Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4
International audience Anthropogenic pollution and wildfires are main producers of carbon monoxide (CO) and black carbon (BC) in the Northern Hemisphere. High concentrations of these compounds are transported into the Arctic troposphere, influencing the ecosystem in high northern latitudes and the g...
Main Authors: | , , , , , , , , , , , , , , , , |
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Other Authors: | , , , , , , , , , , , , , , , , , , , , , , , , , , , |
Format: | Report |
Language: | English |
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HAL CCSD
2015
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Subjects: | |
Online Access: | https://hal.science/hal-00568788 https://hal.science/hal-00568788/document https://hal.science/hal-00568788/file/acpd-11-5935-2011.pdf https://doi.org/10.5194/acpd-11-5935-2011 |
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ftceafr:oai:HAL:hal-00568788v1 |
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record_format |
openpolar |
institution |
Open Polar |
collection |
HAL-CEA (Commissariat à l'énergie atomique et aux énergies alternatives) |
op_collection_id |
ftceafr |
language |
English |
topic |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes |
spellingShingle |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes Tilmes, S. Emmons, L. K. Law, Kathy S. Ancellet, Gérard Schlager, H. Paris, J.-D. Fuelberg, Henry E. Streets, D. G. Wiedinmyer, C. Diskin, G. S. Kondo, Y. Holloway, J. Schwarz, J. P. Spackman, J. R. Campos, T. Nédélec, P. Panchenko, M. V. Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
topic_facet |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes |
description |
International audience Anthropogenic pollution and wildfires are main producers of carbon monoxide (CO) and black carbon (BC) in the Northern Hemisphere. High concentrations of these compounds are transported into the Arctic troposphere, influencing the ecosystem in high northern latitudes and the global climate. The global chemical transport model MOZART-4 is used to quantify the seasonal evolution of the contribution of CO and BC from different source regions in spring and summer 2008 by tagging their emissions. Aircraft observations from the POLARCAT experiments, in particular NASA ARCTAS, NOAA ARCPAC, POLARCAT-France, DLR GRACE and YAK-AEROSIB, as well as the NSF START08/preHIPPO experiments during Spring-Summer 2008 are combined to quantify the representation of simulated tracer characteristics in anthropogenic and fire plumes. In general, the model reproduces CO and BC well. Based on aircraft measurements and FLEXPART back-trajectories, the altitude contribution of emissions coming from different source regions is well captured in the model. Uncertainties of the MOZART-4 model are identified by comparing the data with model results on the flight tracks and using MOPITT satellite observations. Anthropogenic emissions are underestimated by about 10% in high northern latitudes in spring, and shortcomings exist in simulating fire plumes. The remote impact of East-Siberian fire emissions is underestimated for spring, whereas the impact of Southeast Asian fire emissions to mid-latitude CO values is overestimated by the model. In summer, mid-latitude CO values agree well between model and observations, whereas summer high latitude East-Siberian fire emissions in the model are overestimated by 20% in comparison to observations in the region. On the other hand, CO concentrations are underestimated by about 30% over Alaska and Canada at altitudes above 4 km. BC values are overestimated by the model at altitudes above 4 km in summer. Based on MOZART-4, with tagged CO and BC tracers, anthropogenic emissions of Asia, ... |
author2 |
National Center for Atmospheric Research Boulder (NCAR) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) DLR Institut für Physik der Atmosphäre = DLR Institute of Atmospheric Physics (IPA) Deutsches Zentrum für Luft- und Raumfahrt Oberpfaffenhofen-Wessling (DLR) Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA) ICOS-RAMCES (ICOS-RAMCES) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Department of Earth, Ocean and Atmospheric Science Tallahassee (FSU Florida State University Tallahassee (FSU) Argonne National Laboratory Lemont (ANL) NASA Langley Research Center Hampton (LaRC) Research Center for Advanced Science and Technology Tokyo (RCAST) The University of Tokyo (UTokyo) NOAA Earth System Research Laboratory (ESRL) National Oceanic and Atmospheric Administration (NOAA) Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado Boulder -National Oceanic and Atmospheric Administration (NOAA) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) V.E. Zuev Institute of Atmospheric Optics (IAO) Siberian Branch of the Russian Academy of Sciences (SB RAS) |
format |
Report |
author |
Tilmes, S. Emmons, L. K. Law, Kathy S. Ancellet, Gérard Schlager, H. Paris, J.-D. Fuelberg, Henry E. Streets, D. G. Wiedinmyer, C. Diskin, G. S. Kondo, Y. Holloway, J. Schwarz, J. P. Spackman, J. R. Campos, T. Nédélec, P. Panchenko, M. V. |
author_facet |
Tilmes, S. Emmons, L. K. Law, Kathy S. Ancellet, Gérard Schlager, H. Paris, J.-D. Fuelberg, Henry E. Streets, D. G. Wiedinmyer, C. Diskin, G. S. Kondo, Y. Holloway, J. Schwarz, J. P. Spackman, J. R. Campos, T. Nédélec, P. Panchenko, M. V. |
author_sort |
Tilmes, S. |
title |
Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
title_short |
Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
