Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity
Isoprene is important to the formation of secondary organic aerosols and can change the atmospheric oxidation capacity in the remote marine environment. However, the influencing factors of marine atmospheric isoprene are still unclear. Here, we report observed atmospheric isoprene in ambient air alo...
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ftchacadscgigcas:oai:ir.gig.ac.cn:344008/70796 2024-09-15T17:53:31+00:00 Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity Yu, Xiawei Zhang, Yanli Jin, Ruilin Chai, Zhangyan Hu, Qihou Yu, Juan Xing, Jie Zhang, Lulu Kang, Hui Zhang, Yanxu Wang, Xinming Xie, Zhouqing 2023 http://ir.gig.ac.cn/handle/344008/70796 https://doi.org/10.1016/j.atmosenv.2022.119414 英语 eng PERGAMON-ELSEVIER SCIENCE LTD ATMOSPHERIC ENVIRONMENT http://ir.gig.ac.cn/handle/344008/70796 doi:10.1016/j.atmosenv.2022.119414 Environmental Sciences & Ecology Meteorology & Atmospheric Sciences Isoprene Spatial distribution Influencing factors Marine emission capacity Atmospheric removal capacity Environmental Sciences NONMETHANE HYDROCARBONS BOUNDARY-LAYER ARCTIC-OCEAN DIMETHYL SULFIDE SURFACE OCEAN INDIAN-OCEAN NEW-MODEL EMISSIONS OXIDATION SEA 期刊论文 2023 ftchacadscgigcas https://doi.org/10.1016/j.atmosenv.2022.119414 2024-07-29T14:03:11Z Isoprene is important to the formation of secondary organic aerosols and can change the atmospheric oxidation capacity in the remote marine environment. However, the influencing factors of marine atmospheric isoprene are still unclear. Here, we report observed atmospheric isoprene in ambient air along three cruises path from the Arctic Ocean to the Southern Ocean. The levels of isoprene ranged from not detected (ND) to 452 pptv, with an average value of 48 +/- 81 pptv, with large variability. A negative correlation was found between isoprene and latitude (r =-0.40, p < 0.01). The spatial distributions of isoprene flux from oceanic phytoplankton by the modelled results were different from those of observed atmospheric isoprene. The observed isoprene concen-tration was 2-3 orders of magnitude higher than the model estimation. Environmental variables such as tem-perature, wind speed (WS), sea surface temperature (SST), salinity and atmospheric removal capacity can influence the distribution of isoprene. At latitudes north of 60<degrees>S, the marine emission capacity was relatively important and contributed 45.06%. Atmospheric removal capacity was the most important factor for atmo-spheric isoprene, contributing 55.05% to the concentration of atmospheric isoprene in latitudes south of 60 degrees S. Low atmospheric oxidation capacity and wind speed cause high atmospheric isoprene in the Southern Ocean in summer and will eventually affect secondary organic aerosol concentrations. Report Arctic Ocean Phytoplankton Southern Ocean Guangzhou Institute of Geochemistry: GIG OpenIR (Chinese Academy of Sciences) Atmospheric Environment 292 119414 |
institution |
Open Polar |
collection |
Guangzhou Institute of Geochemistry: GIG OpenIR (Chinese Academy of Sciences) |
op_collection_id |
ftchacadscgigcas |
language |
English |
topic |
Environmental Sciences & Ecology Meteorology & Atmospheric Sciences Isoprene Spatial distribution Influencing factors Marine emission capacity Atmospheric removal capacity Environmental Sciences NONMETHANE HYDROCARBONS BOUNDARY-LAYER ARCTIC-OCEAN DIMETHYL SULFIDE SURFACE OCEAN INDIAN-OCEAN NEW-MODEL EMISSIONS OXIDATION SEA |
spellingShingle |
