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aerosol Arctic size distribution particle size 550 radiative forcing Europe climate modeling comparative study trend analysis concentration (composition) Verlagsveröffentlichung article DATE/TIME 114 Physical sciences Arctic Ocean Arctic Oscillation black carbon observatory Aerosol number concentration Atmosphere Atmosphärische Spurenstoffe Log-normal particle size distribution [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Meteorology and Atmospheric Sciences [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] [SDU.STU.ME]Sciences of the Universe [physics]/Earth Sciences/Meteorology Air chemistry observatory normalized concentration at particle diameter 100.24 nm normalized concentration at particle diameter 112.47 nm