Future changes in stratospheric ozone and the role of heterogeneous chemistry
International audience HETEROGENEOUS chemical reactions on the surfaces of solid or liquid particles present in the lower stratosphere may be an important influence on the levels of ozone depletion resulting from increased concentrations of anthropogenic chlorine compounds in the atmosphere1. Such p...
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ftccsdartic:oai:HAL:insu-03585805v1 2023-05-15T13:57:38+02:00 Future changes in stratospheric ozone and the role of heterogeneous chemistry Brasseur, Guy, Granier, Claire Walters, Stacy Atmospheric Chemistry Division Boulder National Center for Atmospheric Research Boulder (NCAR) Service d'aéronomie (SA) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) 1990-12 https://hal-insu.archives-ouvertes.fr/insu-03585805 https://doi.org/10.1038/348626a0 en eng HAL CCSD Nature Publishing Group info:eu-repo/semantics/altIdentifier/doi/10.1038/348626a0 insu-03585805 https://hal-insu.archives-ouvertes.fr/insu-03585805 doi:10.1038/348626a0 ISSN: 0028-0836 EISSN: 1476-4687 Nature https://hal-insu.archives-ouvertes.fr/insu-03585805 Nature, 1990, 348 (6302), pp.626-628. ⟨10.1038/348626a0⟩ [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere info:eu-repo/semantics/article Journal articles 1990 ftccsdartic https://doi.org/10.1038/348626a0 2023-03-19T05:18:23Z International audience HETEROGENEOUS chemical reactions on the surfaces of solid or liquid particles present in the lower stratosphere may be an important influence on the levels of ozone depletion resulting from increased concentrations of anthropogenic chlorine compounds in the atmosphere1. Such processes, occurring on ice particles in polar stratospheric clouds, have been invoked to explain the formation of the springtime ozone hole over Antarctica2,3. Sulphuric acid aerosols injected into the atmosphere following a volcanic eruption may also provide sites for heterogeneous chemistry leading to ozone depletion4. Here we present model calculations that assess the importance of heterogeneous processes in future ozone depletion, assuming that trace-gas concentrations follow the protocol agreed at the recent international convention in London. We find that, even if this protocol is adhered to, reactions on the surface of sulphuric acid aerosol particles could produce significant ozone depletion into the beginning of the next century, especially if a major volcanic eruption (similar to the El Chichón eruption of 19824) takes place. Article in Journal/Newspaper Antarc* Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) Nature 348 6302 626 628 |
institution |
Open Polar |
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Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) |
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ftccsdartic |
language |
English |
topic |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
spellingShingle |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere Brasseur, Guy, Granier, Claire Walters, Stacy Future changes in stratospheric ozone and the role of heterogeneous chemistry |
topic_facet |
[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
description |
International audience HETEROGENEOUS chemical reactions on the surfaces of solid or liquid particles present in the lower stratosphere may be an important influence on the levels of ozone depletion resulting from increased concentrations of anthropogenic chlorine compounds in the atmosphere1. Such processes, occurring on ice particles in polar stratospheric clouds, have been invoked to explain the formation of the springtime ozone hole over Antarctica2,3. Sulphuric acid aerosols injected into the atmosphere following a volcanic eruption may also provide sites for heterogeneous chemistry leading to ozone depletion4. Here we present model calculations that assess the importance of heterogeneous processes in future ozone depletion, assuming that trace-gas concentrations follow the protocol agreed at the recent international convention in London. We find that, even if this protocol is adhered to, reactions on the surface of sulphuric acid aerosol particles could produce significant ozone depletion into the beginning of the next century, especially if a major volcanic eruption (similar to the El Chichón eruption of 19824) takes place. |
author2 |
Atmospheric Chemistry Division Boulder National Center for Atmospheric Research Boulder (NCAR) Service d'aéronomie (SA) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) |
format |
Article in Journal/Newspaper |
author |
Brasseur, Guy, Granier, Claire Walters, Stacy |
author_facet |
Brasseur, Guy, Granier, Claire Walters, Stacy |
author_sort |
Brasseur, Guy, |
title |
Future changes in stratospheric ozone and the role of heterogeneous chemistry |
title_short |
Future changes in stratospheric ozone and the role of heterogeneous chemistry |
title_full |
Future changes in stratospheric ozone and the role of heterogeneous chemistry |
title_fullStr |
Future changes in stratospheric ozone and the role of heterogeneous chemistry |
title_full_unstemmed |
Future changes in stratospheric ozone and the role of heterogeneous chemistry |
title_sort |
future changes in stratospheric ozone and the role of heterogeneous chemistry |
publisher |
HAL CCSD |
publishDate |
1990 |
url |
https://hal-insu.archives-ouvertes.fr/insu-03585805 https://doi.org/10.1038/348626a0 |
genre |
Antarc* |
genre_facet |
Antarc* |
op_source |
ISSN: 0028-0836 EISSN: 1476-4687 Nature https://hal-insu.archives-ouvertes.fr/insu-03585805 Nature, 1990, 348 (6302), pp.626-628. ⟨10.1038/348626a0⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.1038/348626a0 insu-03585805 https://hal-insu.archives-ouvertes.fr/insu-03585805 doi:10.1038/348626a0 |
op_doi |
https://doi.org/10.1038/348626a0 |
container_title |
Nature |
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348 |
container_issue |
6302 |
container_start_page |
626 |
op_container_end_page |
628 |
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1766265354480254976 |