Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?

International audience This study provides dissolved and particulate 230Th and 232Th results as well as particulate 234Th data collected during expeditions to the central Arctic Ocean (GEOTRACES, an international project to identify processes and quantify fluxes that control the distributions of tra...

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Published in:Ocean Science
Main Authors: Valk, Ole, Rutgers Van Der Loeff, Michiel, Geibert, Walter, Gdaniec, Sandra, Moran, S. Bradley, Lepore, Kate, Edwards, Robert Lawrence, Lu, Yanbin, Puigcorbe, Viena, Casacuberta, Nuria, Paffrath, Ronja, Smethie, William, Roy-Barman, Matthieu
Other Authors: Alfred Wegener Institute for Polar and Marine Research (AWI), Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung (AWI), Stockholm University, University of Alaska Fairbanks (UAF), Mount Holyoke College, University of Minnesota System, Nanyang Technological University Singapour, Edith Cowan University (ECU), Commonwealth Scientific and Industrial Research Organisation Canberra (CSIRO)-Planning and Transport Research Centre (PATREC), Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology Zürich (ETH Zürich), University of Oldenburg, Lamont-Doherty Earth Observatory (LDEO), Columbia University New York, Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Géochimie Des Impacts (GEDI), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)
Format: Article in Journal/Newspaper
Language:English
Published: HAL CCSD 2020
Subjects:
Online Access:https://hal-cea.archives-ouvertes.fr/cea-02614695
https://hal-cea.archives-ouvertes.fr/cea-02614695/document
https://hal-cea.archives-ouvertes.fr/cea-02614695/file/os-16-221-2020.pdf
https://doi.org/10.5194/os-16-221-2020
id ftccsdartic:oai:HAL:cea-02614695v1
record_format openpolar
institution Open Polar
collection Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe)
op_collection_id ftccsdartic
language English
topic Panoply
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean
Atmosphere
[SDU.STU.OC]Sciences of the Universe [physics]/Earth Sciences/Oceanography
spellingShingle Panoply
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean
Atmosphere
[SDU.STU.OC]Sciences of the Universe [physics]/Earth Sciences/Oceanography
Valk, Ole
Rutgers Van Der Loeff, Michiel
Geibert, Walter
Gdaniec, Sandra
Moran, S. Bradley
Lepore, Kate
Edwards, Robert Lawrence
Lu, Yanbin
Puigcorbe, Viena
Casacuberta, Nuria
Paffrath, Ronja
Smethie, William
Roy-Barman, Matthieu
Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
topic_facet Panoply
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean
Atmosphere
[SDU.STU.OC]Sciences of the Universe [physics]/Earth Sciences/Oceanography
description International audience This study provides dissolved and particulate 230Th and 232Th results as well as particulate 234Th data collected during expeditions to the central Arctic Ocean (GEOTRACES, an international project to identify processes and quantify fluxes that control the distributions of trace elements; sections GN04 and GIPY11). Constructing a time series of dissolved 230Th from 1991 to 2015 enables the identification of processes that control the temporal development of 230Th distributions in the Amundsen Basin. After 2007, 230Th concentrations decreased significantly over the entire water column, particularly between 300 and 1500 m. This decrease is accompanied by a circulation change, evidenced by a concomitant increase in salinity. A potentially increased inflow of water of Atlantic origin with low dissolved 230Th concentrations leads to the observed depletion in dissolved 230Th in the central Arctic. Because atmospherically derived tracers (chlorofluorocarbon (CFC), sulfur hexafluoride (SF6)) do not reveal an increase in ventilation rate, it is suggested that these interior waters have undergone enhanced scavenging of Th during transit from Fram Strait and the Barents Sea to the central Amundsen Basin. The 230Th depletion propagates downward in the water column by settling particles and reversible scavenging.
author2 Alfred Wegener Institute for Polar and Marine Research (AWI)
Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung (AWI)
Stockholm University
University of Alaska Fairbanks (UAF)
Mount Holyoke College
University of Minnesota System
Nanyang Technological University Singapour
Edith Cowan University (ECU)
Commonwealth Scientific and Industrial Research Organisation Canberra (CSIRO)-Planning and Transport Research Centre (PATREC)
Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology Zürich (ETH Zürich)
University of Oldenburg
Lamont-Doherty Earth Observatory (LDEO)
Columbia University New York
Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE)
Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)
Géochimie Des Impacts (GEDI)
Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)
format Article in Journal/Newspaper
author Valk, Ole
Rutgers Van Der Loeff, Michiel
Geibert, Walter
Gdaniec, Sandra
Moran, S. Bradley
Lepore, Kate
Edwards, Robert Lawrence
Lu, Yanbin
Puigcorbe, Viena
Casacuberta, Nuria
Paffrath, Ronja
Smethie, William
Roy-Barman, Matthieu
author_facet Valk, Ole
Rutgers Van Der Loeff, Michiel
Geibert, Walter
Gdaniec, Sandra
Moran, S. Bradley
Lepore, Kate
Edwards, Robert Lawrence
Lu, Yanbin
Puigcorbe, Viena
Casacuberta, Nuria
Paffrath, Ronja
Smethie, William
Roy-Barman, Matthieu
author_sort Valk, Ole
title Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
title_short Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
title_full Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
title_fullStr Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
title_full_unstemmed Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf?
title_sort decrease in 230th in the amundsen basin since 2007: far-field effect of increased scavenging on the shelf?