Environmental Sciences & Ecology Meteorology & Atmospheric Sciences Isoprene Spatial distribution Influencing factors Marine emission capacity Atmospheric removal capacity Environmental Sciences NONMETHANE HYDROCARBONS BOUNDARY-LAYER ARCTIC-OCEAN DIMETHYL SULFIDE SURFACE OCEAN INDIAN-OCEAN NEW-MODEL EMISSIONS OXIDATION SEA Yu, Xiawei Zhang, Yanli Jin, Ruilin Chai, Zhangyan Hu, Qihou Yu, Juan Xing, Jie Zhang, Lulu Kang, Hui Zhang, Yanxu Wang, Xinming Xie, Zhouqing Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
topic_facet |
Environmental Sciences & Ecology Meteorology & Atmospheric Sciences Isoprene Spatial distribution Influencing factors Marine emission capacity Atmospheric removal capacity Environmental Sciences NONMETHANE HYDROCARBONS BOUNDARY-LAYER ARCTIC-OCEAN DIMETHYL SULFIDE SURFACE OCEAN INDIAN-OCEAN NEW-MODEL EMISSIONS OXIDATION SEA |
description |
Isoprene is important to the formation of secondary organic aerosols and can change the atmospheric oxidation capacity in the remote marine environment. However, the influencing factors of marine atmospheric isoprene are still unclear. Here, we report observed atmospheric isoprene in ambient air along three cruises path from the Arctic Ocean to the Southern Ocean. The levels of isoprene ranged from not detected (ND) to 452 pptv, with an average value of 48 +/- 81 pptv, with large variability. A negative correlation was found between isoprene and latitude (r =-0.40, p < 0.01). The spatial distributions of isoprene flux from oceanic phytoplankton by the modelled results were different from those of observed atmospheric isoprene. The observed isoprene concen-tration was 2-3 orders of magnitude higher than the model estimation. Environmental variables such as tem-perature, wind speed (WS), sea surface temperature (SST), salinity and atmospheric removal capacity can influence the distribution of isoprene. At latitudes north of 60<degrees>S, the marine emission capacity was relatively important and contributed 45.06%. Atmospheric removal capacity was the most important factor for atmo-spheric isoprene, contributing 55.05% to the concentration of atmospheric isoprene in latitudes south of 60 degrees S. Low atmospheric oxidation capacity and wind speed cause high atmospheric isoprene in the Southern Ocean in summer and will eventually affect secondary organic aerosol concentrations. |
format |
Report |
author |
Yu, Xiawei Zhang, Yanli Jin, Ruilin Chai, Zhangyan Hu, Qihou Yu, Juan Xing, Jie Zhang, Lulu Kang, Hui Zhang, Yanxu Wang, Xinming Xie, Zhouqing |
author_facet |
Yu, Xiawei Zhang, Yanli Jin, Ruilin Chai, Zhangyan Hu, Qihou Yu, Juan Xing, Jie Zhang, Lulu Kang, Hui Zhang, Yanxu Wang, Xinming Xie, Zhouqing |
author_sort |
Yu, Xiawei |
title |
Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
title_short |
Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
title_full |
Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
title_fullStr |
Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
title_full_unstemmed |
Spatial distribution of marine atmospheric isoprene in the Southern Hemisphere: Role of atmospheric removal capacity |
title_sort |
spatial distribution of marine atmospheric isoprene in the southern hemisphere: role of atmospheric removal capacity |
publisher |
PERGAMON-ELSEVIER SCIENCE LTD |
publishDate |
2023 |
url |
http://ir.gig.ac.cn/handle/344008/70796 https://doi.org/10.1016/j.atmosenv.2022.119414 |
genre |
Arctic Ocean Phytoplankton Southern Ocean |
genre_facet |
Arctic Ocean Phytoplankton Southern Ocean |
op_relation |
ATMOSPHERIC ENVIRONMENT http://ir.gig.ac.cn/handle/344008/70796 doi:10.1016/j.atmosenv.2022.119414 |
op_doi |
https://doi.org/10.1016/j.atmosenv.2022.119414 |
container_title |
Atmospheric Environment |
container_volume |
292 |
container_start_page |
119414 |
_version_ |
1810429387655348224 |