TCCON and NDACC XCO measurements: difference, discussion and application
Column-averaged dry-air mole fraction of CO (X CO ) measurements are obtained from two ground-based Fourier transform infrared (FTIR) spectrometer networks: the Total Carbon Column Observing Network (TCCON) and the Network for the Detection of Atmospheric Composition Change (NDACC). In this study, t...
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ftcopernicus:oai:publications.copernicus.org:amt77856 2023-05-15T17:48:29+02:00 TCCON and NDACC XCO measurements: difference, discussion and application Zhou, Minqiang Langerock, Bavo Vigouroux, Corinne Sha, Mahesh Kumar Hermans, Christian Metzger, Jean-Marc Chen, Huilin Ramonet, Michel Kivi, Rigel Heikkinen, Pauli Smale, Dan Pollard, David F. Jones, Nicholas Velazco, Voltaire A. García, Omaira E. Schneider, Matthias Palm, Mathias Warneke, Thorsten Mazière, Martine 2019-11-18 application/pdf https://doi.org/10.5194/amt-12-5979-2019 https://amt.copernicus.org/articles/12/5979/2019/ eng eng doi:10.5194/amt-12-5979-2019 https://amt.copernicus.org/articles/12/5979/2019/ eISSN: 1867-8548 Text 2019 ftcopernicus https://doi.org/10.5194/amt-12-5979-2019 2020-07-20T16:22:35Z Column-averaged dry-air mole fraction of CO (X CO ) measurements are obtained from two ground-based Fourier transform infrared (FTIR) spectrometer networks: the Total Carbon Column Observing Network (TCCON) and the Network for the Detection of Atmospheric Composition Change (NDACC). In this study, the differences between the TCCON and NDACC X CO measurements are investigated and discussed based on six NDACC–TCCON sites using data over the period 2007–2017. A direct comparison shows that the NDACC X CO measurements are about 5.5 % larger than the TCCON data at Ny-Ålesund, Bremen, and Izaña (Northern Hemisphere), and the absolute bias between the NDACC and TCCON data is within 2 % at Saint-Denis, Wollongong and Lauder (Southern Hemisphere). The hemispheric dependence of the bias is mainly attributed to their smoothing errors. The systematic smoothing error of the TCCON X CO data varies in the range between 0.2 % (Bremen) and 7.9 % (Lauder), and the random smoothing error varies in the range between 2.0 % and 3.6 %. The systematic smoothing error of NDACC data is between 0.1 % and 0.8 %, and the random smoothing error of NDACC data is about 0.3 %. For TCCON data, the smoothing error is significant because it is higher than the reported uncertainty, particularly at Southern Hemisphere sites. To reduce the influence from the a priori profiles and different vertical sensitivities, the scaled NDACC a priori profiles are used as the common a priori profiles for comparing TCCON and NDACC retrievals. As a result, the biases between TCCON and NDACC X CO measurements become more consistent (5.6 %–8.5 %) with a mean value of 6.8 % at these sites. To determine the sources of the remaining bias, regular AirCore measurements at Orléans and Sodankylä are compared to co-located TCCON measurements. It is found that TCCON X CO measurements are 6.1 ± 1.6 % and 8.0 ± 3.2 % smaller than the AirCore measurements at Orléans and Sodankylä, respectively, indicating that the scaling factor of TCCON X CO data should be around 1.0000 instead of 1.0672. Further investigations should be carried out in the TCCON community to determine the correct scaling factor to be applied to the TCCON X CO data. This paper also demonstrates that the smoothing error must be taken into account when comparing FTIR X CO data, and especially TCCON X CO data, with model or satellite data. Text Ny Ålesund Ny-Ålesund Sodankylä Copernicus Publications: E-Journals Ny-Ålesund Sodankylä ENVELOPE(26.600,26.600,67.417,67.417) Atmospheric Measurement Techniques 12 11 5979 5995 |
institution |
Open Polar |
collection |
Copernicus Publications: E-Journals |
op_collection_id |
ftcopernicus |
language |
English |
description |
