On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments
International audience The growth properties of nucleation mode particles were investigated. The variation of source rates of condensable vapors in different locations and environmental conditions was analyzed. The measurements were performed in background stations in Antarctica and in Finnish Lapla...
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ftccsdartic:oai:HAL:hal-00301483v1 2023-12-03T10:13:23+01:00 On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments Kulmala, M. Petäjä, T. Mönkkönen, P. Koponen, I. K. Dal Maso, M. Aalto, P. P. Lehtinen, K. E. J. Kerminen, V.-M. Department of Physics Helsinki Falculty of Science Helsinki Helsingin yliopisto = Helsingfors universitet = University of Helsinki-Helsingin yliopisto = Helsingfors universitet = University of Helsinki Finnish Meteorological Institute (FMI) 2004-10-29 https://hal.science/hal-00301483 https://hal.science/hal-00301483/document https://hal.science/hal-00301483/file/acpd-4-6943-2004.pdf en eng HAL CCSD European Geosciences Union hal-00301483 https://hal.science/hal-00301483 https://hal.science/hal-00301483/document https://hal.science/hal-00301483/file/acpd-4-6943-2004.pdf info:eu-repo/semantics/OpenAccess ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00301483 Atmospheric Chemistry and Physics Discussions, 2004, 4 (5), pp.6943-6966 [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere info:eu-repo/semantics/article Journal articles 2004 ftccsdartic 2023-11-04T23:55:07Z International audience The growth properties of nucleation mode particles were investigated. The variation of source rates of condensable vapors in different locations and environmental conditions was analyzed. The measurements were performed in background stations in Antarctica and in Finnish Lapland and Boreal Forest stations (SMEAR I and SMEAR II) as well as in polluted urban sites in Athens, Marseille and New Delhi. Taking advantage of only the measured aerosol particles spectral evolution as a function of time the formation and growth properties of nucleation mode aerosols have been evaluated. The diameter growth-rate and condensation sink have been obtained from the measured size distribution dynamics. Using this growth rate and condensation sink, the concentration of condensable vapours and their source rate have been estimated. The growth rates and condensation sinks were between 0.3?20 nm h ?1 and 10 ?4 ?0.07 s ?1 , respectively. The corresponding source rate of condensable vapors varied more than 4 orders of magnitude from 10 3 to over 10 7 cm ?1 s ?1 . The highest condensation sink and source rate values were observed in New Delhi and the smallest values in Antarctica. Article in Journal/Newspaper Antarc* Antarctica Lapland Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) |
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Open Polar |
collection |
Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) |
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ftccsdartic |
language |
English |
topic |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
spellingShingle |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere Kulmala, M. Petäjä, T. Mönkkönen, P. Koponen, I. K. Dal Maso, M. Aalto, P. P. Lehtinen, K. E. J. Kerminen, V.-M. On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
topic_facet |
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere |
description |
International audience The growth properties of nucleation mode particles were investigated. The variation of source rates of condensable vapors in different locations and environmental conditions was analyzed. The measurements were performed in background stations in Antarctica and in Finnish Lapland and Boreal Forest stations (SMEAR I and SMEAR II) as well as in polluted urban sites in Athens, Marseille and New Delhi. Taking advantage of only the measured aerosol particles spectral evolution as a function of time the formation and growth properties of nucleation mode aerosols have been evaluated. The diameter growth-rate and condensation sink have been obtained from the measured size distribution dynamics. Using this growth rate and condensation sink, the concentration of condensable vapours and their source rate have been estimated. The growth rates and condensation sinks were between 0.3?20 nm h ?1 and 10 ?4 ?0.07 s ?1 , respectively. The corresponding source rate of condensable vapors varied more than 4 orders of magnitude from 10 3 to over 10 7 cm ?1 s ?1 . The highest condensation sink and source rate values were observed in New Delhi and the smallest values in Antarctica. |
author2 |
Department of Physics Helsinki Falculty of Science Helsinki Helsingin yliopisto = Helsingfors universitet = University of Helsinki-Helsingin yliopisto = Helsingfors universitet = University of Helsinki Finnish Meteorological Institute (FMI) |
format |
Article in Journal/Newspaper |
author |
Kulmala, M. Petäjä, T. Mönkkönen, P. Koponen, I. K. Dal Maso, M. Aalto, P. P. Lehtinen, K. E. J. Kerminen, V.-M. |
author_facet |
Kulmala, M. Petäjä, T. Mönkkönen, P. Koponen, I. K. Dal Maso, M. Aalto, P. P. Lehtinen, K. E. J. Kerminen, V.-M. |
author_sort |
Kulmala, M. |
title |
On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
title_short |
On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
title_full |
On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
title_fullStr |
On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
title_full_unstemmed |
On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
title_sort |
on the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments |
publisher |
HAL CCSD |
publishDate |
2004 |
url |
https://hal.science/hal-00301483 https://hal.science/hal-00301483/document https://hal.science/hal-00301483/file/acpd-4-6943-2004.pdf |
genre |
Antarc* Antarctica Lapland |
genre_facet |
Antarc* Antarctica Lapland |
op_source |
ISSN: 1680-7367 EISSN: 1680-7375 Atmospheric Chemistry and Physics Discussions https://hal.science/hal-00301483 Atmospheric Chemistry and Physics Discussions, 2004, 4 (5), pp.6943-6966 |
op_relation |
hal-00301483 https://hal.science/hal-00301483 https://hal.science/hal-00301483/document https://hal.science/hal-00301483/file/acpd-4-6943-2004.pdf |
op_rights |
info:eu-repo/semantics/OpenAccess |
_version_ |
1784260130118828032 |