Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion

We present methane (CH 4 ) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH 4 observations from 17 in situ and five...

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Published in:Atmospheric Chemistry and Physics
Main Authors: R. L. Thompson, M. Sasakawa, T. Machida, T. Aalto, D. Worthy, J. V. Lavric, C. Lund Myhre, A. Stohl
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2017
Subjects:
Online Access:https://doi.org/10.5194/acp-17-3553-2017
https://doaj.org/article/f249a74d6c154f66891be55a44faff52
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spelling ftdoajarticles:oai:doaj.org/article:f249a74d6c154f66891be55a44faff52 2023-05-15T16:35:34+02:00 Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion R. L. Thompson M. Sasakawa T. Machida T. Aalto D. Worthy J. V. Lavric C. Lund Myhre A. Stohl 2017-03-01T00:00:00Z https://doi.org/10.5194/acp-17-3553-2017 https://doaj.org/article/f249a74d6c154f66891be55a44faff52 EN eng Copernicus Publications http://www.atmos-chem-phys.net/17/3553/2017/acp-17-3553-2017.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324 1680-7316 1680-7324 doi:10.5194/acp-17-3553-2017 https://doaj.org/article/f249a74d6c154f66891be55a44faff52 Atmospheric Chemistry and Physics, Vol 17, Iss 5, Pp 3553-3572 (2017) Physics QC1-999 Chemistry QD1-999 article 2017 ftdoajarticles https://doi.org/10.5194/acp-17-3553-2017 2022-12-30T23:14:26Z We present methane (CH 4 ) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH 4 observations from 17 in situ and five discrete flask-sampling sites distributed over northern North America and Eurasia. CH 4 fluxes are determined at monthly temporal resolution and on a variable grid with maximum resolution of 1° × 1°. Our inversion finds a CH 4 source from the high northern latitudes of 82 to 84 Tg yr −1 , constituting ∼ 15 % of the global total, compared to 64 to 68 Tg yr −1 (∼ 12 %) in the prior estimates. For northern North America, we estimate a mean source of 16.6 to 17.9 Tg yr −1 , which is dominated by fluxes in the Hudson Bay Lowlands (HBL) and western Canada, specifically the province of Alberta. Our estimate for the HBL, of 2.7 to 3.4 Tg yr −1 , is close to the prior estimate (which includes wetland fluxes from the land surface model, LPX-Bern) and to other independent inversion estimates. However, our estimate for Alberta, of 5.0 to 5.8 Tg yr −1 , is significantly higher than the prior (which also includes anthropogenic sources from the EDGAR-4.2FT2010 inventory). Since the fluxes from this region persist throughout the winter, this may signify that the anthropogenic emissions are underestimated. For northern Eurasia, we find a mean source of 52.2 to 55.5 Tg yr −1 , with a strong contribution from fluxes in the Western Siberian Lowlands (WSL) for which we estimate a source of 19.3 to 19.9 Tg yr −1 . Over the 9-year inversion period, we find significant year-to-year variations in the fluxes, which in North America, and specifically in the HBL, appear to be driven at least in part by soil temperature, while in the WSL, the variability is more dependent on soil moisture. Moreover, we find significant positive trends in the CH 4 fluxes in North America of 0.38 to 0.57 Tg yr −2 , and northern Eurasia of 0.76 to 1.09 Tg yr −2 . In ... Article in Journal/Newspaper Hudson Bay Directory of Open Access Journals: DOAJ Articles Canada Hudson Hudson Bay Atmospheric Chemistry and Physics 17 5 3553 3572
institution Open Polar
collection Directory of Open Access Journals: DOAJ Articles
op_collection_id ftdoajarticles
language English
topic Physics
QC1-999
Chemistry
QD1-999
spellingShingle Physics
QC1-999
Chemistry
QD1-999
R. L. Thompson
M. Sasakawa
T. Machida
T. Aalto
D. Worthy
J. V. Lavric
C. Lund Myhre
A. Stohl
Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
topic_facet Physics
QC1-999
Chemistry
QD1-999
description We present methane (CH 4 ) flux estimates for 2005 to 2013 from a Bayesian inversion focusing on the high northern latitudes (north of 50° N). Our inversion is based on atmospheric transport modelled by the Lagrangian particle dispersion model FLEXPART and CH 4 observations from 17 in situ and five discrete flask-sampling sites distributed over northern North America and Eurasia. CH 4 fluxes are determined at monthly temporal resolution and on a variable grid with maximum resolution of 1° × 1°. Our inversion finds a CH 4 source from the high northern latitudes of 82 to 84 Tg yr −1 , constituting ∼ 15 % of the global total, compared to 64 to 68 Tg yr −1 (∼ 12 %) in the prior estimates. For northern North America, we estimate a mean source of 16.6 to 17.9 Tg yr −1 , which is dominated by fluxes in the Hudson Bay Lowlands (HBL) and western Canada, specifically the province of Alberta. Our estimate for the HBL, of 2.7 to 3.4 Tg yr −1 , is close to the prior estimate (which includes wetland fluxes from the land surface model, LPX-Bern) and to other independent inversion estimates. However, our estimate for Alberta, of 5.0 to 5.8 Tg yr −1 , is significantly higher than the prior (which also includes anthropogenic sources from the EDGAR-4.2FT2010 inventory). Since the fluxes from this region persist throughout the winter, this may signify that the anthropogenic emissions are underestimated. For northern Eurasia, we find a mean source of 52.2 to 55.5 Tg yr −1 , with a strong contribution from fluxes in the Western Siberian Lowlands (WSL) for which we estimate a source of 19.3 to 19.9 Tg yr −1 . Over the 9-year inversion period, we find significant year-to-year variations in the fluxes, which in North America, and specifically in the HBL, appear to be driven at least in part by soil temperature, while in the WSL, the variability is more dependent on soil moisture. Moreover, we find significant positive trends in the CH 4 fluxes in North America of 0.38 to 0.57 Tg yr −2 , and northern Eurasia of 0.76 to 1.09 Tg yr −2 . In ...
format Article in Journal/Newspaper
author R. L. Thompson
M. Sasakawa
T. Machida
T. Aalto
D. Worthy
J. V. Lavric
C. Lund Myhre
A. Stohl
author_facet R. L. Thompson
M. Sasakawa
T. Machida
T. Aalto
D. Worthy
J. V. Lavric
C. Lund Myhre
A. Stohl
author_sort R. L. Thompson
title Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_short Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_full Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_fullStr Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_full_unstemmed Methane fluxes in the high northern latitudes for 2005–2013 estimated using a Bayesian atmospheric inversion
title_sort methane fluxes in the high northern latitudes for 2005–2013 estimated using a bayesian atmospheric inversion
publisher Copernicus Publications
publishDate 2017
url https://doi.org/10.5194/acp-17-3553-2017
https://doaj.org/article/f249a74d6c154f66891be55a44faff52
geographic Canada
Hudson
Hudson Bay
geographic_facet Canada
Hudson
Hudson Bay
genre Hudson Bay
genre_facet Hudson Bay
op_source Atmospheric Chemistry and Physics, Vol 17, Iss 5, Pp 3553-3572 (2017)
op_relation http://www.atmos-chem-phys.net/17/3553/2017/acp-17-3553-2017.pdf
https://doaj.org/toc/1680-7316
https://doaj.org/toc/1680-7324
1680-7316
1680-7324
doi:10.5194/acp-17-3553-2017
https://doaj.org/article/f249a74d6c154f66891be55a44faff52
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container_title Atmospheric Chemistry and Physics
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