Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption
Black carbon (BC) aerosol has important effects on the climate and hydrology of the Tibetan Plateau (TP). An intensive measurement campaign was conducted at Lulang (similar to 3300 m a.s.l. - above sea level), southeastern TP, from September to October 2015, to investigate the sources and physicoche...
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ftchinacascieeca:oai:ir.ieecas.cn:361006/5209 2023-06-11T04:12:44+02:00 Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption Wang, Qiyuan Cao, Junji Han, Yongming Tian, Jie Zhu, Chongshu Zhang, Yonggang Zhang, Ningning Shen, Zhenxing Ni, Haiyan Zhao, Shuyu Wu, Jiarui 2018-04-05 http://ir.ieecas.cn/handle/361006/5209 https://doi.org/10.5194/acp-18-4639-2018 英语 eng ATMOSPHERIC CHEMISTRY AND PHYSICS http://ir.ieecas.cn/handle/361006/5209 doi:10.5194/acp-18-4639-2018 Science & Technology Physical Sciences PARTICLE SOOT PHOTOMETER BROWN CARBON SIZE DISTRIBUTION CLIMATE-CHANGE COASTAL CITY SOUTH CHINA ICE CORE STATE GLACIER HIMALAYAS Meteorology & Atmospheric Sciences Article 期刊论文 2018 ftchinacascieeca https://doi.org/10.5194/acp-18-4639-2018 2023-05-08T13:22:44Z Black carbon (BC) aerosol has important effects on the climate and hydrology of the Tibetan Plateau (TP). An intensive measurement campaign was conducted at Lulang (similar to 3300 m a.s.l. - above sea level), southeastern TP, from September to October 2015, to investigate the sources and physicochemical characteristics of refractory BC (rBC) aerosol. The average rBC mass concentration was 0.31 +/- 0.55 mu g m(-3), which is higher than most prior results for BC on the TP. A clear diurnal cycle in rBC showed high values in the morning and low values in the afternoon. A bivariate polar plot showed that rBC loadings varied with wind speed and direction, which also reflected the dominant transport direction. The estimated net surface rBC transport intensity was +/- 0.05 +/- 0.29 mu g s(-1) m(-2), indicating stronger transport from outside the TP compared with its interior. Cluster analysis and a concentration-weighted trajectory model connected emissions from north India to the high rBC loadings, but the effects of internal TP sources should not be overlooked. The average mass median diameter (MMD) of rBC was 160 +/- 23 nm, with smaller MMDs on rainy days (145 nm) compared with non-rainy days (164 nm). The average number fraction of thickly coated rBC (F-rBC) was 39 +/- 8 %, and it increased with the O-3 mixing ratios from 10:00 to 14:00 LT, indicating that photochemical oxidation played a role in forming rBC coatings. The average rBC absorption enhancement (E-abs) was estimated to be 1.9, suggesting that light absorption by coated rBC particles was greater than for uncoated ones. The E-abs was strongly positively correlated with the F-rBC, indicating an amplification of light absorption for internally mixed rBC. For rBC cores < 170 nm, E-abs was negatively correlated with MMD, but it was nearly constant for rBC cores > 170 nm. Our study provides insight into the sources and evolution of rBC aerosol on the TP, and the results should be useful for improving models of the radiative effects of carbonaceous ... Article in Journal/Newspaper ice core Institute of Earth Environment: IEECAS OpenIR (Chinese Academy of Sciences) Atmospheric Chemistry and Physics 18 7 4639 4656 |
institution |
Open Polar |
collection |
Institute of Earth Environment: IEECAS OpenIR (Chinese Academy of Sciences) |
op_collection_id |
ftchinacascieeca |
language |
English |
topic |
Science & Technology Physical Sciences PARTICLE SOOT PHOTOMETER BROWN CARBON SIZE DISTRIBUTION CLIMATE-CHANGE COASTAL CITY SOUTH CHINA ICE CORE STATE GLACIER HIMALAYAS Meteorology & Atmospheric Sciences |
spellingShingle |