Column-averaged dry-air mole fraction of CO (X CO ) measurements are obtained from two ground-based Fourier transform infrared (FTIR) spectrometer networks: the Total Carbon Column Observing Network (TCCON) and the Network for the Detection of Atmospheric Composition Change (NDACC). In this study, the differences between the TCCON and NDACC X CO measurements are investigated and discussed based on six NDACC–TCCON sites using data over the period 2007–2017. A direct comparison shows that the NDACC X CO measurements are about 5.5 % larger than the TCCON data at Ny-Ålesund, Bremen, and Izaña (Northern Hemisphere), and the absolute bias between the NDACC and TCCON data is within 2 % at Saint-Denis, Wollongong and Lauder (Southern Hemisphere). The hemispheric dependence of the bias is mainly attributed to their smoothing errors. The systematic smoothing error of the TCCON X CO data varies in the range between 0.2 % (Bremen) and 7.9 % (Lauder), and the random smoothing error varies in the range between 2.0 % and 3.6 %. The systematic smoothing error of NDACC data is between 0.1 % and 0.8 %, and the random smoothing error of NDACC data is about 0.3 %. For TCCON data, the smoothing error is significant because it is higher than the reported uncertainty, particularly at Southern Hemisphere sites. To reduce the influence from the a priori profiles and different vertical sensitivities, the scaled NDACC a priori profiles are used as the common a priori profiles for comparing TCCON and NDACC retrievals. As a result, the biases between TCCON and NDACC X CO measurements become more consistent (5.6 %–8.5 %) with a mean value of 6.8 % at these sites. To determine the sources of the remaining bias, regular AirCore measurements at Orléans and Sodankylä are compared to co-located TCCON measurements. It is found that TCCON X CO measurements are 6.1 ± 1.6 % and 8.0 ± 3.2 % smaller than the AirCore measurements at Orléans and Sodankylä, respectively, indicating that the scaling factor of TCCON X CO data should be around 1.0000 instead of 1.0672. Further investigations should be carried out in the TCCON community to determine the correct scaling factor to be applied to the TCCON X CO data. This paper also demonstrates that the smoothing error must be taken into account when comparing FTIR X CO data, and especially TCCON X CO data, with model or satellite data. |
format |
Text |
author |
Zhou, Minqiang Langerock, Bavo Vigouroux, Corinne Sha, Mahesh Kumar Hermans, Christian Metzger, Jean-Marc Chen, Huilin Ramonet, Michel Kivi, Rigel Heikkinen, Pauli Smale, Dan Pollard, David F. Jones, Nicholas Velazco, Voltaire A. García, Omaira E. Schneider, Matthias Palm, Mathias Warneke, Thorsten Mazière, Martine |
spellingShingle |
Zhou, Minqiang Langerock, Bavo Vigouroux, Corinne Sha, Mahesh Kumar Hermans, Christian Metzger, Jean-Marc Chen, Huilin Ramonet, Michel Kivi, Rigel Heikkinen, Pauli Smale, Dan Pollard, David F. Jones, Nicholas Velazco, Voltaire A. García, Omaira E. Schneider, Matthias Palm, Mathias Warneke, Thorsten Mazière, Martine TCCON and NDACC XCO measurements: difference, discussion and application |
author_facet |
Zhou, Minqiang Langerock, Bavo Vigouroux, Corinne Sha, Mahesh Kumar Hermans, Christian Metzger, Jean-Marc Chen, Huilin Ramonet, Michel Kivi, Rigel Heikkinen, Pauli Smale, Dan Pollard, David F. Jones, Nicholas Velazco, Voltaire A. García, Omaira E. Schneider, Matthias Palm, Mathias Warneke, Thorsten Mazière, Martine |
author_sort |
Zhou, Minqiang |
title |
TCCON and NDACC XCO measurements: difference, discussion and application |
title_short |
TCCON and NDACC XCO measurements: difference, discussion and application |
title_full |
TCCON and NDACC XCO measurements: difference, discussion and application |
title_fullStr |
TCCON and NDACC XCO measurements: difference, discussion and application |
title_full_unstemmed |
TCCON and NDACC XCO measurements: difference, discussion and application |
title_sort |
tccon and ndacc xco measurements: difference, discussion and application |
publishDate |
2019 |
url |
https://doi.org/10.5194/amt-12-5979-2019 https://amt.copernicus.org/articles/12/5979/2019/ |
long_lat |
ENVELOPE(26.600,26.600,67.417,67.417) |
geographic |
Ny-Ålesund Sodankylä |
geographic_facet |
Ny-Ålesund Sodankylä |
genre |
Ny Ålesund Ny-Ålesund Sodankylä |
genre_facet |
Ny Ålesund Ny-Ålesund Sodankylä |
op_source |
eISSN: 1867-8548 |
op_relation |
doi:10.5194/amt-12-5979-2019 https://amt.copernicus.org/articles/12/5979/2019/ |
op_doi |
https://doi.org/10.5194/amt-12-5979-2019 |
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Atmospheric Measurement Techniques |
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12 |
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11 |
container_start_page |
5979 |
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5995 |
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1766154567654834176 |