Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship
Abstract Permafrost thawing as a result of global warming is expected to foster the biological remineralization of intact organic carbon and nitrogen and release greenhouse gas (GHG) into the atmosphere, which will have positive feedback for future global warming. However, GHG budgets and their cont...
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crwiley:10.1002/ppp.2176 2024-09-15T18:11:28+00:00 Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship Yang, Ji‐Woong Ahn, Jinho Iwahana, Go Ko, Nayeon Kim, Ji‐Hoon Kim, Kyungmin Fedorov, Alexander Han, Sangyoung National Research Foundation of Korea 2022 http://dx.doi.org/10.1002/ppp.2176 https://onlinelibrary.wiley.com/doi/pdf/10.1002/ppp.2176 https://onlinelibrary.wiley.com/doi/full-xml/10.1002/ppp.2176 en eng Wiley http://onlinelibrary.wiley.com/termsAndConditions#vor Permafrost and Periglacial Processes volume 34, issue 1, page 122-141 ISSN 1045-6740 1099-1530 journal-article 2022 crwiley https://doi.org/10.1002/ppp.2176 2024-07-25T04:19:47Z Abstract Permafrost thawing as a result of global warming is expected to foster the biological remineralization of intact organic carbon and nitrogen and release greenhouse gas (GHG) into the atmosphere, which will have positive feedback for future global warming. However, GHG budgets and their controls in permafrost ground ice are not yet fully understood. This study aims to better understand the control mechanisms of GHG in ground ice by using new gas and chemistry data. In this study, we present new data on carbon dioxide (CO 2 ), methane (CH 4 ), and nitrous oxide (N 2 O) mixing ratios in three different ice wedges, Churapcha, Syrdakh, and Cyuie, located in central Yakutia, Siberia. The GHG mixing ratios in the studied ice wedges range from 0.0% to 13.8% CO 2 , 1.3–91.2 ppm CH 4 , and 0% and 0–1414 N 2 O. In particular, all three ice wedges demonstrate that ice‐wedge samples enriched in CH 4 were depleted in N 2 O mixing ratios and vice versa. N 2 –O 2 –Ar compositions indicate that the studied ice wedges were most likely formed by dry snow or hoarfrost, not by freezing of snow meltwater, and the O 2 ‐consuming biological metabolism was active. Most of the observed GHG mixing ratios cannot be explained without microbial metabolism. The inhibitory impact of denitrification products of nitrate (including N 2 O) could be an important control of the ice‐wedge CH 4 mixing ratio. Article in Journal/Newspaper Ice permafrost Permafrost and Periglacial Processes wedge* Yakutia Siberia Wiley Online Library Permafrost and Periglacial Processes 34 1 122 141 |
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English |
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Abstract Permafrost thawing as a result of global warming is expected to foster the biological remineralization of intact organic carbon and nitrogen and release greenhouse gas (GHG) into the atmosphere, which will have positive feedback for future global warming. However, GHG budgets and their controls in permafrost ground ice are not yet fully understood. This study aims to better understand the control mechanisms of GHG in ground ice by using new gas and chemistry data. In this study, we present new data on carbon dioxide (CO 2 ), methane (CH 4 ), and nitrous oxide (N 2 O) mixing ratios in three different ice wedges, Churapcha, Syrdakh, and Cyuie, located in central Yakutia, Siberia. The GHG mixing ratios in the studied ice wedges range from 0.0% to 13.8% CO 2 , 1.3–91.2 ppm CH 4 , and 0% and 0–1414 N 2 O. In particular, all three ice wedges demonstrate that ice‐wedge samples enriched in CH 4 were depleted in N 2 O mixing ratios and vice versa. N 2 –O 2 –Ar compositions indicate that the studied ice wedges were most likely formed by dry snow or hoarfrost, not by freezing of snow meltwater, and the O 2 ‐consuming biological metabolism was active. Most of the observed GHG mixing ratios cannot be explained without microbial metabolism. The inhibitory impact of denitrification products of nitrate (including N 2 O) could be an important control of the ice‐wedge CH 4 mixing ratio. |
author2 |
National Research Foundation of Korea |
format |
Article in Journal/Newspaper |
author |
Yang, Ji‐Woong Ahn, Jinho Iwahana, Go Ko, Nayeon Kim, Ji‐Hoon Kim, Kyungmin Fedorov, Alexander Han, Sangyoung |
spellingShingle |
Yang, Ji‐Woong Ahn, Jinho Iwahana, Go Ko, Nayeon Kim, Ji‐Hoon Kim, Kyungmin Fedorov, Alexander Han, Sangyoung Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
author_facet |
Yang, Ji‐Woong Ahn, Jinho Iwahana, Go Ko, Nayeon Kim, Ji‐Hoon Kim, Kyungmin Fedorov, Alexander Han, Sangyoung |
author_sort |
Yang, Ji‐Woong |
title |
Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
title_short |
Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
title_full |
Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
title_fullStr |
Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
title_full_unstemmed |
Origin of CO 2 , CH 4 , and N 2 O trapped in ice wedges in central Yakutia and their relationship |
title_sort |
origin of co 2 , ch 4 , and n 2 o trapped in ice wedges in central yakutia and their relationship |
publisher |
Wiley |
publishDate |
2022 |
url |
http://dx.doi.org/10.1002/ppp.2176 https://onlinelibrary.wiley.com/doi/pdf/10.1002/ppp.2176 https://onlinelibrary.wiley.com/doi/full-xml/10.1002/ppp.2176 |
genre |
Ice permafrost Permafrost and Periglacial Processes wedge* Yakutia Siberia |
genre_facet |
Ice permafrost Permafrost and Periglacial Processes wedge* Yakutia Siberia |
op_source |
Permafrost and Periglacial Processes volume 34, issue 1, page 122-141 ISSN 1045-6740 1099-1530 |
op_rights |
http://onlinelibrary.wiley.com/termsAndConditions#vor |
op_doi |
https://doi.org/10.1002/ppp.2176 |
container_title |
Permafrost and Periglacial Processes |
container_volume |
34 |
container_issue |
1 |
container_start_page |
122 |
op_container_end_page |
141 |
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1810449055802720256 |