Chemistry-climate model SOCOL-AERv2-BEv1 with the cosmogenic Beryllium-7 isotope cycle

• Main Authors: Golubenko, Kseniia, Rozanov, Eugene, Kovaltsov, Gennady, Leppänen, Ari-Pekka, Sukhodolov, Timofei, Usoskin, Ilya
• Format: Text
• Language: English
• Published: 2021
• Subjects: Canada; Kerguelen; Kerguelen Island; Northern Finland
• Online Access: https://doi.org/10.5194/gmd-2021-56; https://gmd.copernicus.org/preprints/gmd-2021-56/

Short-living cosmogenic isotope 7 Be, produced by cosmic rays in the atmosphere, is often used as a probe for atmospheric dynamics. Previously, modelling of the beryllium atmospheric transport was performed using simplified box-models or air back-tracing codes. While the ability of full atmospheric dynamics models to model beryllium transport was demonstrated earlier, no such ready-to-use model is currently available. Here we present the chemistry-climate model SOCOL-AERv2-BEv1 to trace isotopes of beryllium in the atmosphere. The SOCOL (SOlar Climate Ozone Links) model has been improved by including modules for the production, deposition, and transport of beryllium. Production was modelled considering both galactic and solar cosmic rays, by applying the CRAC (Cosmic-Ray induced Atmospheric Cascade) model. Radioactive decay of 7 Be was explicitly taken into account. Beryllium transport was modelled without additional gravitational settling due to the small size of the background aerosol particles. An interactive deposition scheme was applied including both wet and dry depositions. The modelling was performed, using a full nudging to the meteorological fields, for the period of 2003–2008 with a spin-up period of 1996–2002. The modelled concentrations of 7 Be in near-ground air were compared with the measured, at a weekly cadence, ones in four nearly antipodal high-latitude locations, two in Northern (Finland and Canada) and two in Southern (Chile and Kerguelen Island) hemispheres. The model results agree with the measurements in the absolute level within error bars, implying that the production, decay and lateral deposition are correctly reproduced by the model. The model also correctly reproduces the temporal variability of 7 Be concentrations on the annual and sub-annual scales, including a perfect reproduction of the annual cycle, dominating data in the Northern hemisphere. We also modelled the production and transport of 7 Be for a major solar energetic-particle event of 20-Jan-2005. Concluding, a new full 3D time-dependent model, based on the SOCOL-AERv2, of beryllium atmospheric production, transport and deposition has been developed. Comparison with the real data of 7 Be concentration in the near-ground air fully validates the model and its high accuracy.