title_full |
Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
title_fullStr |
Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
title_full_unstemmed |
Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 |
title_sort |
source contributions to northern hemisphere co and black carbon during spring and summer 2008 from polarcat and start08/prehippo observations and mozart-4 |
publisher |
HAL CCSD |
publishDate |
2015 |
url |
https://hal.science/hal-00568788 https://hal.science/hal-00568788/document https://hal.science/hal-00568788/file/acpd-11-5935-2011.pdf https://doi.org/10.5194/acpd-11-5935-2011 |
geographic |
Arctic Canada |
geographic_facet |
Arctic Canada |
genre |
Arctic black carbon Alaska |
genre_facet |
Arctic black carbon Alaska |
op_source |
ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00568788 2015 |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.5194/acpd-11-5935-2011 hal-00568788 https://hal.science/hal-00568788 https://hal.science/hal-00568788/document https://hal.science/hal-00568788/file/acpd-11-5935-2011.pdf doi:10.5194/acpd-11-5935-2011 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.5194/acpd-11-5935-2011 |
_version_ |
1801373237770190848 |
spelling |
ftceafr:oai:HAL:hal-00568788v1 2024-06-09T07:44:30+00:00 Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4 Tilmes, S. Emmons, L. K. Law, Kathy S. Ancellet, Gérard Schlager, H. Paris, J.-D. Fuelberg, Henry E. Streets, D. G. Wiedinmyer, C. Diskin, G. S. Kondo, Y. Holloway, J. Schwarz, J. P. Spackman, J. R. Campos, T. Nédélec, P. Panchenko, M. V. National Center for Atmospheric Research Boulder (NCAR) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) DLR Institut für Physik der Atmosphäre = DLR Institute of Atmospheric Physics (IPA) Deutsches Zentrum für Luft- und Raumfahrt Oberpfaffenhofen-Wessling (DLR) Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA) ICOS-RAMCES (ICOS-RAMCES) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Department of Earth, Ocean and Atmospheric Science Tallahassee (FSU Florida State University Tallahassee (FSU) Argonne National Laboratory Lemont (ANL) NASA Langley Research Center Hampton (LaRC) Research Center for Advanced Science and Technology Tokyo (RCAST) The University of Tokyo (UTokyo) NOAA Earth System Research Laboratory (ESRL) National Oceanic and Atmospheric Administration (NOAA) Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado Boulder -National Oceanic and Atmospheric Administration (NOAA) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) V.E. Zuev Institute of Atmospheric Optics (IAO) Siberian Branch of the Russian Academy of Sciences (SB RAS) 2015-12-22 https://hal.science/hal-00568788 https://hal.science/hal-00568788/document https://hal.science/hal-00568788/file/acpd-11-5935-2011.pdf https://doi.org/10.5194/acpd-11-5935-2011 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/acpd-11-5935-2011 hal-00568788 https://hal.science/hal-00568788 https://hal.science/hal-00568788/document https://hal.science/hal-00568788/file/acpd-11-5935-2011.pdf doi:10.5194/acpd-11-5935-2011 info:eu-repo/semantics/OpenAccess ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00568788 2015 [SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes info:eu-repo/semantics/preprint Preprints, Working Papers, . 2015 ftceafr https://doi.org/10.5194/acpd-11-5935-2011 2024-05-16T15:35:58Z International audience Anthropogenic pollution and wildfires are main producers of carbon monoxide (CO) and black carbon (BC) in the Northern Hemisphere. High concentrations of these compounds are transported into the Arctic troposphere, influencing the ecosystem in high northern latitudes and the global climate. The global chemical transport model MOZART-4 is used to quantify the seasonal evolution of the contribution of CO and BC from different source regions in spring and summer 2008 by tagging their emissions. Aircraft observations from the POLARCAT experiments, in particular NASA ARCTAS, NOAA ARCPAC, POLARCAT-France, DLR GRACE and YAK-AEROSIB, as well as the NSF START08/preHIPPO experiments during Spring-Summer 2008 are combined to quantify the representation of simulated tracer characteristics in anthropogenic and fire plumes. In general, the model reproduces CO and BC well. Based on aircraft measurements and FLEXPART back-trajectories, the altitude contribution of emissions coming from different source regions is well captured in the model. Uncertainties of the MOZART-4 model are identified by comparing the data with model results on the flight tracks and using MOPITT satellite observations. Anthropogenic emissions are underestimated by about 10% in high northern latitudes in spring, and shortcomings exist in simulating fire plumes. The remote impact of East-Siberian fire emissions is underestimated for spring, whereas the impact of Southeast Asian fire emissions to mid-latitude CO values is overestimated by the model. In summer, mid-latitude CO values agree well between model and observations, whereas summer high latitude East-Siberian fire emissions in the model are overestimated by 20% in comparison to observations in the region. On the other hand, CO concentrations are underestimated by about 30% over Alaska and Canada at altitudes above 4 km. BC values are overestimated by the model at altitudes above 4 km in summer. Based on MOZART-4, with tagged CO and BC tracers, anthropogenic emissions of Asia, ... Report Arctic black carbon Alaska HAL-CEA (Commissariat à l'énergie atomique et aux énergies alternatives) Arctic Canada |