Science & Technology Physical Sciences PARTICLE SOOT PHOTOMETER BROWN CARBON SIZE DISTRIBUTION CLIMATE-CHANGE COASTAL CITY SOUTH CHINA ICE CORE STATE GLACIER HIMALAYAS Meteorology & Atmospheric Sciences Wang, Qiyuan Cao, Junji Han, Yongming Tian, Jie Zhu, Chongshu Zhang, Yonggang Zhang, Ningning Shen, Zhenxing Ni, Haiyan Zhao, Shuyu Wu, Jiarui Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
topic_facet |
Science & Technology Physical Sciences PARTICLE SOOT PHOTOMETER BROWN CARBON SIZE DISTRIBUTION CLIMATE-CHANGE COASTAL CITY SOUTH CHINA ICE CORE STATE GLACIER HIMALAYAS Meteorology & Atmospheric Sciences |
description |
Black carbon (BC) aerosol has important effects on the climate and hydrology of the Tibetan Plateau (TP). An intensive measurement campaign was conducted at Lulang (similar to 3300 m a.s.l. - above sea level), southeastern TP, from September to October 2015, to investigate the sources and physicochemical characteristics of refractory BC (rBC) aerosol. The average rBC mass concentration was 0.31 +/- 0.55 mu g m(-3), which is higher than most prior results for BC on the TP. A clear diurnal cycle in rBC showed high values in the morning and low values in the afternoon. A bivariate polar plot showed that rBC loadings varied with wind speed and direction, which also reflected the dominant transport direction. The estimated net surface rBC transport intensity was +/- 0.05 +/- 0.29 mu g s(-1) m(-2), indicating stronger transport from outside the TP compared with its interior. Cluster analysis and a concentration-weighted trajectory model connected emissions from north India to the high rBC loadings, but the effects of internal TP sources should not be overlooked. The average mass median diameter (MMD) of rBC was 160 +/- 23 nm, with smaller MMDs on rainy days (145 nm) compared with non-rainy days (164 nm). The average number fraction of thickly coated rBC (F-rBC) was 39 +/- 8 %, and it increased with the O-3 mixing ratios from 10:00 to 14:00 LT, indicating that photochemical oxidation played a role in forming rBC coatings. The average rBC absorption enhancement (E-abs) was estimated to be 1.9, suggesting that light absorption by coated rBC particles was greater than for uncoated ones. The E-abs was strongly positively correlated with the F-rBC, indicating an amplification of light absorption for internally mixed rBC. For rBC cores < 170 nm, E-abs was negatively correlated with MMD, but it was nearly constant for rBC cores > 170 nm. Our study provides insight into the sources and evolution of rBC aerosol on the TP, and the results should be useful for improving models of the radiative effects of carbonaceous ... |
format |
Article in Journal/Newspaper |
author |
Wang, Qiyuan Cao, Junji Han, Yongming Tian, Jie Zhu, Chongshu Zhang, Yonggang Zhang, Ningning Shen, Zhenxing Ni, Haiyan Zhao, Shuyu Wu, Jiarui |
author_facet |
Wang, Qiyuan Cao, Junji Han, Yongming Tian, Jie Zhu, Chongshu Zhang, Yonggang Zhang, Ningning Shen, Zhenxing Ni, Haiyan Zhao, Shuyu Wu, Jiarui |
author_sort |
Wang, Qiyuan |
title |
Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
title_short |
Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
title_full |
Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
title_fullStr |
Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
title_full_unstemmed |
Sources and physicochemical characteristics of black carbon aerosol from the southeastern Tibetan Plateau: internal mixing enhances light absorption |
title_sort |
sources and physicochemical characteristics of black carbon aerosol from the southeastern tibetan plateau: internal mixing enhances light absorption |
publishDate |
2018 |
url |
http://ir.ieecas.cn/handle/361006/5209 https://doi.org/10.5194/acp-18-4639-2018 |
genre |
ice core |
genre_facet |
ice core |
op_relation |
ATMOSPHERIC CHEMISTRY AND PHYSICS http://ir.ieecas.cn/handle/361006/5209 doi:10.5194/acp-18-4639-2018 |
op_doi |
https://doi.org/10.5194/acp-18-4639-2018 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
18 |
container_issue |
7 |
container_start_page |
4639 |
op_container_end_page |
4656 |
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1768388782879408128 |