Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget
Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-round flux and concentration observations from...
Published in: | Elementa: Science of the Anthropocene |
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Main Authors: | , , , , , , , , , , , , , , , , , , , , |
Other Authors: | , , , , |
Format: | Article in Journal/Newspaper |
Language: | English |
Published: |
HAL CCSD
2023
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Subjects: | |
Online Access: | https://hal.science/hal-04292739 https://hal.science/hal-04292739/document https://hal.science/hal-04292739/file/Bartenetal_Elementa2023.pdf https://doi.org/10.1525/elementa.2022.00086 |
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Open Polar |
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Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) |
op_collection_id |
ftccsdartic |
language |
English |
topic |
Ozone deposition Arctic ozone Modelling Atmospheric boundary layer [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces environment [SDU.STU.GL]Sciences of the Universe [physics]/Earth Sciences/Glaciology |
spellingShingle |
Ozone deposition Arctic ozone Modelling Atmospheric boundary layer [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces environment [SDU.STU.GL]Sciences of the Universe [physics]/Earth Sciences/Glaciology Barten, Johannes, G M Ganzeveld, Laurens, N Steeneveld, Gert-Jan Blomquist, Byron, W Angot, Hélène Archer, Stephen, D Bariteau, Ludovic Beck, Ivo Boyer, Matthew von der Gathen, Peter Helmig, Detlev Howard, Dean Hueber, Jacques Jacobi, Hans-Werner Jokinen, Tuija Laurila, Tiia Posman, Kevin, M Quéléver, Lauriane Schmale, Julia Shupe, Matthew, D Krol, Maarten, C Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
topic_facet |
Ozone deposition Arctic ozone Modelling Atmospheric boundary layer [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces environment [SDU.STU.GL]Sciences of the Universe [physics]/Earth Sciences/Glaciology |
description |
Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-round flux and concentration observations from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) campaign and simulations with a single-column atmospheric chemistry and meteorological model (SCM). Based on eddy-covariance O3 surface flux observations, we find a median surface resistance on the order of 20,000 s m−1, resulting in a dry deposition velocity of approximately 0.005 cm s−1. This surface resistance is up to an order of magnitude larger than traditionally used values in many atmospheric chemistry and transport models. The SCM is able to accurately represent the yearly cycle, with maxima above 40 ppb in the winter and minima around 15 ppb at the end of summer. However, the observed springtime ozone depletion events are not captured by the SCM. In winter, the modelled PBL O3 budget is governed by dry deposition at the surface mostly compensated by downward turbulent transport of O3 towards the surface. Advection, which is accounted for implicitly by nudging to reanalysis data, poses a substantial, mostly negative, contribution to the simulated PBL O3 budget in summer. During episodes with low wind speed (<5 m s−1) and shallow PBL (<50 m), the 7-day mean dry deposition removal rate can reach up to 1.0 ppb h−1. Our study highlights the importance of an accurate description of dry deposition to Arctic sea ice in models to quantify the current and future O3 sink in the Arctic, impacting the tropospheric O3 budget, which has been modified in the last century largely due to anthropogenic activities. |
author2 |
Ecole Polytechnique Fédérale de Lausanne (EPFL) University of Colorado Boulder Institut des Géosciences de l’Environnement (IGE) Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ) Université Grenoble Alpes (UGA) |
format |
Article in Journal/Newspaper |
author |
Barten, Johannes, G M Ganzeveld, Laurens, N Steeneveld, Gert-Jan Blomquist, Byron, W Angot, Hélène Archer, Stephen, D Bariteau, Ludovic Beck, Ivo Boyer, Matthew von der Gathen, Peter Helmig, Detlev Howard, Dean Hueber, Jacques Jacobi, Hans-Werner Jokinen, Tuija Laurila, Tiia Posman, Kevin, M Quéléver, Lauriane Schmale, Julia Shupe, Matthew, D Krol, Maarten, C |
author_facet |
Barten, Johannes, G M Ganzeveld, Laurens, N Steeneveld, Gert-Jan Blomquist, Byron, W Angot, Hélène Archer, Stephen, D Bariteau, Ludovic Beck, Ivo Boyer, Matthew von der Gathen, Peter Helmig, Detlev Howard, Dean Hueber, Jacques Jacobi, Hans-Werner Jokinen, Tuija Laurila, Tiia Posman, Kevin, M Quéléver, Lauriane Schmale, Julia Shupe, Matthew, D Krol, Maarten, C |
author_sort |
Barten, Johannes, G M |
title |
Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
title_short |
Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
title_full |
Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
title_fullStr |
Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
title_full_unstemmed |
Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget |
title_sort |
low ozone dry deposition rates to sea ice during the mosaic field campaign: implications for the arctic boundary layer ozone budget |
publisher |
HAL CCSD |
publishDate |
2023 |
url |
https://hal.science/hal-04292739 https://hal.science/hal-04292739/document https://hal.science/hal-04292739/file/Bartenetal_Elementa2023.pdf https://doi.org/10.1525/elementa.2022.00086 |
geographic |
Arctic |
geographic_facet |
Arctic |
genre |
Arctic Sea ice |
genre_facet |
Arctic Sea ice |
op_source |
EISSN: 2325-1026 Elementa: Science of the Anthropocene https://hal.science/hal-04292739 Elementa: Science of the Anthropocene, 2023, 11 (1), pp.00086. ⟨10.1525/elementa.2022.00086⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.1525/elementa.2022.00086 hal-04292739 https://hal.science/hal-04292739 https://hal.science/hal-04292739/document https://hal.science/hal-04292739/file/Bartenetal_Elementa2023.pdf doi:10.1525/elementa.2022.00086 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.1525/elementa.2022.00086 |
container_title |
Elementa: Science of the Anthropocene |
container_volume |
11 |
container_issue |
1 |
_version_ |
1788058602417684480 |
spelling |
ftccsdartic:oai:HAL:hal-04292739v1 2024-01-14T10:03:57+01:00 Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget Barten, Johannes, G M Ganzeveld, Laurens, N Steeneveld, Gert-Jan Blomquist, Byron, W Angot, Hélène Archer, Stephen, D Bariteau, Ludovic Beck, Ivo Boyer, Matthew von der Gathen, Peter Helmig, Detlev Howard, Dean Hueber, Jacques Jacobi, Hans-Werner Jokinen, Tuija Laurila, Tiia Posman, Kevin, M Quéléver, Lauriane Schmale, Julia Shupe, Matthew, D Krol, Maarten, C Ecole Polytechnique Fédérale de Lausanne (EPFL) University of Colorado Boulder Institut des Géosciences de l’Environnement (IGE) Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ) Université Grenoble Alpes (UGA) 2023-02-15 https://hal.science/hal-04292739 https://hal.science/hal-04292739/document https://hal.science/hal-04292739/file/Bartenetal_Elementa2023.pdf https://doi.org/10.1525/elementa.2022.00086 en eng HAL CCSD University of California Press info:eu-repo/semantics/altIdentifier/doi/10.1525/elementa.2022.00086 hal-04292739 https://hal.science/hal-04292739 https://hal.science/hal-04292739/document https://hal.science/hal-04292739/file/Bartenetal_Elementa2023.pdf doi:10.1525/elementa.2022.00086 info:eu-repo/semantics/OpenAccess EISSN: 2325-1026 Elementa: Science of the Anthropocene https://hal.science/hal-04292739 Elementa: Science of the Anthropocene, 2023, 11 (1), pp.00086. ⟨10.1525/elementa.2022.00086⟩ Ozone deposition Arctic ozone Modelling Atmospheric boundary layer [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces environment [SDU.STU.GL]Sciences of the Universe [physics]/Earth Sciences/Glaciology info:eu-repo/semantics/article Journal articles 2023 ftccsdartic https://doi.org/10.1525/elementa.2022.00086 2023-12-16T23:42:22Z Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-round flux and concentration observations from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) campaign and simulations with a single-column atmospheric chemistry and meteorological model (SCM). Based on eddy-covariance O3 surface flux observations, we find a median surface resistance on the order of 20,000 s m−1, resulting in a dry deposition velocity of approximately 0.005 cm s−1. This surface resistance is up to an order of magnitude larger than traditionally used values in many atmospheric chemistry and transport models. The SCM is able to accurately represent the yearly cycle, with maxima above 40 ppb in the winter and minima around 15 ppb at the end of summer. However, the observed springtime ozone depletion events are not captured by the SCM. In winter, the modelled PBL O3 budget is governed by dry deposition at the surface mostly compensated by downward turbulent transport of O3 towards the surface. Advection, which is accounted for implicitly by nudging to reanalysis data, poses a substantial, mostly negative, contribution to the simulated PBL O3 budget in summer. During episodes with low wind speed (<5 m s−1) and shallow PBL (<50 m), the 7-day mean dry deposition removal rate can reach up to 1.0 ppb h−1. Our study highlights the importance of an accurate description of dry deposition to Arctic sea ice in models to quantify the current and future O3 sink in the Arctic, impacting the tropospheric O3 budget, which has been modified in the last century largely due to anthropogenic activities. Article in Journal/Newspaper Arctic Sea ice Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) Arctic Elementa: Science of the Anthropocene 11 1 |