The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign
International audience Measurements of individual NO y components were carried out at Halley station in coastal Antarctica. The measurements were made as part of the CHABLIS campaign (Chemistry of the Antarctic Boundary Layer and the Interface with Snow) and cover over half a year, from austral wint...
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ftccsdartic:oai:HAL:hal-00302680v1 2023-11-12T04:05:09+01:00 The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign Jones, A. E. Wolff, E. W. Ames, D. Bauguitte, S. J.-B. Clemitshaw, K. C. Fleming, Z. Mills, G. P. Saiz-Lopez, A. Salmon, R. A. Sturges, W. T. Worton, D. R. British Antarctic Survey (BAS) Natural Environment Research Council (NERC) Dept. of Environmental Science and Technology Imperial College of Science School of Environmental Sciences Norwich University of East Anglia Norwich (UEA) 2007-03-28 https://hal.science/hal-00302680 https://hal.science/hal-00302680/document https://hal.science/hal-00302680/file/acpd-7-4127-2007.pdf en eng HAL CCSD European Geosciences Union hal-00302680 https://hal.science/hal-00302680 https://hal.science/hal-00302680/document https://hal.science/hal-00302680/file/acpd-7-4127-2007.pdf info:eu-repo/semantics/OpenAccess ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00302680 Atmospheric Chemistry and Physics Discussions, 2007, 7 (2), pp.4127-4163 [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere info:eu-repo/semantics/article Journal articles 2007 ftccsdartic 2023-10-21T23:12:07Z International audience Measurements of individual NO y components were carried out at Halley station in coastal Antarctica. The measurements were made as part of the CHABLIS campaign (Chemistry of the Antarctic Boundary Layer and the Interface with Snow) and cover over half a year, from austral winter 2004 through to austral summer 2005. They are the longest duration and most extensive NO y budget study carried out to date in polar regions. Results show clear dominance of organic NO y compounds (PAN and MeONO 2 ) during the winter months, with low concentrations of inorganic NO y , but a reversal of this situation towards summer when the balance shifts in favour of inorganic NO y . Multi-seasonal measurements of surface snow nitrate correlate strongly with inorganic NO y species. One case study in August suggested that particulate nitrate was the dominant source of nitrate to the snowpack, but this was not the consistent picture throughout the measurement period. An analysis of NO x production rates showed that emissions of NO x from the snowpack dominate over gas-phase sources of "new NO x ", suggesting that, for certain periods in the past, the flux of NO x into the boundary layer can be calculated from ice core nitrate data. Article in Journal/Newspaper Antarc* Antarctic Antarctica ice core Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) Antarctic Austral Halley Station ENVELOPE(-26.541,-26.541,-75.581,-75.581) The Antarctic |
institution |
Open Polar |
collection |
Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) |
op_collection_id |
ftccsdartic |
language |
English |
topic |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
spellingShingle |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere Jones, A. E. Wolff, E. W. Ames, D. Bauguitte, S. J.-B. Clemitshaw, K. C. Fleming, Z. Mills, G. P. Saiz-Lopez, A. Salmon, R. A. Sturges, W. T. Worton, D. R. The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
topic_facet |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
description |
International audience Measurements of individual NO y components were carried out at Halley station in coastal Antarctica. The measurements were made as part of the CHABLIS campaign (Chemistry of the Antarctic Boundary Layer and the Interface with Snow) and cover over half a year, from austral winter 2004 through to austral summer 2005. They are the longest duration and most extensive NO y budget study carried out to date in polar regions. Results show clear dominance of organic NO y compounds (PAN and MeONO 2 ) during the winter months, with low concentrations of inorganic NO y , but a reversal of this situation towards summer when the balance shifts in favour of inorganic NO y . Multi-seasonal measurements of surface snow nitrate correlate strongly with inorganic NO y species. One case study in August suggested that particulate nitrate was the dominant source of nitrate to the snowpack, but this was not the consistent picture throughout the measurement period. An analysis of NO x production rates showed that emissions of NO x from the snowpack dominate over gas-phase sources of "new NO x ", suggesting that, for certain periods in the past, the flux of NO x into the boundary layer can be calculated from ice core nitrate data. |
author2 |
British Antarctic Survey (BAS) Natural Environment Research Council (NERC) Dept. of Environmental Science and Technology Imperial College of Science School of Environmental Sciences Norwich University of East Anglia Norwich (UEA) |
format |
Article in Journal/Newspaper |
author |
Jones, A. E. Wolff, E. W. Ames, D. Bauguitte, S. J.-B. Clemitshaw, K. C. Fleming, Z. Mills, G. P. Saiz-Lopez, A. Salmon, R. A. Sturges, W. T. Worton, D. R. |
author_facet |
Jones, A. E. Wolff, E. W. Ames, D. Bauguitte, S. J.-B. Clemitshaw, K. C. Fleming, Z. Mills, G. P. Saiz-Lopez, A. Salmon, R. A. Sturges, W. T. Worton, D. R. |
author_sort |
Jones, A. E. |
title |
The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
title_short |
The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
title_full |
The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
title_fullStr |
The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
title_full_unstemmed |
The multi-seasonal NO y budget in coastal Antarctica and its link with surface snow and ice core nitrate: results from the CHABLIS campaign |
title_sort |
multi-seasonal no y budget in coastal antarctica and its link with surface snow and ice core nitrate: results from the chablis campaign |
publisher |
HAL CCSD |
publishDate |
2007 |
url |
https://hal.science/hal-00302680 https://hal.science/hal-00302680/document https://hal.science/hal-00302680/file/acpd-7-4127-2007.pdf |
long_lat |
ENVELOPE(-26.541,-26.541,-75.581,-75.581) |
geographic |
Antarctic Austral Halley Station The Antarctic |
geographic_facet |
Antarctic Austral Halley Station The Antarctic |
genre |
Antarc* Antarctic Antarctica ice core |
genre_facet |
Antarc* Antarctic Antarctica ice core |
op_source |
ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00302680 Atmospheric Chemistry and Physics Discussions, 2007, 7 (2), pp.4127-4163 |
op_relation |
hal-00302680 https://hal.science/hal-00302680 https://hal.science/hal-00302680/document https://hal.science/hal-00302680/file/acpd-7-4127-2007.pdf |
op_rights |
info:eu-repo/semantics/OpenAccess |
_version_ |
1782341898143268864 |