publisher HAL CCSD
publishDate 2020
url https://hal-cea.archives-ouvertes.fr/cea-02614695
https://hal-cea.archives-ouvertes.fr/cea-02614695/document
https://hal-cea.archives-ouvertes.fr/cea-02614695/file/os-16-221-2020.pdf
https://doi.org/10.5194/os-16-221-2020
long_lat ENVELOPE(74.000,74.000,87.000,87.000)
geographic Amundsen Basin
Arctic
Arctic Ocean
Barents Sea
geographic_facet Amundsen Basin
Arctic
Arctic Ocean
Barents Sea
genre amundsen basin
Arctic
Arctic Ocean
Barents Sea
Fram Strait
genre_facet amundsen basin
Arctic
Arctic Ocean
Barents Sea
Fram Strait
op_source ISSN: 1812-0784
EISSN: 1812-0792
Ocean Science
https://hal-cea.archives-ouvertes.fr/cea-02614695
Ocean Science, European Geosciences Union, 2020, 16 (1), pp.221-234. ⟨10.5194/os-16-221-2020⟩
op_relation info:eu-repo/semantics/altIdentifier/doi/10.5194/os-16-221-2020
cea-02614695
https://hal-cea.archives-ouvertes.fr/cea-02614695
https://hal-cea.archives-ouvertes.fr/cea-02614695/document
https://hal-cea.archives-ouvertes.fr/cea-02614695/file/os-16-221-2020.pdf
doi:10.5194/os-16-221-2020
op_rights http://creativecommons.org/licenses/by/
info:eu-repo/semantics/OpenAccess
op_doi https://doi.org/10.5194/os-16-221-2020
container_title Ocean Science
container_volume 16
container_issue 1
container_start_page 221
op_container_end_page 234
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spelling ftccsdartic:oai:HAL:cea-02614695v1 2023-05-15T13:22:39+02:00 Decrease in 230Th in the Amundsen Basin since 2007: far-field effect of increased scavenging on the shelf? Valk, Ole Rutgers Van Der Loeff, Michiel Geibert, Walter Gdaniec, Sandra Moran, S. Bradley Lepore, Kate Edwards, Robert Lawrence Lu, Yanbin Puigcorbe, Viena Casacuberta, Nuria Paffrath, Ronja Smethie, William Roy-Barman, Matthieu Alfred Wegener Institute for Polar and Marine Research (AWI) Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung (AWI) Stockholm University University of Alaska Fairbanks (UAF) Mount Holyoke College University of Minnesota System Nanyang Technological University Singapour Edith Cowan University (ECU) Commonwealth Scientific and Industrial Research Organisation Canberra (CSIRO)-Planning and Transport Research Centre (PATREC) Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology Zürich (ETH Zürich) University of Oldenburg Lamont-Doherty Earth Observatory (LDEO) Columbia University New York Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE) Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ) Géochimie Des Impacts (GEDI) Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ) 2020 https://hal-cea.archives-ouvertes.fr/cea-02614695 https://hal-cea.archives-ouvertes.fr/cea-02614695/document https://hal-cea.archives-ouvertes.fr/cea-02614695/file/os-16-221-2020.pdf https://doi.org/10.5194/os-16-221-2020 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/os-16-221-2020 cea-02614695 https://hal-cea.archives-ouvertes.fr/cea-02614695 https://hal-cea.archives-ouvertes.fr/cea-02614695/document https://hal-cea.archives-ouvertes.fr/cea-02614695/file/os-16-221-2020.pdf doi:10.5194/os-16-221-2020 http://creativecommons.org/licenses/by/ info:eu-repo/semantics/OpenAccess ISSN: 1812-0784 EISSN: 1812-0792 Ocean Science https://hal-cea.archives-ouvertes.fr/cea-02614695 Ocean Science, European Geosciences Union, 2020, 16 (1), pp.221-234. ⟨10.5194/os-16-221-2020⟩ Panoply [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere [SDU.STU.OC]Sciences of the Universe [physics]/Earth Sciences/Oceanography info:eu-repo/semantics/article Journal articles 2020 ftccsdartic https://doi.org/10.5194/os-16-221-2020 2021-12-19T00:59:09Z International audience This study provides dissolved and particulate 230Th and 232Th results as well as particulate 234Th data collected during expeditions to the central Arctic Ocean (GEOTRACES, an international project to identify processes and quantify fluxes that control the distributions of trace elements; sections GN04 and GIPY11). Constructing a time series of dissolved 230Th from 1991 to 2015 enables the identification of processes that control the temporal development of 230Th distributions in the Amundsen Basin. After 2007, 230Th concentrations decreased significantly over the entire water column, particularly between 300 and 1500 m. This decrease is accompanied by a circulation change, evidenced by a concomitant increase in salinity. A potentially increased inflow of water of Atlantic origin with low dissolved 230Th concentrations leads to the observed depletion in dissolved 230Th in the central Arctic. Because atmospherically derived tracers (chlorofluorocarbon (CFC), sulfur hexafluoride (SF6)) do not reveal an increase in ventilation rate, it is suggested that these interior waters have undergone enhanced scavenging of Th during transit from Fram Strait and the Barents Sea to the central Amundsen Basin. The 230Th depletion propagates downward in the water column by settling particles and reversible scavenging. Article in Journal/Newspaper amundsen basin Arctic Arctic Ocean Barents Sea Fram Strait Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe) Amundsen Basin ENVELOPE(74.000,74.000,87.000,87.000) Arctic Arctic Ocean Barents Sea Ocean Science 16 1 221 234