Present and future aerosol impacts on Arctic climate change in the GISS-E2.1 Earth system model

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Im, Ulas, Tsigaridis, Kostas, Faluvegi, Gregory, Langen, Peter L., French, Joshua P., Mahmood, Rashed, Thomas, Manu A., Salzen, Knut, Thomas, Daniel C., Whaley, Cynthia H., Klimont, Zbigniew, Skov, Henrik, Brandt, Jørgen
• Format: Text
• Language: English
• Published: 2021
• Subjects: Arctic; Ari; black carbon; Climate change; Sea ice
• Online Access: https://doi.org/10.5194/acp-21-10413-2021; https://acp.copernicus.org/articles/21/10413/2021/

The Arctic is warming 2 to 3 times faster than the global average, partly due to changes in short-lived climate forcers (SLCFs) including aerosols. In order to study the effects of atmospheric aerosols in this warming, recent past (1990–2014) and future (2015–2050) simulations have been carried out using the GISS-E2.1 Earth system model to study the aerosol burdens and their radiative and climate impacts over the Arctic ( >60 ∘ N), using anthropogenic emissions from the Eclipse V6b and the Coupled Model Intercomparison Project Phase 6 (CMIP6) databases, while global annual mean greenhouse gas concentrations were prescribed and kept fixed in all simulations. Results showed that the simulations have underestimated observed surface aerosol levels, in particular black carbon (BC) and sulfate ( <math xmlns="http://www.w3.org/1998/Math/MathML" id="M3" display="inline" overflow="scroll" dspmath="mathml"><mrow class="chem"><msubsup><mi mathvariant="normal">SO</mi><mn mathvariant="normal">4</mn><mrow><mn mathvariant="normal">2</mn><mo>-</mo></mrow></msubsup></mrow></math> <svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="29pt" height="17pt" class="svg-formula" dspmath="mathimg" md5hash="6060a0eb6022af681aa55d19b3180df9"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-10413-2021-ie00001.svg" width="29pt" height="17pt" src="acp-21-10413-2021-ie00001.png"/></svg:svg> ), by more than 50 %, with the smallest biases calculated for the atmosphere-only simulations, where winds are nudged to reanalysis data. CMIP6 simulations performed slightly better in reproducing the observed surface aerosol concentrations and climate parameters, compared to the Eclipse simulations. In addition, simulations where atmosphere and ocean are fully coupled had slightly smaller biases in aerosol levels compared to atmosphere-only simulations without nudging. Arctic BC, organic aerosol (OA), and <math xmlns="http://www.w3.org/1998/Math/MathML" id="M4" display="inline" overflow="scroll" dspmath="mathml"><mrow class="chem"><msubsup><mi mathvariant="normal">SO</mi><mn mathvariant="normal">4</mn><mrow><mn mathvariant="normal">2</mn><mo>-</mo></mrow></msubsup></mrow></math> <svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="29pt" height="17pt" class="svg-formula" dspmath="mathimg" md5hash="544235742d8f4a0f97153436b699bab8"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-10413-2021-ie00002.svg" width="29pt" height="17pt" src="acp-21-10413-2021-ie00002.png"/></svg:svg> burdens decrease significantly in all simulations by 10 %–60 % following the reductions of 7 %–78 % in emission projections, with the Eclipse ensemble showing larger reductions in Arctic aerosol burdens compared to the CMIP6 ensemble. For the 2030–2050 period, the Eclipse ensemble simulated a radiative forcing due to aerosol–radiation interactions ( RF ARI ) of <math xmlns="http://www.w3.org/1998/Math/MathML" id="M6" display="inline" overflow="scroll" dspmath="mathml"><mrow><mo>-</mo><mn mathvariant="normal">0.39</mn><mo>±</mo><mn mathvariant="normal">0.01</mn></mrow></math> <svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="64pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="aafee4724c88d7325eca1cf08d50e976"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-10413-2021-ie00003.svg" width="64pt" height="10pt" src="acp-21-10413-2021-ie00003.png"/></svg:svg> W m −2 , which is −0.08 W m −2 larger than the 1990–2010 mean forcing ( −0.32 W m −2 ), of which <math xmlns="http://www.w3.org/1998/Math/MathML" id="M12" display="inline" overflow="scroll" dspmath="mathml"><mrow><mo>-</mo><mn mathvariant="normal">0.24</mn><mo>±</mo><mn mathvariant="normal">0.01</mn></mrow></math> <svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="64pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="a0c6a8aaa00926f494c19262568b2d9a"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-10413-2021-ie00004.svg" width="64pt" height="10pt" src="acp-21-10413-2021-ie00004.png"/></svg:svg> W m −2 was attributed to the anthropogenic aerosols. The CMIP6 ensemble simulated a RF ARI of −0.35 to −0.40 W m −2 for the same period, which is −0.01 to −0.06 W m −2 larger than the 1990–2010 mean forcing of −0.35 W m −2 . The scenarios with little to no mitigation (worst-case scenarios) led to very small changes in the RF ARI , while scenarios with medium to large emission mitigations led to increases in the negative RF ARI , mainly due to the decrease in the positive BC forcing and the decrease in the negative <math xmlns="http://www.w3.org/1998/Math/MathML" id="M25" display="inline" overflow="scroll" dspmath="mathml"><mrow class="chem"><msubsup><mi mathvariant="normal">SO</mi><mn mathvariant="normal">4</mn><mrow><mn mathvariant="normal">2</mn><mo>-</mo></mrow></msubsup></mrow></math> <svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="29pt" height="17pt" class="svg-formula" dspmath="mathimg" md5hash="66431dc7c7d5e1df65243409a551c241"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-10413-2021-ie00005.svg" width="29pt" height="17pt" src="acp-21-10413-2021-ie00005.png"/></svg:svg> forcing. The anthropogenic aerosols accounted for −0.24 to −0.26 W m −2 of the net RF ARI in 2030–2050 period, in Eclipse and CMIP6 ensembles, respectively. Finally, all simulations showed an increase in the Arctic surface air temperatures throughout the simulation period. By 2050, surface air temperatures are projected to increase by 2.4 to 2.6 ∘ C in the Eclipse ensemble and 1.9 to 2.6 ∘ C in the CMIP6 ensemble, compared to the 1990–2010 mean. Overall, results show that even the scenarios with largest emission reductions leads to similar impact on the future Arctic surface air temperatures and sea-ice extent compared to scenarios with smaller emission reductions, implying reductions of greenhouse emissions are still necessary to mitigate climate change.