Inventory of African desert dust events in the north-central Iberian Peninsula in 2003–2014 based on sun-photometer–AERONET and particulate-mass–EMEP data

A reliable identification of desert dust (DD) episodes over north-central Spain is carried out based on the AErosol RObotic NETwork (AERONET) columnar aerosol sun photometer (aerosol optical depth, AOD, and Ångström exponent, α ) and European Monitoring and Evaluation Programme (EMEP) surface partic...

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Bibliographic Details
Published in:Atmospheric Chemistry and Physics
Main Authors: V. E. Cachorro, M. A. Burgos, D. Mateos, C. Toledano, Y. Bennouna, B. Torres, Á. M. de Frutos, Á. Herguedas
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2016
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Online Access:https://doi.org/10.5194/acp-16-8227-2016
https://doaj.org/article/bfd13f3db48440158f5dcbe01e4a0ec8
Description
Summary:A reliable identification of desert dust (DD) episodes over north-central Spain is carried out based on the AErosol RObotic NETwork (AERONET) columnar aerosol sun photometer (aerosol optical depth, AOD, and Ångström exponent, α ) and European Monitoring and Evaluation Programme (EMEP) surface particulate-mass concentration (PM x , x = 10, 2.5, and 2.5–10 µm) as the main core data. The impact of DD on background aerosol conditions is detectable by means of aerosol load thresholds and complementary information provided by HYSPLIT (Hybrid Single Particle Lagrangian Integrated Trajectory Model) air mass back trajectories, MODIS (Moderate Resolution Imaging Spectroradiometer) images, forecast aerosol models, and synoptic maps, which have been carefully reviewed by a human observer for each day included in the DD inventory. This identification method allows the detection of low and moderate DD intrusions and also of mixtures of mineral dust with other aerosol types by means of the analysis of α . During the period studied (2003–2014), a total of 152 DD episodes composed of 418 days are identified. Overall, this means ∼ 13 episodes and ∼ 35 days per year with DD intrusion, representing 9.5 % days year −1 . During the identified DD intrusions, 19 daily exceedances over 50 µg m −3 are reported at the surface. The occurrence of DD event days during the year peaks in March and June, with a marked minimum in April and lowest occurrence in winter. A large interannual variability is observed showing a statistically significant temporal decreasing trend of ∼ 3 days year −1 . The DD impact on the aerosol climatology is addressed by evaluating the DD contribution in magnitude and percent (in brackets) for AOD, PM 10 , PM 2.5 , and PM 2.5 − 10 , obtaining mean values of 0.015 (11.5 %), 1.3 µg m −3 (11.8 %), 0.55 µg m −3 (8.5 %) and 0.79 µg m −3 (16.1 %), respectively. Annual cycles of the DD contribution for AOD and PM 10 present two maxima – one in summer (0.03 and 2.4 µg m −3 for AOD in June and PM 10 in August) and another in ...