Particulate emissions from large North American wildfires estimated using a new top-down method
Particulate matter emissions from wildfires affect climate, weather and air quality. However, existing global and regional aerosol emission estimates differ by a factor of up to 4 between different methods. Using a novel approach, we estimate daily total particulate matter (TPM) emissions from large...
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ftdoajarticles:oai:doaj.org/article:3faf791606064e34971f84eabaf86596 2023-05-15T13:07:03+02:00 Particulate emissions from large North American wildfires estimated using a new top-down method T. Nikonovas P. R. J. North S. H. Doerr 2017-05-01T00:00:00Z https://doi.org/10.5194/acp-17-6423-2017 https://doaj.org/article/3faf791606064e34971f84eabaf86596 EN eng Copernicus Publications http://www.atmos-chem-phys.net/17/6423/2017/acp-17-6423-2017.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324 1680-7316 1680-7324 doi:10.5194/acp-17-6423-2017 https://doaj.org/article/3faf791606064e34971f84eabaf86596 Atmospheric Chemistry and Physics, Vol 17, Iss 10, Pp 6423-6438 (2017) Physics QC1-999 Chemistry QD1-999 article 2017 ftdoajarticles https://doi.org/10.5194/acp-17-6423-2017 2022-12-31T12:12:14Z Particulate matter emissions from wildfires affect climate, weather and air quality. However, existing global and regional aerosol emission estimates differ by a factor of up to 4 between different methods. Using a novel approach, we estimate daily total particulate matter (TPM) emissions from large wildfires in North American boreal and temperate regions. Moderate Resolution Imaging Spectroradiometer (MODIS) fire location and aerosol optical thickness (AOT) data sets are coupled with HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) atmospheric dispersion simulations, attributing identified smoke plumes to sources. Unlike previous approaches, the method (i) combines information from both satellite and AERONET (AErosol RObotic NETwork) observations to take into account aerosol water uptake and plume specific mass extinction efficiency when converting smoke AOT to TPM, and (ii) does not depend on instantaneous emission rates observed during individual satellite overpasses, which do not sample night-time emissions. The method also allows multiple independent estimates for the same emission period from imagery taken on consecutive days. Repeated fire-emitted AOT estimates for the same emission period over 2 to 3 days of plume evolution show increases in plume optical thickness by approximately 10 % for boreal events and by 40 % for temperate emissions. Inferred median water volume fractions for aged boreal and temperate smoke observations are 0.15 and 0.47 respectively, indicating that the increased AOT is partly explained by aerosol water uptake. TPM emission estimates for boreal events, which predominantly burn during daytime, agree closely with bottom-up Global Fire Emission Database (GFEDv4) and Global Fire Assimilation System (GFASv1.0) inventories, but are lower by approximately 30 % compared to Quick Fire Emission Dataset (QFEDv2) PM 2. 5 , and are higher by approximately a factor of 2 compared to Fire Energetics and Emissions Research (FEERv1) TPM estimates. The discrepancies are larger for ... Article in Journal/Newspaper Aerosol Robotic Network Directory of Open Access Journals: DOAJ Articles Atmospheric Chemistry and Physics 17 10 6423 6438 |
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Physics QC1-999 Chemistry QD1-999 |
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Physics QC1-999 Chemistry QD1-999 T. Nikonovas P. R. J. North S. H. Doerr Particulate emissions from large North American wildfires estimated using a new top-down method |
topic_facet |
Physics QC1-999 Chemistry QD1-999 |
description |
Particulate matter emissions from wildfires affect climate, weather and air quality. However, existing global and regional aerosol emission estimates differ by a factor of up to 4 between different methods. Using a novel approach, we estimate daily total particulate matter (TPM) emissions from large wildfires in North American boreal and temperate regions. Moderate Resolution Imaging Spectroradiometer (MODIS) fire location and aerosol optical thickness (AOT) data sets are coupled with HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) atmospheric dispersion simulations, attributing identified smoke plumes to sources. Unlike previous approaches, the method (i) combines information from both satellite and AERONET (AErosol RObotic NETwork) observations to take into account aerosol water uptake and plume specific mass extinction efficiency when converting smoke AOT to TPM, and (ii) does not depend on instantaneous emission rates observed during individual satellite overpasses, which do not sample night-time emissions. The method also allows multiple independent estimates for the same emission period from imagery taken on consecutive days. Repeated fire-emitted AOT estimates for the same emission period over 2 to 3 days of plume evolution show increases in plume optical thickness by approximately 10 % for boreal events and by 40 % for temperate emissions. Inferred median water volume fractions for aged boreal and temperate smoke observations are 0.15 and 0.47 respectively, indicating that the increased AOT is partly explained by aerosol water uptake. TPM emission estimates for boreal events, which predominantly burn during daytime, agree closely with bottom-up Global Fire Emission Database (GFEDv4) and Global Fire Assimilation System (GFASv1.0) inventories, but are lower by approximately 30 % compared to Quick Fire Emission Dataset (QFEDv2) PM 2. 5 , and are higher by approximately a factor of 2 compared to Fire Energetics and Emissions Research (FEERv1) TPM estimates. The discrepancies are larger for ... |
format |
Article in Journal/Newspaper |
author |
T. Nikonovas P. R. J. North S. H. Doerr |
author_facet |
T. Nikonovas P. R. J. North S. H. Doerr |
author_sort |
T. Nikonovas |
title |
Particulate emissions from large North American wildfires estimated using a new top-down method |
title_short |
Particulate emissions from large North American wildfires estimated using a new top-down method |
title_full |
Particulate emissions from large North American wildfires estimated using a new top-down method |
title_fullStr |
Particulate emissions from large North American wildfires estimated using a new top-down method |
title_full_unstemmed |
Particulate emissions from large North American wildfires estimated using a new top-down method |
title_sort |
particulate emissions from large north american wildfires estimated using a new top-down method |
publisher |
Copernicus Publications |
publishDate |
2017 |
url |
https://doi.org/10.5194/acp-17-6423-2017 https://doaj.org/article/3faf791606064e34971f84eabaf86596 |
genre |
Aerosol Robotic Network |
genre_facet |
Aerosol Robotic Network |
op_source |
Atmospheric Chemistry and Physics, Vol 17, Iss 10, Pp 6423-6438 (2017) |
op_relation |
http://www.atmos-chem-phys.net/17/6423/2017/acp-17-6423-2017.pdf https://doaj.org/toc/1680-7316 https://doaj.org/toc/1680-7324 1680-7316 1680-7324 doi:10.5194/acp-17-6423-2017 https://doaj.org/article/3faf791606064e34971f84eabaf86596 |
op_doi |
https://doi.org/10.5194/acp-17-6423-2017 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
17 |
container_issue |
10 |
container_start_page |
6423 |
op_container_end_page |
6438 |
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1766032729511559168 |