ 127 I atomic ratios in the Antarctic surface seawater ((6.1-13) × 10 -12 ) are about 2 orders of magnitude lower than those in the Antarctic snow ((6.8-9.5) × 10 -10 ), but 4-6 times higher than the prenuclear level (1.5 × 10 -12 ), indicating a predominantly anthropogenic source of 129 I in the Antarctic environment. The 129 I level in snow in Antarctica is 2-4 orders of magnitude lower than that in the Northern Hemisphere, but is not significantly higher than that observed in other sites in the Southern Hemisphere. This feature indicates that 129 I in Antarctic snow mainly originates from atmospheric nuclear weapons testing from 1945 to 1980; resuspension and re-emission of the fallout 129 I in the Southern Hemisphere maintains the 129 I level in the Antarctic atmosphere. 129 I directly released to the atmosphere and re-emitted marine discharged 129 I from reprocessing plants in Europe might not significantly disperse to Antarctica. Article in Journal/Newspaper Antarc* Antarctic Antarctica Technical University of Denmark: DTU Orbit Antarctic The Antarctic Environmental Science & Technology 49 11 6691 6700 |
institution |
Open Polar |
collection |
Technical University of Denmark: DTU Orbit |
op_collection_id |
ftdtupubl |
language |
English |
topic |
Nuclear fuel reprocessing Nuclear weapons Seawater Snow Anthropogenic sources Northern Hemispheres Nuclear activities Nuclear weapons testing Orders of magnitude Reprocessing plant Southern Hemisphere Volatile pollutants Iodine /dk/atira/pure/sustainabledevelopmentgoals/life_below_water name=SDG 14 - Life Below Water |
spellingShingle |
Nuclear fuel reprocessing Nuclear weapons Seawater Snow Anthropogenic sources Northern Hemispheres Nuclear activities Nuclear weapons testing Orders of magnitude Reprocessing plant Southern Hemisphere Volatile pollutants Iodine /dk/atira/pure/sustainabledevelopmentgoals/life_below_water name=SDG 14 - Life Below Water Xing, Shan Hou, Xiaolin Aldahan, Ala Possnert, Göran Shi, Keliang Yi, Peng Zhou, Weijian Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
topic_facet |
Nuclear fuel reprocessing Nuclear weapons Seawater Snow Anthropogenic sources Northern Hemispheres Nuclear activities Nuclear weapons testing Orders of magnitude Reprocessing plant Southern Hemisphere Volatile pollutants Iodine /dk/atira/pure/sustainabledevelopmentgoals/life_below_water name=SDG 14 - Life Below Water |
description |
Anthropogenic 129 I has been released to the environment in different ways and chemical species by human nuclear activities since the 1940s. These sources provide ideal tools to trace the dispersion of volatile pollutants in the atmosphere. Snow and seawater samples collected in Bellingshausen, Amundsen, and Ross Seas in Antarctica in 2011 were analyzed for 129 I and 127 I, including organic forms; it was observed that 129 I/ 127 I atomic ratios in the Antarctic surface seawater ((6.1-13) × 10 -12 ) are about 2 orders of magnitude lower than those in the Antarctic snow ((6.8-9.5) × 10 -10 ), but 4-6 times higher than the prenuclear level (1.5 × 10 -12 ), indicating a predominantly anthropogenic source of 129 I in the Antarctic environment. The 129 I level in snow in Antarctica is 2-4 orders of magnitude lower than that in the Northern Hemisphere, but is not significantly higher than that observed in other sites in the Southern Hemisphere. This feature indicates that 129 I in Antarctic snow mainly originates from atmospheric nuclear weapons testing from 1945 to 1980; resuspension and re-emission of the fallout 129 I in the Southern Hemisphere maintains the 129 I level in the Antarctic atmosphere. 129 I directly released to the atmosphere and re-emitted marine discharged 129 I from reprocessing plants in Europe might not significantly disperse to Antarctica. |
format |
Article in Journal/Newspaper |
author |
Xing, Shan Hou, Xiaolin Aldahan, Ala Possnert, Göran Shi, Keliang Yi, Peng Zhou, Weijian |
author_facet |
Xing, Shan Hou, Xiaolin Aldahan, Ala Possnert, Göran Shi, Keliang Yi, Peng Zhou, Weijian |
author_sort |
Xing, Shan |
title |
Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
title_short |
Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
title_full |
Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
title_fullStr |
Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
title_full_unstemmed |
Iodine-129 in Snow and Seawater in the Antarctic: Level and Source |
title_sort |
iodine-129 in snow and seawater in the antarctic: level and source |
publishDate |
2015 |
url |
https://orbit.dtu.dk/en/publications/439f7dc7-025e-4115-aa14-4091c150ca40 https://doi.org/10.1021/acs.est.5b01234 |
geographic |
Antarctic The Antarctic |
geographic_facet |
Antarctic The Antarctic |
genre |
Antarc* Antarctic Antarctica |
genre_facet |
Antarc* Antarctic Antarctica |
op_source |
Xing , S , Hou , X , Aldahan , A , Possnert , G , Shi , K , Yi , P & Zhou , W 2015 , ' Iodine-129 in Snow and Seawater in the Antarctic: Level and Source ' , Environmental Science and Technology , vol. 49 , no. 11 , pp. 6691-6700 . https://doi.org/10.1021/acs.est.5b01234 |
op_relation |
https://orbit.dtu.dk/en/publications/439f7dc7-025e-4115-aa14-4091c150ca40 |
op_rights |
info:eu-repo/semantics/closedAccess |
op_doi |
https://doi.org/10.1021/acs.est.5b01234 |
container_title |
Environmental Science & Technology |
container_volume |
49 |
container_issue |
11 |
container_start_page |
6691 |
op_container_end_page |
6700 |
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1786160802571485184 |