MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves

Space borne infrared limb emission measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) reveal the formation of a belt of polar stratospheric clouds (PSCs) of nitric acid trihydrate (NAT) particles over Antarctica in mid-June 2003. By mesoscale microphysical simulati...

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Published in:Atmospheric Chemistry and Physics
Main Authors: Höpfner, M., Larsen, N., Spang, R., Luo, B. P., Ma, J., Svendsen, S. H., Eckermann, S. D., Knudsen, B., Massoli, P., Cairo, F., Stiller, G., Clarmann, T., Fischer, H.
Format: Text
Language:English
Published: 2018
Subjects:
Online Access:https://doi.org/10.5194/acp-6-1221-2006
https://www.atmos-chem-phys.net/6/1221/2006/
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spelling ftcopernicus:oai:publications.copernicus.org:acp4253 2023-05-15T13:55:27+02:00 MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves Höpfner, M. Larsen, N. Spang, R. Luo, B. P. Ma, J. Svendsen, S. H. Eckermann, S. D. Knudsen, B. Massoli, P. Cairo, F. Stiller, G. Clarmann, T. Fischer, H. 2018-06-28 application/pdf https://doi.org/10.5194/acp-6-1221-2006 https://www.atmos-chem-phys.net/6/1221/2006/ eng eng doi:10.5194/acp-6-1221-2006 https://www.atmos-chem-phys.net/6/1221/2006/ eISSN: 1680-7324 Text 2018 ftcopernicus https://doi.org/10.5194/acp-6-1221-2006 2019-12-24T09:58:54Z Space borne infrared limb emission measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) reveal the formation of a belt of polar stratospheric clouds (PSCs) of nitric acid trihydrate (NAT) particles over Antarctica in mid-June 2003. By mesoscale microphysical simulations we show that this sudden onset of NAT PSCs was caused by heterogeneous nucleation on ice in the cooling phases of large-amplitude stratospheric mountain waves over the Antarctic Peninsula and the Ellsworth Mountains. MIPAS observations of PSCs before this event show no indication for the presence of NAT clouds with volume densities larger than about 0.3 µm 3 /cm 3 and radii smaller than 3 µm, but are consistent with supercooled droplets of ternary H 2 SO 4 /HNO 3 /H 2 O solution (STS). Simulations indicate that homogeneous surface nucleation rates have to be reduced by three orders of magnitude to comply with the observations. Text Antarc* Antarctic Antarctic Peninsula Antarctica Copernicus Publications: E-Journals Antarctic Antarctic Peninsula Ellsworth Mountains ENVELOPE(-85.000,-85.000,-78.750,-78.750) The Antarctic Atmospheric Chemistry and Physics 6 5 1221 1230
institution Open Polar
collection Copernicus Publications: E-Journals
op_collection_id ftcopernicus
language English
description Space borne infrared limb emission measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) reveal the formation of a belt of polar stratospheric clouds (PSCs) of nitric acid trihydrate (NAT) particles over Antarctica in mid-June 2003. By mesoscale microphysical simulations we show that this sudden onset of NAT PSCs was caused by heterogeneous nucleation on ice in the cooling phases of large-amplitude stratospheric mountain waves over the Antarctic Peninsula and the Ellsworth Mountains. MIPAS observations of PSCs before this event show no indication for the presence of NAT clouds with volume densities larger than about 0.3 µm 3 /cm 3 and radii smaller than 3 µm, but are consistent with supercooled droplets of ternary H 2 SO 4 /HNO 3 /H 2 O solution (STS). Simulations indicate that homogeneous surface nucleation rates have to be reduced by three orders of magnitude to comply with the observations.
format Text
author Höpfner, M.
Larsen, N.
Spang, R.
Luo, B. P.
Ma, J.
Svendsen, S. H.
Eckermann, S. D.
Knudsen, B.
Massoli, P.
Cairo, F.
Stiller, G.
Clarmann, T.
Fischer, H.
spellingShingle Höpfner, M.
Larsen, N.
Spang, R.
Luo, B. P.
Ma, J.
Svendsen, S. H.
Eckermann, S. D.
Knudsen, B.
Massoli, P.
Cairo, F.
Stiller, G.
Clarmann, T.
Fischer, H.
MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
author_facet Höpfner, M.
Larsen, N.
Spang, R.
Luo, B. P.
Ma, J.
Svendsen, S. H.
Eckermann, S. D.
Knudsen, B.
Massoli, P.
Cairo, F.
Stiller, G.
Clarmann, T.
Fischer, H.
author_sort Höpfner, M.
title MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
title_short MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
title_full MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
title_fullStr MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
title_full_unstemmed MIPAS detects Antarctic stratospheric belt of NAT PSCs caused by mountain waves
title_sort mipas detects antarctic stratospheric belt of nat pscs caused by mountain waves
publishDate 2018
url https://doi.org/10.5194/acp-6-1221-2006
https://www.atmos-chem-phys.net/6/1221/2006/
long_lat ENVELOPE(-85.000,-85.000,-78.750,-78.750)
geographic Antarctic
Antarctic Peninsula
Ellsworth Mountains
The Antarctic
geographic_facet Antarctic
Antarctic Peninsula
Ellsworth Mountains
The Antarctic
genre Antarc*
Antarctic
Antarctic Peninsula
Antarctica
genre_facet Antarc*
Antarctic
Antarctic Peninsula
Antarctica
op_source eISSN: 1680-7324
op_relation doi:10.5194/acp-6-1221-2006
https://www.atmos-chem-phys.net/6/1221/2006/
op_doi https://doi.org/10.5194/acp-6-1221-2006
container_title Atmospheric Chemistry and Physics
container_volume 6
container_issue 5
container_start_page 1221
op_container_end_page 1230
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