Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor
The effects of the flow rates of cyclopentane (CP) and methane gas, operating pressure, and experimental temperature on the formation of c-yclopentane-methane hydrate were investigated using a novel bubble column reactor. The results indicated that, with either an increase of the operating pressure...
Published in: | Industrial & Engineering Chemistry Research |
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Online Access: | http://ir.giec.ac.cn/handle/344007/10568 https://doi.org/10.1021/ie202422c |
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ftchacadsciegiec:oai:ir.giec.ac.cn:344007/10568 2023-05-15T17:11:52+02:00 Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor Lv, Qiu-Nan Li, Xiao-Sen Xu, Chun-Gang Chen, Zhao-Yang 2012-05-02 http://ir.giec.ac.cn/handle/344007/10568 https://doi.org/10.1021/ie202422c 英语 eng INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH http://ir.giec.ac.cn/handle/344007/10568 doi:10.1021/ie202422c Science & Technology Technology Engineering GAS HYDRATE CARBON-DIOXIDE CAPTURE CO2 WATER Chemical Article 期刊论文 2012 ftchacadsciegiec https://doi.org/10.1021/ie202422c 2022-09-23T14:12:28Z The effects of the flow rates of cyclopentane (CP) and methane gas, operating pressure, and experimental temperature on the formation of c-yclopentane-methane hydrate were investigated using a novel bubble column reactor. The results indicated that, with either an increase of the operating pressure or a decrease of the experimental temperature, the induction time decreased whereas the cumulative gas consumption and gas conversion ratio increased. In addition, with an increase of the flow rate of methane gas, the induction time decreased, whereas the cumulative gas consumption increased. The gas conversion ratio increased first from 61.5% to 93.1% when the flow rate of methane gas increased from 159 to 234 mL/min and then decreased from 93.1% to 83.2% when the flow rate of methane gas continuously increased from 234 mL/min to 308.9 mL/min. This decrease was attributed to an increase of the discharge rate of methane from the reactor. It was noted the average methane consumption rate could be effectively enhanced with an increase of the flow rate of gas at relatively low pressure and high temperature. The flow rate of CP had a minimal effect on the cumulative gas consumption and gas conversion ratio. However, an increase of the flow rate of CP could reduce the induction time. Article in Journal/Newspaper Methane hydrate Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences: GIEC OpenIR Industrial & Engineering Chemistry Research 51 17 5967 5975 |
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Open Polar |
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Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences: GIEC OpenIR |
op_collection_id |
ftchacadsciegiec |
language |
English |
topic |
Science & Technology Technology Engineering GAS HYDRATE CARBON-DIOXIDE CAPTURE CO2 WATER Chemical |
spellingShingle |
Science & Technology Technology Engineering GAS HYDRATE CARBON-DIOXIDE CAPTURE CO2 WATER Chemical Lv, Qiu-Nan Li, Xiao-Sen Xu, Chun-Gang Chen, Zhao-Yang Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
topic_facet |
Science & Technology Technology Engineering GAS HYDRATE CARBON-DIOXIDE CAPTURE CO2 WATER Chemical |
description |
The effects of the flow rates of cyclopentane (CP) and methane gas, operating pressure, and experimental temperature on the formation of c-yclopentane-methane hydrate were investigated using a novel bubble column reactor. The results indicated that, with either an increase of the operating pressure or a decrease of the experimental temperature, the induction time decreased whereas the cumulative gas consumption and gas conversion ratio increased. In addition, with an increase of the flow rate of methane gas, the induction time decreased, whereas the cumulative gas consumption increased. The gas conversion ratio increased first from 61.5% to 93.1% when the flow rate of methane gas increased from 159 to 234 mL/min and then decreased from 93.1% to 83.2% when the flow rate of methane gas continuously increased from 234 mL/min to 308.9 mL/min. This decrease was attributed to an increase of the discharge rate of methane from the reactor. It was noted the average methane consumption rate could be effectively enhanced with an increase of the flow rate of gas at relatively low pressure and high temperature. The flow rate of CP had a minimal effect on the cumulative gas consumption and gas conversion ratio. However, an increase of the flow rate of CP could reduce the induction time. |
format |
Article in Journal/Newspaper |
author |
Lv, Qiu-Nan Li, Xiao-Sen Xu, Chun-Gang Chen, Zhao-Yang |
author_facet |
Lv, Qiu-Nan Li, Xiao-Sen Xu, Chun-Gang Chen, Zhao-Yang |
author_sort |
Lv, Qiu-Nan |
title |
Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
title_short |
Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
title_full |
Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
title_fullStr |
Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
title_full_unstemmed |
Experimental Investigation of the Formation of Cyclopentane-Methane Hydrate in a Novel and Large-Size Bubble Column Reactor |
title_sort |
experimental investigation of the formation of cyclopentane-methane hydrate in a novel and large-size bubble column reactor |
publishDate |
2012 |
url |
http://ir.giec.ac.cn/handle/344007/10568 https://doi.org/10.1021/ie202422c |
genre |
Methane hydrate |
genre_facet |
Methane hydrate |
op_relation |
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH http://ir.giec.ac.cn/handle/344007/10568 doi:10.1021/ie202422c |
op_doi |
https://doi.org/10.1021/ie202422c |
container_title |
Industrial & Engineering Chemistry Research |
container_volume |
51 |
container_issue |
17 |
container_start_page |
5967 |
op_container_end_page |
5975 |
_version_ |
1766068624506748928 |