Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei
The eastern North Atlantic (ENA) is a region dominated by pristine marine environment and subtropical marine boundary layer clouds. Under unperturbed atmospheric conditions, the regional aerosol regime in the ENA varies seasonally due to different seasonal surface-ocean biogenic emissions, removal p...
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ftdoajarticles:oai:doaj.org/article:fad8cf07fd5442ffba30a1fae12f64f7 2023-05-15T17:30:11+02:00 Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei F. Gallo J. Uin K. J. Sanchez R. H. Moore J. Wang R. Wood F. Mei C. Flynn S. Springston E. B. Azevedo C. Kuang A. C. Aiken 2023-04-01T00:00:00Z https://doi.org/10.5194/acp-23-4221-2023 https://doaj.org/article/fad8cf07fd5442ffba30a1fae12f64f7 EN eng Copernicus Publications https://acp.copernicus.org/articles/23/4221/2023/acp-23-4221-2023.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324 doi:10.5194/acp-23-4221-2023 1680-7316 1680-7324 https://doaj.org/article/fad8cf07fd5442ffba30a1fae12f64f7 Atmospheric Chemistry and Physics, Vol 23, Pp 4221-4246 (2023) Physics QC1-999 Chemistry QD1-999 article 2023 ftdoajarticles https://doi.org/10.5194/acp-23-4221-2023 2023-04-09T00:32:28Z The eastern North Atlantic (ENA) is a region dominated by pristine marine environment and subtropical marine boundary layer clouds. Under unperturbed atmospheric conditions, the regional aerosol regime in the ENA varies seasonally due to different seasonal surface-ocean biogenic emissions, removal processes, and meteorological regimes. However, during periods when the marine boundary layer aerosol in the ENA is impacted by particles transported from continental sources, aerosol properties within the marine boundary layer change significantly, affecting the concentration of cloud condensation nuclei (CCN). Here, we investigate the impact of long-range transported continental aerosol on the regional aerosol regime in the ENA using data collected at the U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility on Graciosa Island in 2017 during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign. We develop an algorithm that integrates number concentrations of particles with optical particle dry diameter ( D p ) between 100 and 1000 nm, single scattering albedo, and black carbon concentration to identify multiday events (with duration > 24 consecutive hours) of long-range continental aerosol transport in the ENA. In 2017, we detected nine multiday events of long-range transported particles that correspond to ∼ 7.5 % of the year. For each event, we perform HYSPLIT 10 d backward trajectories analysis, and we evaluate CALIPSO aerosol products to assess, respectively, the origins and compositions of aerosol particles arriving at the ENA site. Subsequently, we group the events into three categories, (1) mixture of dust and marine aerosols, (2) mixture of marine and polluted continental aerosols from industrialized areas, and (3) biomass burning aerosol from North America and Canada, and we evaluate their influence on aerosol population and cloud condensation nuclei in terms of potential activation fraction and concentrations at supersaturation of 0.1 % and ... Article in Journal/Newspaper North Atlantic Directory of Open Access Journals: DOAJ Articles Canada Atmospheric Chemistry and Physics 23 7 4221 4246 |
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language |
English |
topic |
Physics QC1-999 Chemistry QD1-999 |
spellingShingle |
Physics QC1-999 Chemistry QD1-999 F. Gallo J. Uin K. J. Sanchez R. H. Moore J. Wang R. Wood F. Mei C. Flynn S. Springston E. B. Azevedo C. Kuang A. C. Aiken Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
topic_facet |
Physics QC1-999 Chemistry QD1-999 |
description |
The eastern North Atlantic (ENA) is a region dominated by pristine marine environment and subtropical marine boundary layer clouds. Under unperturbed atmospheric conditions, the regional aerosol regime in the ENA varies seasonally due to different seasonal surface-ocean biogenic emissions, removal processes, and meteorological regimes. However, during periods when the marine boundary layer aerosol in the ENA is impacted by particles transported from continental sources, aerosol properties within the marine boundary layer change significantly, affecting the concentration of cloud condensation nuclei (CCN). Here, we investigate the impact of long-range transported continental aerosol on the regional aerosol regime in the ENA using data collected at the U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility on Graciosa Island in 2017 during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign. We develop an algorithm that integrates number concentrations of particles with optical particle dry diameter ( D p ) between 100 and 1000 nm, single scattering albedo, and black carbon concentration to identify multiday events (with duration > 24 consecutive hours) of long-range continental aerosol transport in the ENA. In 2017, we detected nine multiday events of long-range transported particles that correspond to ∼ 7.5 % of the year. For each event, we perform HYSPLIT 10 d backward trajectories analysis, and we evaluate CALIPSO aerosol products to assess, respectively, the origins and compositions of aerosol particles arriving at the ENA site. Subsequently, we group the events into three categories, (1) mixture of dust and marine aerosols, (2) mixture of marine and polluted continental aerosols from industrialized areas, and (3) biomass burning aerosol from North America and Canada, and we evaluate their influence on aerosol population and cloud condensation nuclei in terms of potential activation fraction and concentrations at supersaturation of 0.1 % and ... |
format |
Article in Journal/Newspaper |
author |
F. Gallo J. Uin K. J. Sanchez R. H. Moore J. Wang R. Wood F. Mei C. Flynn S. Springston E. B. Azevedo C. Kuang A. C. Aiken |
author_facet |
F. Gallo J. Uin K. J. Sanchez R. H. Moore J. Wang R. Wood F. Mei C. Flynn S. Springston E. B. Azevedo C. Kuang A. C. Aiken |
author_sort |
F. Gallo |
title |
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
title_short |
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
title_full |
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
title_fullStr |
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
title_full_unstemmed |
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei |
title_sort |
long-range transported continental aerosol in the eastern north atlantic: three multiday event regimes influence cloud condensation nuclei |
publisher |
Copernicus Publications |
publishDate |
2023 |
url |
https://doi.org/10.5194/acp-23-4221-2023 https://doaj.org/article/fad8cf07fd5442ffba30a1fae12f64f7 |
geographic |
Canada |
geographic_facet |
Canada |
genre |
North Atlantic |
genre_facet |
North Atlantic |
op_source |
Atmospheric Chemistry and Physics, Vol 23, Pp 4221-4246 (2023) |
op_relation |
https://acp.copernicus.org/articles/23/4221/2023/acp-23-4221-2023.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324 doi:10.5194/acp-23-4221-2023 1680-7316 1680-7324 https://doaj.org/article/fad8cf07fd5442ffba30a1fae12f64f7 |
op_doi |
https://doi.org/10.5194/acp-23-4221-2023 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
23 |
container_issue |
7 |
container_start_page |
4221 |
op_container_end_page |
4246 |
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1766126009642385408 |