Widespread polar stratospheric ice clouds in the 2015–2016 Arctic winter – implications for ice nucleation

• Published in: Atmospheric Chemistry and Physics
• Main Authors: C. Voigt, A. Dörnbrack, M. Wirth, S. M. Groß, M. C. Pitts, L. R. Poole, R. Baumann, B. Ehard, B.-M. Sinnhuber, W. Woiwode, H. Oelhaf
• Format: Article in Journal/Newspaper
• Language: English
• Published: Copernicus Publications 2018
• Subjects: Physics; QC1-999; Chemistry; QD1-999; Arctic
• Online Access: https://doi.org/10.5194/acp-18-15623-2018; https://doaj.org/article/f040f2bad33d4cb6922c25e65fd140e2

Low planetary wave activity led to a stable vortex with exceptionally cold temperatures in the 2015–2016 Arctic winter. Extended areas with temperatures below the ice frost point temperature T ice persisted over weeks in the Arctic stratosphere as derived from the 36-year temperature climatology of the ERA-Interim reanalysis data set of the European Centre for Medium-Range Weather Forecasts (ECMWF). These extreme conditions promoted the formation of widespread polar stratospheric ice clouds (ice PSCs). The space-borne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument on board the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) satellite continuously measured ice PSCs for about a month with maximum extensions of up to 2×10 6 km 2 in the stratosphere. On 22 January 2016, the WALES (Water Vapor Lidar Experiment in Space – airborne demonstrator) lidar on board the High Altitude and Long Range Research Aircraft HALO detected an ice PSC with a horizontal length of more than 1400 km. The ice PSC extended between 18 and 24 km altitude and was surrounded by nitric acid trihydrate (NAT) particles, supercooled ternary solution (STS) droplets and particle mixtures. The ice PSC occurrence histogram in the backscatter ratio to particle depolarization ratio optical space exhibits two ice modes with high or low particle depolarization ratios. Domain-filling 8-day back-trajectories starting in the high particle depolarization (high-depol) ice mode are continuously below the NAT equilibrium temperature T NAT and decrease below T ice ∼ 10 h prior to the observation. Their matches with CALIPSO PSC curtain plots demonstrate the presence of NAT PSCs prior to high-depol ice, suggesting that the ice had nucleated on NAT. Vice versa, STS or no PSCs were detected by CALIPSO prior to the ice mode with low particle depolarization ratio. In addition to ice nucleation in STS potentially having meteoric inclusions, we find evidence for ice nucleation on NAT in the Arctic winter 2015–2016. The ...