Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe
Ground-based Fourier transform infrared (FTIR) measurements of solar absorption spectra can provide ozone total columns with a precision of 2% but also independent partial column amounts in about four vertical layers, one in the troposphere and three in the stratosphere up to about 45km, with a prec...
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ftcopernicus:oai:publications.copernicus.org:acp26257 2023-05-15T13:43:09+02:00 Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe Vigouroux, C. Blumenstock, T. Coffey, M. Errera, Q. García, O. Jones, N. B. Hannigan, J. W. Hase, F. Liley, B. Mahieu, E. Mellqvist, J. Notholt, J. Palm, M. Persson, G. Schneider, M. Servais, C. Smale, D. Thölix, L. De Mazière, M. 2018-09-11 application/pdf https://doi.org/10.5194/acp-15-2915-2015 https://www.atmos-chem-phys.net/15/2915/2015/ eng eng doi:10.5194/acp-15-2915-2015 https://www.atmos-chem-phys.net/15/2915/2015/ eISSN: 1680-7324 Text 2018 ftcopernicus https://doi.org/10.5194/acp-15-2915-2015 2019-12-24T09:53:41Z Ground-based Fourier transform infrared (FTIR) measurements of solar absorption spectra can provide ozone total columns with a precision of 2% but also independent partial column amounts in about four vertical layers, one in the troposphere and three in the stratosphere up to about 45km, with a precision of 5–6%. We use eight of the Network for the Detection of Atmospheric Composition Change (NDACC) stations having a long-term time series of FTIR ozone measurements to study the total and vertical ozone trends and variability, namely, Ny-Ålesund (79° N), Thule (77° N), Kiruna (68° N), Harestua (60° N), Jungfraujoch (47° N), Izaña (28° N), Wollongong (34° S) and Lauder (45° S). The length of the FTIR time series varies by station but is typically from about 1995 to present. We applied to the monthly means of the ozone total and four partial columns a stepwise multiple regression model including the following proxies: solar cycle, quasi-biennial oscillation (QBO), El Niño–Southern Oscillation (ENSO), Arctic and Antarctic Oscillation (AO/AAO), tropopause pressure (TP), equivalent latitude (EL), Eliassen–Palm flux (EPF), and volume of polar stratospheric clouds (VPSC). At the Arctic stations, the trends are found mostly negative in the troposphere and lower stratosphere, very mixed in the middle stratosphere, positive in the upper stratosphere due to a large increase in the 1995–2003 period, and non-significant when considering the total columns. The trends for mid-latitude and subtropical stations are all non-significant, except at Lauder in the troposphere and upper stratosphere and at Wollongong for the total columns and the lower and middle stratospheric columns where they are found positive. At Jungfraujoch, the upper stratospheric trend is close to significance (+0.9 ± 1.0% decade −1 ). Therefore, some signs of the onset of ozone mid-latitude recovery are observed only in the Southern Hemisphere, while a few more years seem to be needed to observe it at the northern mid-latitude station. Text Antarc* Antarctic Arctic Kiruna Ny Ålesund Ny-Ålesund Copernicus Publications: E-Journals Antarctic Arctic Kiruna Ny-Ålesund Atmospheric Chemistry and Physics 15 6 2915 2933 |
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Open Polar |
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Copernicus Publications: E-Journals |
op_collection_id |
ftcopernicus |
language |
English |
description |
Ground-based Fourier transform infrared (FTIR) measurements of solar absorption spectra can provide ozone total columns with a precision of 2% but also independent partial column amounts in about four vertical layers, one in the troposphere and three in the stratosphere up to about 45km, with a precision of 5–6%. We use eight of the Network for the Detection of Atmospheric Composition Change (NDACC) stations having a long-term time series of FTIR ozone measurements to study the total and vertical ozone trends and variability, namely, Ny-Ålesund (79° N), Thule (77° N), Kiruna (68° N), Harestua (60° N), Jungfraujoch (47° N), Izaña (28° N), Wollongong (34° S) and Lauder (45° S). The length of the FTIR time series varies by station but is typically from about 1995 to present. We applied to the monthly means of the ozone total and four partial columns a stepwise multiple regression model including the following proxies: solar cycle, quasi-biennial oscillation (QBO), El Niño–Southern Oscillation (ENSO), Arctic and Antarctic Oscillation (AO/AAO), tropopause pressure (TP), equivalent latitude (EL), Eliassen–Palm flux (EPF), and volume of polar stratospheric clouds (VPSC). At the Arctic stations, the trends are found mostly negative in the troposphere and lower stratosphere, very mixed in the middle stratosphere, positive in the upper stratosphere due to a large increase in the 1995–2003 period, and non-significant when considering the total columns. The trends for mid-latitude and subtropical stations are all non-significant, except at Lauder in the troposphere and upper stratosphere and at Wollongong for the total columns and the lower and middle stratospheric columns where they are found positive. At Jungfraujoch, the upper stratospheric trend is close to significance (+0.9 ± 1.0% decade −1 ). Therefore, some signs of the onset of ozone mid-latitude recovery are observed only in the Southern Hemisphere, while a few more years seem to be needed to observe it at the northern mid-latitude station. |
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Text |
author |
Vigouroux, C. Blumenstock, T. Coffey, M. Errera, Q. García, O. Jones, N. B. Hannigan, J. W. Hase, F. Liley, B. Mahieu, E. Mellqvist, J. Notholt, J. Palm, M. Persson, G. Schneider, M. Servais, C. Smale, D. Thölix, L. De Mazière, M. |
spellingShingle |
Vigouroux, C. Blumenstock, T. Coffey, M. Errera, Q. García, O. Jones, N. B. Hannigan, J. W. Hase, F. Liley, B. Mahieu, E. Mellqvist, J. Notholt, J. Palm, M. Persson, G. Schneider, M. Servais, C. Smale, D. Thölix, L. De Mazière, M. Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
author_facet |
Vigouroux, C. Blumenstock, T. Coffey, M. Errera, Q. García, O. Jones, N. B. Hannigan, J. W. Hase, F. Liley, B. Mahieu, E. Mellqvist, J. Notholt, J. Palm, M. Persson, G. Schneider, M. Servais, C. Smale, D. Thölix, L. De Mazière, M. |
author_sort |
Vigouroux, C. |
title |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
title_short |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
title_full |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
title_fullStr |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
title_full_unstemmed |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
title_sort |
trends of ozone total columns and vertical distribution from ftir observations at eight ndacc stations around the globe |
publishDate |
2018 |
url |
https://doi.org/10.5194/acp-15-2915-2015 https://www.atmos-chem-phys.net/15/2915/2015/ |
geographic |
Antarctic Arctic Kiruna Ny-Ålesund |
geographic_facet |
Antarctic Arctic Kiruna Ny-Ålesund |
genre |
Antarc* Antarctic Arctic Kiruna Ny Ålesund Ny-Ålesund |
genre_facet |
Antarc* Antarctic Arctic Kiruna Ny Ålesund Ny-Ålesund |
op_source |
eISSN: 1680-7324 |
op_relation |
doi:10.5194/acp-15-2915-2015 https://www.atmos-chem-phys.net/15/2915/2015/ |
op_doi |
https://doi.org/10.5194/acp-15-2915-2015 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
15 |
container_issue |
6 |
container_start_page |
2915 |
op_container_end_page |
2933 |
_version_ |
1766185307508572160 |