Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water

Abstract This paper reports an experimental study of methane hydrate crystallization, crystallization and dissociation cycles are performed in an isothermal and isobaric pressurised stirred reactor. Both methane gas consumption and methane hydrate particles population size distribution (PSD) (calcul...

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Published in:The Canadian Journal of Chemical Engineering
Main Authors: Pic, Jean‐Stéphane, Herri, Jean‐Michel, Cournil, Michel
Format: Article in Journal/Newspaper
Language:English
Published: Wiley 2001
Subjects:
Online Access:http://dx.doi.org/10.1002/cjce.5450790310
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spelling crwiley:10.1002/cjce.5450790310 2024-06-02T08:10:23+00:00 Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water Pic, Jean‐Stéphane Herri, Jean‐Michel Cournil, Michel 2001 http://dx.doi.org/10.1002/cjce.5450790310 https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fcjce.5450790310 https://onlinelibrary.wiley.com/doi/pdf/10.1002/cjce.5450790310 en eng Wiley http://onlinelibrary.wiley.com/termsAndConditions#vor The Canadian Journal of Chemical Engineering volume 79, issue 3, page 374-383 ISSN 0008-4034 1939-019X journal-article 2001 crwiley https://doi.org/10.1002/cjce.5450790310 2024-05-03T10:45:30Z Abstract This paper reports an experimental study of methane hydrate crystallization, crystallization and dissociation cycles are performed in an isothermal and isobaric pressurised stirred reactor. Both methane gas consumption and methane hydrate particles population size distribution (PSD) (calculated from turbidimetric measurements) are recorded. The influence of pressure, stirring and two kinetic inhibitors (PVP and FXAP) is quantified. The crucial moment of the additive introduction (dissolved before or injected during crystallization) is particularly focused on. Finally, the bases of a kinetic inhibition model are raised, introducing a dead zone for crystal nucleation and growth.' Article in Journal/Newspaper Methane hydrate Wiley Online Library The Canadian Journal of Chemical Engineering 79 3 374 383
institution Open Polar
collection Wiley Online Library
op_collection_id crwiley
language English
description Abstract This paper reports an experimental study of methane hydrate crystallization, crystallization and dissociation cycles are performed in an isothermal and isobaric pressurised stirred reactor. Both methane gas consumption and methane hydrate particles population size distribution (PSD) (calculated from turbidimetric measurements) are recorded. The influence of pressure, stirring and two kinetic inhibitors (PVP and FXAP) is quantified. The crucial moment of the additive introduction (dissolved before or injected during crystallization) is particularly focused on. Finally, the bases of a kinetic inhibition model are raised, introducing a dead zone for crystal nucleation and growth.'
format Article in Journal/Newspaper
author Pic, Jean‐Stéphane
Herri, Jean‐Michel
Cournil, Michel
spellingShingle Pic, Jean‐Stéphane
Herri, Jean‐Michel
Cournil, Michel
Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
author_facet Pic, Jean‐Stéphane
Herri, Jean‐Michel
Cournil, Michel
author_sort Pic, Jean‐Stéphane
title Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
title_short Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
title_full Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
title_fullStr Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
title_full_unstemmed Experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
title_sort experimental influence of kinetic inhibitors on methane hydrate particle size distribution during batch crystallization in water
publisher Wiley
publishDate 2001
url http://dx.doi.org/10.1002/cjce.5450790310
https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fcjce.5450790310
https://onlinelibrary.wiley.com/doi/pdf/10.1002/cjce.5450790310
genre Methane hydrate
genre_facet Methane hydrate
op_source The Canadian Journal of Chemical Engineering
volume 79, issue 3, page 374-383
ISSN 0008-4034 1939-019X
op_rights http://onlinelibrary.wiley.com/termsAndConditions#vor
op_doi https://doi.org/10.1002/cjce.5450790310
container_title The Canadian Journal of Chemical Engineering
container_volume 79
container_issue 3
container_start_page 374
op_container_end_page 383
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