High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS
In this paper, we investigate how to achieve high-accuracy radiocarbon measurements by accelerator mass spectrometry (AMS) and present measurement series (performed on archived CO 2 ) of 14 CO 2 between 1985 and 1991 for Point Barrow (Alaska) and the South Pole. We report in detail the measurement p...
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Online Access: | http://dx.doi.org/10.1017/s0033822200038807 https://www.cambridge.org/core/services/aop-cambridge-core/content/view/S0033822200038807 |
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crcambridgeupr:10.1017/s0033822200038807 2024-06-23T07:45:53+00:00 High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS Meijer, H A J Pertuisot, M H van der Plicht, J 2006 http://dx.doi.org/10.1017/s0033822200038807 https://www.cambridge.org/core/services/aop-cambridge-core/content/view/S0033822200038807 en eng Cambridge University Press (CUP) https://www.cambridge.org/core/terms Radiocarbon volume 48, issue 3, page 355-372 ISSN 0033-8222 1945-5755 journal-article 2006 crcambridgeupr https://doi.org/10.1017/s0033822200038807 2024-06-05T04:04:26Z In this paper, we investigate how to achieve high-accuracy radiocarbon measurements by accelerator mass spectrometry (AMS) and present measurement series (performed on archived CO 2 ) of 14 CO 2 between 1985 and 1991 for Point Barrow (Alaska) and the South Pole. We report in detail the measurement plan, the error sources, and the calibration scheme that enabled us to reach a combined uncertainty of better than ±3%. The δ 13 C correction and a suggestion for a span (or 2-point) calibration for the 14 C scale are discussed in detail. In addition, we report new, accurate values for the calibration and reference materials Ox2 and IAEA-C6 with respect to Oxl. The atmospheric 14 CO 2 records (1985–1991) are presented as well and are compared with other existing records for that period. The Point Barrow record agrees very well with the existing Fruholmen (northern Norway) record from the same latitude. The South Pole record shows a small seasonal cycle but with an extreme phase with a maximum on January 1st (±13 days). Together with its generally elevated 14 C level compared to the Neumayer record (coastal Antarctica), this makes our South Pole data set a valuable additional source of information for global carbon cycle modeling using 14 CO 2 as a constraint. Article in Journal/Newspaper Antarc* Antarctica Barrow Northern Norway Point Barrow South pole South pole Alaska Cambridge University Press Neumayer Norway South Pole Radiocarbon 48 3 355 372 |
institution |
Open Polar |
collection |
Cambridge University Press |
op_collection_id |
crcambridgeupr |
language |
English |
description |
In this paper, we investigate how to achieve high-accuracy radiocarbon measurements by accelerator mass spectrometry (AMS) and present measurement series (performed on archived CO 2 ) of 14 CO 2 between 1985 and 1991 for Point Barrow (Alaska) and the South Pole. We report in detail the measurement plan, the error sources, and the calibration scheme that enabled us to reach a combined uncertainty of better than ±3%. The δ 13 C correction and a suggestion for a span (or 2-point) calibration for the 14 C scale are discussed in detail. In addition, we report new, accurate values for the calibration and reference materials Ox2 and IAEA-C6 with respect to Oxl. The atmospheric 14 CO 2 records (1985–1991) are presented as well and are compared with other existing records for that period. The Point Barrow record agrees very well with the existing Fruholmen (northern Norway) record from the same latitude. The South Pole record shows a small seasonal cycle but with an extreme phase with a maximum on January 1st (±13 days). Together with its generally elevated 14 C level compared to the Neumayer record (coastal Antarctica), this makes our South Pole data set a valuable additional source of information for global carbon cycle modeling using 14 CO 2 as a constraint. |
format |
Article in Journal/Newspaper |
author |
Meijer, H A J Pertuisot, M H van der Plicht, J |
spellingShingle |
Meijer, H A J Pertuisot, M H van der Plicht, J High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
author_facet |
Meijer, H A J Pertuisot, M H van der Plicht, J |
author_sort |
Meijer, H A J |
title |
High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
title_short |
High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
title_full |
High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
title_fullStr |
High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
title_full_unstemmed |
High-Accuracy 14 C Measurements for Atmospheric CO 2 Samples by AMS |
title_sort |
high-accuracy 14 c measurements for atmospheric co 2 samples by ams |
publisher |
Cambridge University Press (CUP) |
publishDate |
2006 |
url |
http://dx.doi.org/10.1017/s0033822200038807 https://www.cambridge.org/core/services/aop-cambridge-core/content/view/S0033822200038807 |
geographic |
Neumayer Norway South Pole |
geographic_facet |
Neumayer Norway South Pole |
genre |
Antarc* Antarctica Barrow Northern Norway Point Barrow South pole South pole Alaska |
genre_facet |
Antarc* Antarctica Barrow Northern Norway Point Barrow South pole South pole Alaska |
op_source |
Radiocarbon volume 48, issue 3, page 355-372 ISSN 0033-8222 1945-5755 |
op_rights |
https://www.cambridge.org/core/terms |
op_doi |
https://doi.org/10.1017/s0033822200038807 |
container_title |
Radiocarbon |
container_volume |
48 |
container_issue |
3 |
container_start_page |
355 |
op_container_end_page |
372 |
_version_ |
1802642851939483648 |