Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols

Abstract Sulfur‐based stratospheric aerosol intervention (SAI) can cool the climate, but also heats the tropical lower stratosphere if done with injections at low latitudes. We explore the role of this heating in the climate response to SAI, by using mechanistic experiments that remove the effects o...

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Published in:Geophysical Research Letters
Main Authors: Elia Wunderlin, Gabriel Chiodo, Timofei Sukhodolov, Sandro Vattioni, Daniele Visioni, Simone Tilmes
Format: Article in Journal/Newspaper
Language:English
Published: Wiley 2024
Subjects:
Online Access:https://doi.org/10.1029/2023GL107285
https://doaj.org/article/ce2c417ac9954209b6d1425dae250cf3
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spelling ftdoajarticles:oai:doaj.org/article:ce2c417ac9954209b6d1425dae250cf3 2024-09-15T17:43:46+00:00 Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols Elia Wunderlin Gabriel Chiodo Timofei Sukhodolov Sandro Vattioni Daniele Visioni Simone Tilmes 2024-02-01T00:00:00Z https://doi.org/10.1029/2023GL107285 https://doaj.org/article/ce2c417ac9954209b6d1425dae250cf3 EN eng Wiley https://doi.org/10.1029/2023GL107285 https://doaj.org/toc/0094-8276 https://doaj.org/toc/1944-8007 1944-8007 0094-8276 doi:10.1029/2023GL107285 https://doaj.org/article/ce2c417ac9954209b6d1425dae250cf3 Geophysical Research Letters, Vol 51, Iss 4, Pp n/a-n/a (2024) Geophysics. Cosmic physics QC801-809 article 2024 ftdoajarticles https://doi.org/10.1029/2023GL107285 2024-08-05T17:49:23Z Abstract Sulfur‐based stratospheric aerosol intervention (SAI) can cool the climate, but also heats the tropical lower stratosphere if done with injections at low latitudes. We explore the role of this heating in the climate response to SAI, by using mechanistic experiments that remove the effects of longwave absorption of sulfate aerosols above the tropopause. If longwave absorption by stratospheric aerosols is disabled, the heating of the tropical tropopause and most of the related side effects are strongly alleviated and the cooling per Tg‐S injected is 40% bigger. Such side‐effects include the poleward expansion of eddy‐driven jets, acceleration of the stratospheric residual circulation, and delay of Antarctic ozone recovery. Our results add to other recent findings on SAI side effects and demonstrate that SAI scenarios with low‐latitude injections of absorptive materials may result in atmospheric effects and regional climate changes that are comparable to those produced by the CO2 warming signal. Article in Journal/Newspaper Antarc* Antarctic Directory of Open Access Journals: DOAJ Articles Geophysical Research Letters 51 4
institution Open Polar
collection Directory of Open Access Journals: DOAJ Articles
op_collection_id ftdoajarticles
language English
topic Geophysics. Cosmic physics
QC801-809
spellingShingle Geophysics. Cosmic physics
QC801-809
Elia Wunderlin
Gabriel Chiodo
Timofei Sukhodolov
Sandro Vattioni
Daniele Visioni
Simone Tilmes
Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
topic_facet Geophysics. Cosmic physics
QC801-809
description Abstract Sulfur‐based stratospheric aerosol intervention (SAI) can cool the climate, but also heats the tropical lower stratosphere if done with injections at low latitudes. We explore the role of this heating in the climate response to SAI, by using mechanistic experiments that remove the effects of longwave absorption of sulfate aerosols above the tropopause. If longwave absorption by stratospheric aerosols is disabled, the heating of the tropical tropopause and most of the related side effects are strongly alleviated and the cooling per Tg‐S injected is 40% bigger. Such side‐effects include the poleward expansion of eddy‐driven jets, acceleration of the stratospheric residual circulation, and delay of Antarctic ozone recovery. Our results add to other recent findings on SAI side effects and demonstrate that SAI scenarios with low‐latitude injections of absorptive materials may result in atmospheric effects and regional climate changes that are comparable to those produced by the CO2 warming signal.
format Article in Journal/Newspaper
author Elia Wunderlin
Gabriel Chiodo
Timofei Sukhodolov
Sandro Vattioni
Daniele Visioni
Simone Tilmes
author_facet Elia Wunderlin
Gabriel Chiodo
Timofei Sukhodolov
Sandro Vattioni
Daniele Visioni
Simone Tilmes
author_sort Elia Wunderlin
title Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
title_short Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
title_full Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
title_fullStr Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
title_full_unstemmed Side Effects of Sulfur‐Based Geoengineering Due To Absorptivity of Sulfate Aerosols
title_sort side effects of sulfur‐based geoengineering due to absorptivity of sulfate aerosols
publisher Wiley
publishDate 2024
url https://doi.org/10.1029/2023GL107285
https://doaj.org/article/ce2c417ac9954209b6d1425dae250cf3
genre Antarc*
Antarctic
genre_facet Antarc*
Antarctic
op_source Geophysical Research Letters, Vol 51, Iss 4, Pp n/a-n/a (2024)
op_relation https://doi.org/10.1029/2023GL107285
https://doaj.org/toc/0094-8276
https://doaj.org/toc/1944-8007
1944-8007
0094-8276
doi:10.1029/2023GL107285
https://doaj.org/article/ce2c417ac9954209b6d1425dae250cf3
op_doi https://doi.org/10.1029/2023GL107285
container_title Geophysical Research Letters
container_volume 51
container_issue 4
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