Understanding Sources and Drivers of Size-Resolved Aerosol in the High Arctic Islands of Svalbard Using a Receptor Model Coupled with Machine Learning

• Published in: Environmental Science & Technology
• Main Authors: Song, Congbo, Becagli, Silvia, Beddows, D.C.S., Brean, James, Browse, Jo, Dai, Qili, Dall'Osto, Manuel, Ferracci, Valerio, Harrison, Roy M., Harris, Neil R. P., Li, Weijun, Jones, Anna E., Kirchgäßner, Amélie, Kramawijaya, Agung Ghani, Kurganskiy, Alexander, Lupi, Angelo, Mazzola, Mauro, Severi, Mirko, Traversi, Rita, Shi, Zongbo
• Other Authors: Natural Environment Research Council (UK), Agencia Estatal de Investigación (España)
• Format: Article in Journal/Newspaper
• Language: English
• Published: American Chemical Society 2022
• Subjects: Arctic; Source apportionment; Positive matrix factorization; Machine learning; Particle number concentration; Meteorology; Svalbard; Climate change; Sea ice
• Online Access: http://hdl.handle.net/10261/278916; https://doi.org/10.1021/acs.est.1c07796; https://doi.org/10.13039/501100011033; https://doi.org/10.13039/501100000270

10 pages, 3 figures, 1 table, supporting information https://doi.org/10.1021/acs.est.1c07796 Atmospheric aerosols are important drivers of Arctic climate change through aerosol–cloud–climate interactions. However, large uncertainties remain on the sources and processes controlling particle numbers in both fine and coarse modes. Here, we applied a receptor model and an explainable machine learning technique to understand the sources and drivers of particle numbers from 10 nm to 20 μm in Svalbard. Nucleation, biogenic, secondary, anthropogenic, mineral dust, sea salt and blowing snow aerosols and their major environmental drivers were identified. Our results show that the monthly variations in particles are highly size/source dependent and regulated by meteorology. Secondary and nucleation aerosols are the largest contributors to potential cloud condensation nuclei (CCN, particle number with a diameter larger than 40 nm as a proxy) in the Arctic. Nonlinear responses to temperature were found for biogenic, local dust particles and potential CCN, highlighting the importance of melting sea ice and snow. These results indicate that the aerosol factors will respond to rapid Arctic warming differently and in a nonlinear fashion This research was supported by the Natural Environment Research Council (grant no. NE/S00579X/1) and endorsed by the Surface Ocean-Lower Atmosphere Study (SOLAS) With the institutional support of the ‘Severo Ochoa Centre of Excellence’ accreditation (CEX2019-000928-S) Peer reviewed