A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy

Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-sca...

Full description

Bibliographic Details
Published in:Atmospheric Measurement Techniques
Main Authors: Seidl, Andrew W., Sodemann, Harald, Steen-Larsen, Hans Christian
Format: Text
Language:English
Published: 2023
Subjects:
Online Access:https://doi.org/10.5194/amt-16-769-2023
https://amt.copernicus.org/articles/16/769/2023/
id ftcopernicus:oai:publications.copernicus.org:amt105069
record_format openpolar
spelling ftcopernicus:oai:publications.copernicus.org:amt105069 2023-05-15T15:05:07+02:00 A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy Seidl, Andrew W. Sodemann, Harald Steen-Larsen, Hans Christian 2023-02-09 application/pdf https://doi.org/10.5194/amt-16-769-2023 https://amt.copernicus.org/articles/16/769/2023/ eng eng doi:10.5194/amt-16-769-2023 https://amt.copernicus.org/articles/16/769/2023/ eISSN: 1867-8548 Text 2023 ftcopernicus https://doi.org/10.5194/amt-16-769-2023 2023-02-13T17:22:55Z Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-scale exchanges taking place between the surface and atmosphere. It is especially important to resolve the vertical structure of these processes. We have designed the ISE-CUBE system as a modular CRDS deployment system for profiling stable water isotopes in the surface layer, specifically the lowermost 2 m above the surface. We tested the system during a 2-week field campaign during February–March 2020 in Ny-Ålesund, Svalbard, Norway, with ambient temperatures down to −30 ∘ C. The system functioned suitably throughout the campaign, with field periods exhibiting only a marginal increase in isotopic measurement uncertainty (30 %) as compared to optimal laboratory operation. Over the 2 m profiling range, we have been able to measure and resolve gradients on the temporal and spatial scales needed in an Arctic environment. Text Arctic Ny Ålesund Ny-Ålesund Svalbard Copernicus Publications: E-Journals Arctic Norway Ny-Ålesund Svalbard Atmospheric Measurement Techniques 16 3 769 790
institution Open Polar
collection Copernicus Publications: E-Journals
op_collection_id ftcopernicus
language English
description Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-scale exchanges taking place between the surface and atmosphere. It is especially important to resolve the vertical structure of these processes. We have designed the ISE-CUBE system as a modular CRDS deployment system for profiling stable water isotopes in the surface layer, specifically the lowermost 2 m above the surface. We tested the system during a 2-week field campaign during February–March 2020 in Ny-Ålesund, Svalbard, Norway, with ambient temperatures down to −30 ∘ C. The system functioned suitably throughout the campaign, with field periods exhibiting only a marginal increase in isotopic measurement uncertainty (30 %) as compared to optimal laboratory operation. Over the 2 m profiling range, we have been able to measure and resolve gradients on the temporal and spatial scales needed in an Arctic environment.
format Text
author Seidl, Andrew W.
Sodemann, Harald
Steen-Larsen, Hans Christian
spellingShingle Seidl, Andrew W.
Sodemann, Harald
Steen-Larsen, Hans Christian
A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
author_facet Seidl, Andrew W.
Sodemann, Harald
Steen-Larsen, Hans Christian
author_sort Seidl, Andrew W.
title A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_short A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_full A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_fullStr A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_full_unstemmed A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_sort modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
publishDate 2023
url https://doi.org/10.5194/amt-16-769-2023
https://amt.copernicus.org/articles/16/769/2023/
geographic Arctic
Norway
Ny-Ålesund
Svalbard
geographic_facet Arctic
Norway
Ny-Ålesund
Svalbard
genre Arctic
Ny Ålesund
Ny-Ålesund
Svalbard
genre_facet Arctic
Ny Ålesund
Ny-Ålesund
Svalbard
op_source eISSN: 1867-8548
op_relation doi:10.5194/amt-16-769-2023
https://amt.copernicus.org/articles/16/769/2023/
op_doi https://doi.org/10.5194/amt-16-769-2023
container_title Atmospheric Measurement Techniques
container_volume 16
container_issue 3
container_start_page 769
op_container_end_page 790
_version_ 1766336872398716928