Creep of CarbFix basalt: influence of rock–fluid interaction
Geological carbon sequestration provides permanent CO 2 storage to mitigate the current high concentration of CO 2 in the atmosphere. CO 2 mineralization in basalts has been proven to be one of the most secure storage options. For successful implementation and future improvements of this technology,...
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ftcopernicus:oai:publications.copernicus.org:se97616 2023-05-15T16:50:47+02:00 Creep of CarbFix basalt: influence of rock–fluid interaction Xing, Tiange Ghaffari, Hamed O. Mok, Ulrich Pec, Matej 2022-01-14 application/pdf https://doi.org/10.5194/se-13-137-2022 https://se.copernicus.org/articles/13/137/2022/ eng eng doi:10.5194/se-13-137-2022 https://se.copernicus.org/articles/13/137/2022/ eISSN: 1869-9529 Text 2022 ftcopernicus https://doi.org/10.5194/se-13-137-2022 2022-01-17T17:22:17Z Geological carbon sequestration provides permanent CO 2 storage to mitigate the current high concentration of CO 2 in the atmosphere. CO 2 mineralization in basalts has been proven to be one of the most secure storage options. For successful implementation and future improvements of this technology, the time-dependent deformation behavior of reservoir rocks in the presence of reactive fluids needs to be studied in detail. We conducted load-stepping creep experiments on basalts from the CarbFix site (Iceland) under several pore fluid conditions (dry, H 2 O saturated and H 2 O + CO 2 saturated) at temperature, T ≈80 ∘ C and effective pressure, P eff =50 MPa, during which we collected mechanical, acoustic and pore fluid chemistry data. We observed transient creep at stresses as low as 11 % of the failure strength. Acoustic emissions (AEs) correlated strongly with strain accumulation, indicating that the creep deformation was a brittle process in agreement with microstructural observations. The rate and magnitude of AEs were higher in fluid-saturated experiments than in dry conditions. We infer that the predominant mechanism governing creep deformation is time- and stress-dependent subcritical dilatant cracking. Our results suggest that the presence of aqueous fluids exerts first-order control on creep deformation of basaltic rocks, while the composition of the fluids plays only a secondary role under the studied conditions. Text Iceland Copernicus Publications: E-Journals Solid Earth 13 1 137 160 |
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English |
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Geological carbon sequestration provides permanent CO 2 storage to mitigate the current high concentration of CO 2 in the atmosphere. CO 2 mineralization in basalts has been proven to be one of the most secure storage options. For successful implementation and future improvements of this technology, the time-dependent deformation behavior of reservoir rocks in the presence of reactive fluids needs to be studied in detail. We conducted load-stepping creep experiments on basalts from the CarbFix site (Iceland) under several pore fluid conditions (dry, H 2 O saturated and H 2 O + CO 2 saturated) at temperature, T ≈80 ∘ C and effective pressure, P eff =50 MPa, during which we collected mechanical, acoustic and pore fluid chemistry data. We observed transient creep at stresses as low as 11 % of the failure strength. Acoustic emissions (AEs) correlated strongly with strain accumulation, indicating that the creep deformation was a brittle process in agreement with microstructural observations. The rate and magnitude of AEs were higher in fluid-saturated experiments than in dry conditions. We infer that the predominant mechanism governing creep deformation is time- and stress-dependent subcritical dilatant cracking. Our results suggest that the presence of aqueous fluids exerts first-order control on creep deformation of basaltic rocks, while the composition of the fluids plays only a secondary role under the studied conditions. |
format |
Text |
author |
Xing, Tiange Ghaffari, Hamed O. Mok, Ulrich Pec, Matej |
spellingShingle |
Xing, Tiange Ghaffari, Hamed O. Mok, Ulrich Pec, Matej Creep of CarbFix basalt: influence of rock–fluid interaction |
author_facet |
Xing, Tiange Ghaffari, Hamed O. Mok, Ulrich Pec, Matej |
author_sort |
Xing, Tiange |
title |
Creep of CarbFix basalt: influence of rock–fluid interaction |
title_short |
Creep of CarbFix basalt: influence of rock–fluid interaction |
title_full |
Creep of CarbFix basalt: influence of rock–fluid interaction |
title_fullStr |
Creep of CarbFix basalt: influence of rock–fluid interaction |
title_full_unstemmed |
Creep of CarbFix basalt: influence of rock–fluid interaction |
title_sort |
creep of carbfix basalt: influence of rock–fluid interaction |
publishDate |
2022 |
url |
https://doi.org/10.5194/se-13-137-2022 https://se.copernicus.org/articles/13/137/2022/ |
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Iceland |
genre_facet |
Iceland |
op_source |
eISSN: 1869-9529 |
op_relation |
doi:10.5194/se-13-137-2022 https://se.copernicus.org/articles/13/137/2022/ |
op_doi |
https://doi.org/10.5194/se-13-137-2022 |
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Solid Earth |
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160 |
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1766040892511092736 |